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Galactic cosmic rays undergo complex nuclear interactions with nuclei within planetary bodies that have little to no atmosphere. Radiation transport simulations are a key tool used in understanding the neutron and gamma ray albedo coming from these interactions and tracing these signals back to geochemical composition of the target. We study the validity of the code Geant4 for simulating such interactions by comparing simulation results to data from the Apollo 17 Lunar Neutron Probe Experiment. Different assumptions regarding the physics are explored to demonstrate how these impact the Geant4 simulation results. In general, all of the Geant4 results overpredict the data; however, certain physics lists perform better than others. In addition, we show that results from the radiation transport code MCNP6 are similar to those obtained using Geant4. [ABSTRACT FROM AUTHOR]