1. Neutron and x-ray evidence of charge melting in ferromagnetic layered colossal magnetoresistance manganites (invited)
- Author
-
Raymond Osborn, O. H. Seeck, John F. Mitchell, Z. Islam, Joël Mesot, Stephan Rosenkranz, J. W. Lynn, S. K. Sinha, and L. Vasiliu-Doloc
- Subjects
Materials science ,Colossal magnetoresistance ,Magnetoresistance ,Condensed matter physics ,Scattering ,Neutron diffraction ,General Physics and Astronomy ,Antiferromagnetism ,ddc:530 ,Neutron scattering ,Metal–insulator transition ,Polaron - Abstract
Recent x-ray and neutron scattering studies have revealed static diffuse scattering due to polarons in the paramagnetic phase of the colossal magnetoresistive manganites La2-2xSr1+2xMn2O7, with x = 0.40 and 0.44. We show that the polarons exhibit short-range incommensurate correlations that grow with decreasing temperature, but disappear abruptly at the combined ferromagnetic and metal-insulator transition in the x = 0.40 system because of the sudden charge delocalization, while persisting at low temperature in the antiferromagnetic x = 0.44 system. The "melting" of the polaron ordering as we cool through T-C occurs with the collapse of the polaron scattering itself in the x = 0.40 system. This short-range polaron order is characterized by an ordering wave vector q = (0.3,0,1) that is almost independent of x for x greater than or equal to 0.38, and is consistent with a model of disordered stripes. (C) 2001 American Institute of Physics.
- Published
- 2001
- Full Text
- View/download PDF