1. Possible nitric acid coating formation over Pinatubo aerosols inferred with a microphysical code: A case study during EASOE
- Author
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Jean-Pierre Wolf, Vincenzo Rizi, Leopoldo Stefanutti, Guido Visconti, Gianluca Redaelli, and Marco Verdecchia
- Subjects
Vulcanian eruption ,Atmospheric sciences ,Aerosol ,chemistry.chemical_compound ,Geophysics ,Atmosphere of Earth ,Lidar ,chemistry ,Nitric acid ,Atmospheric chemistry ,Ozone layer ,General Earth and Planetary Sciences ,Environmental science ,Stratosphere - Abstract
Lidar observations at Sodankyla (Finland) on January 9 and 11 1992, made as part of the European Arctic Stratospheric Ozone Experiment (EASOE), showed very different profiles of backscattering ratio. A prominent layer was seen between potential temperatures of 420 and 445K on January 9, which was nearly absent in the backscattering profile between these isentropic surfaces on the 11th. Examination of the trajectories of the airmasses reaching Sodankyla on these days lead us to suggest that the larger returns on January 9th could arise from the formation of a nitric acid coating on volcanic aerosols. Simulations using a microphysical model produce results consistent with this suggestion. We conclude that nitric acid condensation on January 9 can explain the measurements, but that independent information would be needed to quantify the characteristics of the aerosol substrate.
- Published
- 1994
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