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The contribution of heterogeneous ice nucleation to the formation of cirrus cloud ice crystals is still not well quantified. This results in large uncertainties when predicting cirrus radiative effects and their role in Earth's climate system. The goal of this case study is to simulate the composition, and thus activation conditions, of ice nucleating particles (INPs) to evaluate their contribution to heterogeneous cirrus ice formation in relation to homogeneous ice nucleation. For this, the regional model COSMO—Aerosols and Reactive Trace Gases (COSMO-ART) was used to simulate a synoptic cirrus cloud over Texas on 13 April 2011. The simulated INP composition was then compared to measured ice residual particle (IRP) composition from the actual event obtained during the NASA Midlatitude Airborne Cirrus Properties Experiment (MACPEX) aircraft campaign. These IRP measurements indicated that the dominance of heterogeneous ice nucleation was mainly driven by mineral dust with contributions from a variety of other particle types. Applying realistic activation thresholds and concentrations of airborne transported mineral dust and biomass-burning particles, the model implementing the heterogeneous ice nucleation parameterization scheme of Ullrich et al. is able to reproduce the overall dominating ice formation mechanism in contrast to the model simulation with the scheme of Phillips et al. However, the model showed flaws in reproducing the IRP composition. [ABSTRACT FROM AUTHOR]

A theoretical framework is presented that exposes the radiative-dynamical relationships that govern the subcritical destabilization of African easterly waves (AEWs) by Saharan mineral dust (SMD) aerosols. The framework is built on coupled equations for quasigeostrophic potential vorticity (PV), temperature, and SMD mixing ratio. A perturbation analysis yields, for a subcritical, but otherwise arbitrary, zonal-mean background state, analytical expressions for the growth rate and frequency of theAEWs. The expressions are functions of the domain-averaged wave activity,which is generated by the direct radiative effects of theSMD. Thewave activity is primarily modulated by the Doppler-shifted phase speed and the background gradients in PV and SMD. Using an idealized version of the Weather Research and Forecasting (WRF) Model coupled to an interactive dust model, a linear analysis shows that, for a subcritical African easterly jet (AEJ) and a background SMD distribution that are consistent with observations, the SMD destabilizes the AEWs and slows their westward propagation, in agreement with the theoretical prediction. The SMD-induced growth rates are commensurate with, and can sometimes exceed, those obtained in previous dust-free studies in which the AEWs grow on AEJs that are supercritical with respect to the threshold for barotropic-baroclinic instability. The clarity of the theoretical framework can serve as a tool for understanding and predicting the effects of SMD aerosols on the linear instability of AEWs in subcritical, zonal-mean AEJs. [ABSTRACT FROM AUTHOR]