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An observational program to study variations of the vertical distribution of CO in the Venus atmosphere is presented. Measurements of the J = 0 - 1 absorption line at 2.6 mm wavelength are reported for two phase angles in 1977, one near eastern elongation (February) and the other near inferior conjunction (April). The two spectra are significantly different, with the April absorption line being narrower and deeper. The results of numerical inversion calculations show that the CO mixing ratio increases by a factor of approximately 100 between 78 and 100 km and that the CO abundance above approximately 100 km is greatest on the night-side hemisphere. These conclusions are in qualitative agreement with theoretical models. In addition to the CO observations, a search for other molecules was made to provide further information on the composition of the Venus middle atmosphere. The J = 0 - 1 transition of (C-13)O was detected and upper limits were derived for nine other molecules.

Measurements of Jupiter's disk-temperature spectrum in the 20- to 24-GHz (1.5 cm less than lambda less than 1.25 cm) region are reported. These data are combined with previously published data to produce a uniformly calibrated thermal spectrum of Jupiter in the wavelength interval 0.85 to 2.1 cm. Model studies are carried out to determine optimum pressure-temperature profiles for an assumed radiative-convective temperature structure. It is found that the temperature at the 1-bar total effective pressure level is between 140 and 165 K, with a most probable value of 153 K, provided that NH3 is uniformly saturated in the clouds on a global scale. We show that the temperature profile for the microwave model is approximately 20 K cooler than the profiles derived from infrared data. An explanation of this discrepancy is discussed in terms of a model which invokes different NH3 distributions in the belts and zones.

The theoretical disk brightness temperature spectra for Uranus are computed and compared with the observed microwave spectrum. It is shown that the emission observed at short centimeter wavelengths originates deep below the region where ammonia would ordinarily begin to condense. We demonstrate that this result is inconsistent with a wide range of atmospheric models in which the partial pressure of NH3 is given by the vapor-pressure equation in the upper atmosphere. It is estimated that the ammonia mixing ratio must be less than 10 to the minus 6 in the 150 to 200 K temperature range. This is two orders of magnitude less than the expected mixing ratio based on solar abundances. The evidence for this depletion and a possible explanation are discussed.

Radio observations of Jupiter have been carried out at Goldstone, CA at a wavelength of 13 cm during the oppositions of 1969 and 1971. In 1969, circular-polarization and total-flux measurements were made with a 64-m radio telescope. From May through October 1971, Jupiter's flux density was measured at weekly intervals with a 26-m antenna. The upper limit to the degree of circular polarization over the longitude ranges 10-100 deg and 160-250 deg System III (1957.0) is 1%; the flux data have been used to derive a magnetospheric rotation period which is approximately 0.37 sec longer than the IAU System III (1957.0). The flux-density data define beaming curves which are apparently different from 11-cm beaming curves measured in 1964. Jupiter's peak flux density decreased by 20% between 1964 and 1971, and 8% between 1969 and 1971.