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Weng H.K., Nagakubo A., Ogi H., et al. "Phonon propagation in isotopic diamond superlattices", Physical Review B, 104(5), 054112, 2021. https://doi.org/10.1103/physrevb.104.054112., The out-of-plane thermal conductivity and elastic constant of epitaxial [100] C12/C13 superlattice diamonds with layer thicknesses of 1, 30, and 100 nm are evaluated by picosecond ultrasound spectroscopy. The measured elastic constants of the superlattices are equivalent to those of single-layer diamond thin films. This result confirms our success in synthesizing superlattice specimens with few defects at the interfaces. Therefore, the phonon transport behavior is governed by the mass difference, not the interfacial defects. The measured thermal conductivity of the superlattices is lower than that of a pure C12 isotope diamond thin film. We estimated the lattice thermal conductivity using the lattice dynamics calculation, attributing the lowered thermal conductivity to the decrease in the phonon group velocity in superlattices. We further consider the effect of mini-umklapp scattering in the superlattice, which explains the dependence of the thermal conductivity on the layer thickness. We reveal that the mini-umklapp scattering effect becomes significant only for an isotope diamond superlattice because of the high Debye temperature and large relative mass difference.

Ogi H., Masuda S., Nagakubo A., et al. Physical Review B, 93(2), 024112, 2016. Copyright 2016 by the American Physical Society., Surface waves are often excited by interdigitated transducers consisting of many nanostrips attached on a substrate, and it has been recognized that the mass and stiffness of the attached nanostrips affect surface-wave resonances to some extent. Here, we reveal the more noticeable influence of the interfacial stiffness between strips and substrate at high frequencies. This influence is confirmed by exciting and detecting surface-wave resonances up to ∼6 GHz by picosecond ultrasound spectroscopy. The resonance frequency significantly decreases and attenuation increases as the interfacial stiffness decreases for silicon substrate. However, low-attenuation branches appear along the Rayleigh-wave-resonance dispersion curve for silica substrate, and the resonance frequencies remain nearly identical to those of the Rayleigh waves. Previous models fail to reproduce these surface-wave resonance behaviors. The proposed theoretical model, involving the interfacial stiffness, consistently explained them, indicating the importance of the interface bond strength in designing surface-wave resonators.