1. Electronic Structure of Above-Room-Temperature van der Waals Ferromagnet Fe3GaTe2
- Author
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Lee, Ji-Eun, Yan, Shaohua, Oh, Sehoon, Hwang, Jinwoong, Denlinger, Jonathan D, Hwang, Choongyu, Lei, Hechang, Mo, Sung-Kwan, Park, Young, and Ryu, Hyejin
- Subjects
Quantum Physics ,Physical Sciences ,Condensed Matter Physics ,Fe3GaTe2 ,room-temperature vander Waals ferromagnet ,high-T (C) ferromagnet ,electronic structures ,Heisenbergexchange interaction ,magnetic anisotropy energy ,Heisenberg exchange interaction ,high-TC ferromagnet ,room-temperature van der Waals ferromagnet ,Nanoscience & Nanotechnology - Abstract
Fe3GaTe2, a recently discovered van der Waals ferromagnet, demonstrates intrinsic ferromagnetism above room temperature, necessitating a comprehensive investigation of the microscopic origins of its high Curie temperature (TC). In this study, we reveal the electronic structure of Fe3GaTe2 in its ferromagnetic ground state using angle-resolved photoemission spectroscopy and density functional theory calculations. Our results establish a consistent correspondence between the measured band structure and theoretical calculations, underscoring the significant contributions of the Heisenberg exchange interaction (Jex) and magnetic anisotropy energy to the development of the high-TC ferromagnetic ordering in Fe3GaTe2. Intriguingly, we observe substantial modifications to these crucial driving factors through doping, which we attribute to alterations in multiple spin-splitting bands near the Fermi level. These findings provide valuable insights into the underlying electronic structure and its correlation with the emergence of high-TC ferromagnetic ordering in Fe3GaTe2.
- Published
- 2023