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The raw materials of geopolymer come from industrial wastes, which have the advantages of lower carbon emissions and less energy consumption compared with traditional cement products. However, it still has the disadvantages of low strength, easy cracking, and low production efficiency, which limit its engineering application and development. At present, with the application and development of nanotechnology in the field of materials, it is found that nanomaterials have a good filling effect on composites, which greatly improves the integrity of the composites. It has become a very popular research direction to optimize and improve the engineering application performance of geopolymer concrete (GPC) by nanomaterials. The modification of nanomaterials can further improve the properties of GPC and expand its application fields in engineering and life. Based on people’s strong interest in nanomaterial-modified GPC and providing the latest and complete research status for further related work, this paper summarized the key technical problems in the field of nanomaterials-modified GPC in the past decade. Those include the modification mechanism, dispersion mode, and mechanical properties of nanomaterials. At the same time, the application bottlenecks and key problems of nanomaterials-modified GPC are comprehensively analyzed. Finally, the prospects and challenges of future work in this field are discussed.

For the high demand for cement-based materials in buildings, improving the performance of cement-based materials has become the focus of relevant researchers. In recent years, nanomaterials have broad prospects in many fields such as architecture by virtue of their “lightweight, high strength, and strong solidity” characteristics. As a modifier of cement-based materials, it has also become a research hotspot. Graphene oxide (GO) is one of the most representative graphene-based nanomaterials. Because of its extremely high specific surface area and excellent physical properties, it has greatly improved the properties of cement-based materials. GO acts as an enhancer of cement composites that brings people unlimited imagination. The research progress of GO-modified cement-based materials is reviewed. The purpose is to point out the limitations of current research and provide a reference for later research. The dispersion treatment of GO and the properties of its modified cement-based materials are analyzed and summarized. In addition, the further research work that is needed and future development prospect are discussed.

In the recent decades, traditional concrete poses a great challenge to the modernization of the construction industry because of low tensile strength, poor toughness, and weak resistance to cracking. To overcome these problems, ultra-high performance concrete (UHPC) with superior mechanical properties and durability is developed for broad application prospect in the future engineering construction. However, UHPC is less eco-friendly because it consumes more cement compared with the traditional concrete. The manufacturing of cement produces large amounts of carbon dioxide and therefore leads to the greenhouse effect. Nanomaterials consist of microstructural features that range from 0.1 to 100 nm in size, which exhibit the novel properties different from their bulk counterparts, including filling effect, surface activity, and environmental sustainability. This paper reviews the effect of various nanomaterials used in UHPC to partially replace the cement or as an additive on the microstructures, mechanical properties, and other properties of UHPC. In addition, the limitations and shortcomings of the current research are analyzed and summarized, and development directions are provided for future research on the application of nanomaterials in UHPC.

In recent years, with the higher requirements for the performance of cement-based materials and the call for energy conservation and environmental protection, a wave of research on new materials has set off, and various high-performance concrete and more environmentally friendly geopolymers have appeared in the public. With a view to solving the defects of energy consumption, environmental protection and low toughness of traditional cement-based materials. At the same time, nanomaterials have become a focus of current research. Therefore, the research on the properties of cement-based materials and geopolymers modified by graphene and its derivatives has aroused extensive interest of researchers. Graphene-based nanomaterials are one of them. Because of their large specific surface area, excellent physical properties have been favored by many researchers. This paper reviews the research progress of graphene-based nanomaterials in improving the properties of cement-based materials and geopolymer materials, and points out the main challenges and development prospects of such materials in the construction field in the future.