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1. Investigation of two-photon absorption behavior in symmetrical acceptor-pi-acceptor derivatives with dimesitylboryl end-groups. Evidence of new engineering routes for TPA/transparency trade-off optimization.

Author

Chariot M, Porrès L, Entwistle CD, Beeby A, Marder TB, and Blanchard-Desce M

Subjects
Boron Compounds chemical synthesis, Molecular Structure, Boron Compounds chemistry, Photons
Abstract

Investigations of the non-linear optical properties of a novel series of A-pi-A quadrupoles, based on dimesitylboron end-groups, reveal the promising potential of elongated vinylboranes derivatives for combined enhanced two-photon absorption cross-section and improved transparency in the visible region. In addition, the excited state lifetime can be significantly enhanced in A-pi-A'-pi-A derivatives. This opens a new route towards optimized molecules for optical power limiting.

Published
2005
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