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Forward-backward stochastic differential equations (FBSDEs) have received more and more attention in the past two decades. FBSDEs can be applied to many fields, such as economics and finance, engineering control, population dynamics analysis, and so on. In most cases, FBSDEs are nonlinear and high-dimensional and cannot be obtained as analytic solutions. Therefore, it is necessary and important to design their numerical approximation methods. In this paper, a novel numerical method of multi-dimensional coupled FBSDEs is proposed based on a fractional Fourier fast transform (FrFFT) algorithm, which is used to compute the Fourier and inverse Fourier transforms. For the forward component of FBSDEs, time discretization is used as well as the backward equation to yield a recursive system with terminal conditions. For the numerical experiments to be successful, three types of numerical methods were used to solve the problem, which ensured the efficiency and speed of computation. Finally, the numerical methods for different examples are verified. [ABSTRACT FROM AUTHOR]