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The study focused on technological readiness and computer self-efficacy as predictors of E-learning adoption by Library and Information Science (LIS) students in Nigeria. While literatures have suggested that E-learning adoption is context based, there is a need to examine the predictors of E-learning adoption within the Nigerian context, given the increasing need for E-learning adoption as a result of the COVID-19 Pandemic. As a result, the study used the descriptive correlational research design to study a group of LIS students in Nigeria. Consequently, LIS students in the Nigeria Library and Information Science Students (NLISS) Facebook group were used for the study. The population of the group was 1,807 at the time the study was conducted and the sample size for the study was 320 randomly selected respondents. The sample size was achieved using the Krejcie, R. V., and D. W. Morgan. 1970. "Determining Sample Size for Research Activities." Educational and Psychological Measurement 30: 607–10 table for determining sample size. Data was collected from the respondents using a closed-ended questionnaire consisting of adapted scales for all the variables. The 223 responses retrieved within a period of three weeks were analysed using descriptive and inferential statistics. The findings from the investigation showed technological readiness, computer self-efficacy and E-learning adoption of the LIS students is very high. Though technological readiness and computer self-efficacy had relative contribution to E-learning adoption, computer self-efficacy had higher contribution. The study also revealed that significant relationships exist between technological readiness and E-learning adoption, computer self-efficacy and E-learning adoption, technological readiness and computer self-efficacy, while technological readiness and computer self-efficacy had joint prediction on E-learning adoption by LIS students in Nigeria. The study therefore emphasized the need to consider certain individual factors as criteria to the successful adoption of E-learning among LIS students in Nigeria. [ABSTRACT FROM AUTHOR]