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Under the existence of system uncertainties, external disturbances, and input nonlinearity, complete synchronization and anti-synchronization between two chaotic gyros are achieved by introducing a novel adaptive terminal sliding mode (ATSM) controller. In the literature, by taking account of input nonlinearity, the magnitudes of bounded nonlinear dynamics of synchronous error system were required in the designed sliding mode controller. In this study, the proposed ATSM controller associated with time-varying feedback gains can tackle nonlinear dynamics according to the novel adaptive rules. These feedback gains are not necessary to be determined in advance but updated by the adaptive rules without known the magnitudes of bounded nonlinear dynamics, system uncertainties, and external disturbances. Sufficient conditions to guarantee stable synchronization are given in the sense of the Lyapunov stability theorem, and the numerical simulations are performed to verify the effectiveness of presented schemes.