Search

A buoyant plume model is used to explore the ability of flood basalt eruptions to inject climate-relevant gases into the stratosphere. An example from the 1986 Izu-Oshima basaltic fissure eruption validates the model's ability to reproduce the observed maximum plume heights of 12–16 km above sea level, sustained above fire-fountains. The model predicts maximum plume heights of 13–17 km for source widths of between 4–16 m when 32% (by mass) of the erupted magma is fragmented and involved in the buoyant plume (effective volatile content of 6 wt%). Assuming that the Miocene-age Roza eruption (part of the Columbia River Basalt Group) sustained fire-fountains of similar height to Izu-Oshima (1.6 km above the vent), we show that the Roza eruption could have sustained buoyant ash and gas plumes that extended into the stratosphere at ∼45°N. Assuming 5 km long active fissure segments and 9000 Mt of SO2 released during explosive phases over a 10–15 year duration, the ∼180km of known Roza fissure length could have supported ∼36 explosive events/phases, each with a duration of 3–4 days. Each 5 km fissure segment could have emitted 62 Mt of SO2 per day into the stratosphere while actively fountaining, the equivalent of about three 1991 Mount Pinatubo eruptions per day. Each fissure segment could have had one to several vents, which subsequently produced lava without significant fountaining for a longer period within the decades-long eruption. Sensitivity of plume rise height to ancient atmospheric conditions is explored. Although eruptions in the Deccan Traps (∼66Ma) may have generated buoyant plumes that rose to altitudes in excess of 18 km, they may not have reached the stratosphere because the tropopause was substantially higher in the late Cretaceous. Our results indicate that some flood basalt eruptions, such as Roza, were capable of repeatedly injecting large masses of SO2 into the stratosphere. Thus sustained flood basalt eruptions could have influenced climate on time scales of decades to centuries but the location (i.e., latitude) of the province and relevant paleoclimate is important and must be considered.

International audience; Geochemical interpretations of continental flood basalts usually assume that individual lava flows represent compositionally homogenous and rapidly erupted products of large well-mixed magma reservoirs. However, inflated pāhoehoe lavas may develop over considerable periods of time and preserve chemical variations that can be temporally linked through flow formation to eruption sequence thus providing an understanding of magma evolution over the timescale of a single eruption. This study presents comprehensive major, trace element and Re-Os isotope data for a single eruption that formed the 2660 km3 Sand Hollow flow field in the Columbia River Basalt Province, USA. Major and trace element variations accompanying flow emplacement (e.g. MgO 3.09-4.55 wt%, Ni 17.5-25.6 ppm) are consistent with fractional crystallisation, but other petrogenetic processes or variable sources cannot be distinguished. However, there is a systematic shift in the initial 187Os/188Os isotope composition of the magma (age corrected to 15.27 Ma), from 0.174 (lava core) to 1.444 (lava crust) within a single 35 m thick sheet lobe. Lava crust values are more radiogenic than any known mantle source, consistent with previous data indicating that neither an enriched reservoir nor the sub-continental lithospheric mantle are likely to have sourced these basalts. Rather, these data indicate that lavas emplaced during the earliest stages of eruption have higher degrees of crustal contamination. These results highlight the limitations of applying chemostratigraphic correlation across continental flood basalt provinces, the use of single data points to define melt sources and magmatic processes, and the dangers of using conventional isochron techniques in such basalt sequences for absolute chronology.

A very likely cause of widespread environmental impacts of flood basalt eruptions is the emission of sulfur, chlorine, and possibly fluorine from the erupting magma. We present new data on the S contents of rare glass inclusions and matrix glasses preserved in quenched lava selvages from lava fields of the Columbia River Basalt Group (CRBG; Ginkgo, Sand Hollow and Sentinel Gap flows, Wanapum Basalt Formation). We compare these results with published data from Neral and Jawar Formation lavas (Deccan Traps, India) and the Roza flow (CRBG). CRBG glass inclusions have up to 2000 ppm S and 15–16 wt.% FeOtotal. By contrast, the Deccan examples have about 1400 ppm S and 10 wt.% FeOtotal. Several of the glass inclusions are partly degassed, indicating entrapment during magma rise, and matrix glasses are typically more evolved than glass inclusions due to small amounts of in situ crystallization. Using only the highest S inclusions and taking account of the effect of in situ crystallization and degassing on the S content of the residual matrix glasses indicates S yields of about 0.07 to 0.1 wt.% from Deccan eruptions and about 0.15 wt.% from Wanapum (CRBG) eruptions. The pre-eruptive S contents of these magmas correlate with weight% FeOtotal in the same way as undegassed sulfide-saturated mid-ocean ridge basalts. Using oceanic basalts to define a sulfide saturation line, and data on S contents of degassed basalts, we propose an equation to estimate the weight% S yield (ΔS) from initially sulfide-saturated basalt liquid without the need to find well-preserved, rare, undegassed glass inclusions and matrix glasses: Δ S = ( 0.0 1418 × FeO total − 0.0 6381) ± 0.0 2635. This compares well with independent estimates derived from the petrologic method by taking the difference in S concentration of glass inclusions and matrix glass. Applying our method to the aphyric Grande Ronde Basalts of the CRBG implies a total yield of about 1000 Gt SO2 delivered into the Miocene atmosphere in intermittent bursts of

We examine the role that flood basalt eruptions may have played during times of mass extinction through the release of volcanic gases. Continental flood basalt provinces have formed by numerous eruptions over a short period of geologic time, characteristically a few million years. Within this period, a short-lived climactic phase that lasts about 1 Ma typically emplaces a large proportion of the lava volume. This phase consists of a series of huge eruptions, each yielding 10 3 –10 4 km 3 of magma. Each eruption lasted on the order of a decade or more, and built an immense pāhoehoe-dominated lava flow field by eruptive activity along fissures tens to hundreds of km long. High fire-fountains, emanating from vents along the fissures, at times sustained eruption columns that lofted gas and ash into the upper troposphere and lower stratosphere while the lava flows covered huge areas. The combination of large eruption magnitudes, maintained high effusion rates during eruptions, and the repeated nature of the characteristic, large-scale eruptive activity occurs in Earth history only during periods of flood basalt volcanism. Based on recent analogs and determination of volatile contents of ancient flood basalt lavas, we estimate that individual eruptions were capable of releasing 10,000 Tg of SO 2 , resulting in atmospheric loadings of 1000 Tg a − 1 during a sustained decade-long eruptive event. We apply this model of flood basalt volcanism to estimate the potential mass of CO 2 and SO 2 released during formation of the ∼ 65 Ma Deccan province. The Deccan lava-pile contains the record of hundreds of enormous pāhoehoe flow-fields erupted within a period of about 1 Ma. Consequently, atmospheric perturbations associated with SO 2 emissions from just one of these long-lasting eruptions were likely to have been severe, and constantly augmented over a decade or longer. By contrast, the amounts of CO 2 released would have been small compared with the mass already present in the atmosphere, and thus much more limited in effect. Individual eruptions were followed by hiatuses of hundreds to thousands of years during which the gas contributions to the atmosphere would be recycled. It is clear that the nature and potential atmospheric impact of a series of huge-volume, repeated, long-term degassing events requires further investigation in conjunction with appropriate climate models.