1. Superparamagnetic relaxation in iron nanoclusters measured by low energy muon spin rotation
- Author
-
Elvezio Morenzoni, A. Hofer, M. Birke, H Glückler, Thomas Prokscha, A Schatz, Hubertus Luetkens, E. M. Forgan, Ch. Niedermayer, H.P Weber, Timothy J. Jackson, T.M Riseman, G. Schatz, Chris Binns, and J Litterst
- Subjects
Magnetization ,Magnetic anisotropy ,Condensed matter physics ,Remanence ,Chemistry ,Relaxation (NMR) ,General Materials Science ,Activation energy ,Muon spin spectroscopy ,Condensed Matter Physics ,Molecular physics ,Nanoclusters ,Superparamagnetism - Abstract
Low energy (16 keV) muons were used to probe the dynamic magnetic behaviour of iron nanoclusters embedded in a silver thin film matrix. The silver film was 500 nm thick and contained a volume fraction of 0.1% iron. Measurements were made in a field of 25 mT, applied normal to the plane of the film, in the temperature range 4.7 K to 300 K. At temperatures above 20 K thermal activation of the cluster moments was seen as a narrowing of the field distribution sensed by the implanted muons. An intrinsic cluster relaxation time of τ0 = 12 ± 4 ns and an activation energy of 51 ± 9 K were deduced from fits to the data. SQUID magnetometry of thicker (1.5 µm) but otherwise identical films on graphite substrates showed the clusters to have a volume of the order of 10-26 m3, from which a cubic anisotropy constant of K = 2.3 ± 0.4 × 105 J m-3 was calculated. Remanence measurements showed no evidence of a preferred orientation for the magnetization of the cluster assembly.
- Published
- 2000
- Full Text
- View/download PDF