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The authors at ANU were supported by the Australian Research Council. The authors at DSI were supported by DSI core funds and A*STAR SERC Pharos program, Grant 152 73 00025 (Singapore).

Meta-optics based on optically-resonant dielectric nanostructures is a rapidly developing research field with many potential applications. Halide perovskite metasurfaces emerged recently as a novel platform for meta-optics, and they offer unique opportunities for control of light in optoelectronic devices. Here we employ the generalized Kerker conditions to overlap electric and magnetic Mie resonances in each meta-atom of MAPbBr3 perovskite metasurface and demonstrate broadband suppression of reflection down to 4%. We reveal also that metasurface nanostructuring is also beneficial for the enhancement of photoluminescence. Our results may be useful for applications of nanostructured halide perovskites in photovoltaics and semi-transparent multifunctional metadevices where reflection reduction is important for their high efficiency.

Dewetting of thin metal films is one of the most widespread method for functional plasmonic nanostructures fabrication. However, simple thermal-induced dewetting does not allow to control degree of nanostructures order without additional lithographic process steps. Here we propose a novel method for lithography-free and large-scale fabrication of plasmonic nanostructures via controllable femtosecond laser-induced dewetting. The method is based on femtosecond laser surface pattering of a thin film followed by a nanoscale hydrodynamical instability, which is found to be very controllable under specific irradiation conditions. We achieve control over degree of nanostructures order by changing laser irradiation parametrs and film thickness. This allowed us to exploit the method for the broad range of applications: resonant light absorbtion and scattering, sensing, and potential improving of thin-film solar cells.

Plasmonic nanoparticles coupled with metallic films forming nanometer scale cavities have recently emerged as a powerful tool for enhancement of light-matter interaction. Despite high efficiency for sensing and light emission, such nanocavities exhibit harmful and uncontrolled optical heating which limits the ranges of light intensities and working temperature. In contrast to plasmonic nanoparticles, all-dielectric counterparts possess low Ohmic losses, high temperature stability along with a strong temperature-dependent Raman response. Here, we demonstrate that a silicon nanoparticle coupled with a thin gold film can serve as a multifunctional metal-dielectric (hybrid) nanocavity operating up to 1200 K. Resonant interaction of light with such nanocavity enables molecular sensing, heat-induced molecular events (protein unfolding), and their real-time tracing with a nanoscale thermometry through the monitoring enhanced Raman scattering both from the nanoparticle and analyzed molecules. We model numerically the thermo-optical properties of the hybrid nanocavity and reveal two alternative regimes of operation - with and without strong optical heating while other functionalities are preserved. We believe that the concept of the multifunctional hybrid nanocavities holds great potential for diverse photochemical and photophysical applications.

Surface electromagnetic waves are characterized by the intrinsic spin-orbit interaction which results in the fascinating spin-momentum locking. Therefore, directional coupling of light to surface waves can be achieved through chiral nanoantennas. Here, we show that dielectric nanoantenna provides chiral response with strong spectral dependence due to the interference of electric and magnetic dipole momenta when placed in the vicinity of the metal-air interface. Remarkably, chiral behaviour in the proposed scheme does not require elliptical polarization of the pump beam or the geometric chirality of the nanoantenna. We show that the proposed ultracompact and simple dielectric nanoantenna allows for both directional launching of surface plasmon polaritons on a thin gold film and their demultiplexing with a high spectral resolution.