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Magnetospheric substorms drive energetic electron precipitation into the Earth's atmosphere. We use the output from a substorm model to describe electron precipitation forcing of the atmosphere during an active substorm period in April–May 2007. We provide the first estimate of substorm impact on the neutral composition of the polar middle atmosphere. Model simulations show that the enhanced ionization from a series of substorms leads to an estimated ozone loss of 5–50% in the mesospheric column depending on season. This is similar in scale to small to medium solar proton events (SPEs). This effect on polar ozone balance is potentially more important on long time scales (months to years) than the impulsive but sporadic (few SPE/year versus three to four substorms/day) effect of SPEs. Our results suggest that substorms should be considered an important source of energetic particle precipitation into the atmosphere and included in high-top chemistry-climate models.

[1] Using a ground-based microwave radiometer at Troll Station, Antarctica (72°S, 2.5°E,L = 4.76), we have observed a decrease of 20–70% in the mesospheric ozone, coincident with increased nitric oxide, between 60 km and 75 km altitude associated with energetic electron precipitation (E > 30 keV) during a moderate geomagnetic storm (minimum Dst of −79 nT) in late July 2009. NOAA satellite data were used to identify the precipitating particles and to characterize their energy, spatial distribution and temporal variation over Antarctica during this isolated storm. Both the ozone decrease and nitric oxide increase initiate with the onset of the storm, and persist for several days after the precipitation ends, descending in the downward flow of the polar vortex. These combined data present a unique case study of the temporal and spatial morphology of chemical changes induced by electron precipitation during moderate geomagnetic storms, indicating that these commonplace events can cause significant effects on the middle mesospheric ozone distribution.

[1] We report the first ground-based passive microwave observations made from Troll station, Antarctica, which show enhanced mesospheric nitric oxide (NO) volume mixing ratio reaching levels of 1.2 ppmv, or 2–3 orders of magnitude above background, at 70–80 km during small, relatively isolated geomagnetic storms in 2008. The mesospheric NO peaked 2 days after enhanced NO at higher altitudes (110–150 km) measured by the SABER satellite, and 2 days after peaks in the >30 keV and >300 keV electron flux measured by POES, although the 300 keV electron flux remained high. High time resolution data shows that mesospheric NO was enhanced at night and decayed during the day and built up to high levels over a period of 3–4 days. The altitude profile of mesospheric NO suggests direct production by ∼300 keV electron precipitation. Simulations using the Sodankyla Ion and Neutral Chemistry model show that the delay between thermospheric and mesospheric NO enhancements was primarily a result of the weaker production rate at lower altitudes by ∼300 keV electrons competing against strong day-time losses.