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Mn-based hard magnets are potentially suitable for advanced ultra-high frequency spintronics applications because they exhibit the Larmor precession of magnetization at THz wave-range frequencies with low magnetic relaxation. However, the low magnetic relaxation properties are not well understood; thus, a more detailed study is necessary. In this study, magnetization precessions in L10 Mn1.54Ga, D022 Mn2.12Ga, and C38 MnAlGe epitaxial films grown on MgO substrates were investigated using an all-optical pump-probe method under a magnetic field of ~20 kOe. The coherent magnetization precessions at frequencies of more than 0.1, 0.2, and 0.3 THz for the C38 MnAlGe, L10 Mn1.54Ga, and D022 Mn2.12Ga films, respectively, were clearly measured. The effective damping constant for the C38 MnAlGe film was smaller than the previously reported value measured at 10 kOe by a factor of 2, whereas those showed a large angular dependence. The effective damping constants for the L10 Mn1.54Ga and D022 Mn2.12Ga films were independent of the field angle and approximately identical to the values measured at 10 kOe. Thus, it was concluded that the values for the Gilbert damping constant, α, were 0.008 and 0.012 for the L10 Mn1.54Ga and D022 Mn2.12Ga films, respectively. The possible origin of the discrepancy between the experimental and theoretical a values for these films is discussed. [ABSTRACT FROM AUTHOR]

We have fabricated bilayer films of tetragonal Heusler-like D022 Mn3Ga and cubic Heusler Co2FeZ (Z=Si and Al) on (100) single-crystalline MgO substrates and investigated their structural and interfacial exchange coupling. The coupling in the Mn3Ga/Co2FeAl bilayer was either ferromagnetic or antiferromagnetic, depending on annealing temperature, whereas only antiferromagnetic exchange coupling was observed in the Mn3Ga/Co2FeSi bilayers. The effects of annealing on the structure and coupling strength in the bilayers are discussed. [ABSTRACT FROM AUTHOR]

The precessional magnetization dynamics of L10 MnGa/Fe bilayers with a large perpendicular magnetic anisotropy are investigated using vector network analyzer ferromagnetic resonance (VNA-FMR) and time-resolved magneto-optical Kerr effect (TRMOKE). The MnGa/Fe(1 nm) bilayer exhibited perpendicular magnetization and MnGa/Fe(2 and 5 nm) bilayers showed in-plane magnetizations. The VNA-FMR and TRMOKE data for these bilayers are well explained from calculations, based on the coupled Landau-Lifshitz equations, taking into account the interfacial exchange coupling of 2.4 erg/cm². [ABSTRACT FROM AUTHOR]