AbstractThis paper compiles and correlates for the first time Cretaceous to Eocene palynostratigraphies across the Arctic. It focuses on Greenland and adjacent areas, including the Labrador–Baffin Seaway, onshore Nuussuaq Basin in central West Greenland, onshore southern East Greenland, central East Greenland, North-East Greenland, eastern North Greenland and the Danmarkshavn Basin, but also extends to the Canadian Arctic Archipelago and the Barents Sea region offshore Norway. The paper compiles data from more than three decades of detailed Arctic palynological analyses, based mainly on dinoflagellate cysts. It gives a historical overview of the Cretaceous to Paleogene palaeontological studies of Greenland and presents an overview of 85 palynological intervals and numerous bioevents. The palynological assemblages from the Labrador–Baffin Seaway, Nuussuaq Basin and north-east Baffin Bay reflect the opening of the Labrador–Baffin Seaway, from a brackish to freshwater environment in a large embayment in the Early Cretaceous to an open marine seaway in the Late Cretaceous. Assemblages reveal dinoflagellate cyst provincialism between the opening stages of the Labrador–Baffin Seaway and the already opened Greenland–Norwegian–Barents seaway. The Upper Cretaceous global Oceanic Anoxic Event 2 (OAE2) spanning the Cenomanian/Turonian boundary is recognised from Arctic Canada, north-east Baffin Bay, Nuussuaq Basin in central West Greenland, and North-East Greenland, and is mapped and correlated based on dinoflagellate cyst stratigraphy and carbon isotope (δ13Corg) curves. The dinoflagellate cyst assemblages of the Cretaceous/Paleogene boundary are correlated from the Labrador Sea across to the Nuussuaq Basin in central West Greenland; in both areas the earliest Danian palynological assemblage is represented by incoming warm-water species. The presence of the global Paleocene–Eocene Thermal Maximum (PETM) in the Paleogene successions in North-East Greenland and in exploration wells in the Labrador–Baffin Seaway is indicated by the incoming of the warm-water dinoflagellate cyst species Axiodinium augustum. [ABSTRACT FROM AUTHOR]