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We have studied both theoretically and experimentally symmetric and asymmetric planar metallic Split Ring Resonators. We demonstrate that introducing structural asymmetry makes it possible to excite several higher order modes of both even (l = 2) and odd (l = 3, 5) order, which are otherwise inaccessible for a normally incident plane wave in symmetric structures. Experimentally we observe that the even mode resonances of asymmetric resonators have a quality factor 5.8 times higher than the higher order odd resonances. ispartof: Optics Express vol:21 issue:13 pages:15464-15474 ispartof: location:United States status: published

Chirality effects in optical second harmonic generation (SHG) are studied in periodic planar arrays of gold G-shaped nanostructures. We show that G-shaped structures of different handedness demonstrate different SHG efficiency for the left and right circular polarizations, as well as the opposite directions of the SHG polarization plane rotation. The observed effects are interpreted as the appearance of chirality in the SHG response which allows clear distinguishing of two enantiomers.

While it has been demonstrated that, above its resolution limit, Second Harmonic Generation (SHG) microscopy can map chiral local field enhancements, below that limit, structural defects were found to play a major role. Here we show that, even below the resolution limit, the contributions from chiral local field enhancements to the SHG signal can dominate over those by structural defects. We report highly homogeneous SHG micrographs of star-shaped gold nanostructures, where the SHG circular dichroism effect is clearly visible from virtually every single nanostructure. Most likely, size and geometry determine the dominant contributions to the SHG signal in nanostructured systems. (C) 2011 Optical Society of America ispartof: Optics Express vol:20 issue:1 pages:256-264 ispartof: location:United States status: published