1. Scale-invariant magnetic anisotropy in RuCl3 at high magnetic fields
- Author
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Michael Lawler, Ross D. McDonald, Fedor Balakirev, Jon Betts, Maja D. Bachmann, Arkady Shekhter, Dmitry A. Sokolov, Mun Chan, Johanna C. Palmstrom, David Graf, Brad Ramshaw, Jacob Ruff, You Lai, Gregory S. Boebinger, Marcus Schmidt, Kimberly Modic, and Philip J. W. Moll
- Subjects
Physics ,Strongly Correlated Electrons (cond-mat.str-el) ,Condensed matter physics ,media_common.quotation_subject ,FOS: Physical sciences ,General Physics and Astronomy ,Frustration ,Scale invariance ,01 natural sciences ,Inelastic neutron scattering ,010305 fluids & plasmas ,3. Good health ,Magnetic field ,Condensed Matter - Strongly Correlated Electrons ,symbols.namesake ,Magnetic anisotropy ,Lattice (order) ,0103 physical sciences ,symbols ,Quantum spin liquid ,010306 general physics ,Raman spectroscopy ,media_common - Abstract
In RuCl$_3$, inelastic neutron scattering and Raman spectroscopy reveal a continuum of non-spin-wave excitations that persists to high temperature, suggesting the presence of a spin liquid state on a honeycomb lattice. In the context of the Kitaev model, magnetic fields introduce finite interactions between the elementary excitations, and thus the effects of high magnetic fields - comparable to the spin exchange energy scale - must be explored. Here we report measurements of the magnetotropic coefficient - the second derivative of the free energy with respect to magnetic field orientation - over a wide range of magnetic fields and temperatures. We find that magnetic field and temperature compete to determine the magnetic response in a way that is independent of the large intrinsic exchange interaction energy. This emergent scale-invariant magnetic anisotropy provides evidence for a high degree of exchange frustration that favors the formation of a spin liquid state in RuCl$_3$., Comment: arXiv admin note: substantial text overlap with arXiv:1901.09245. Nature Physics
- Published
- 2020