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• Land-use types, seasons, slope position significantly affected SOC and SWC. • Revegetation increased SWS consumption and SOC accumulation. • There was a positive linear relationship between SOC and SWC. • Planting grass and shrubs is recommended in the semi-arid hilly and gully regions. Understanding the response of soil organic carbon (SOC) and moisture to different land-use types, slope positions, seasonal variations, and their interactions has great significance for land use and management. However, the coupling effects of SOC and soil moisture in typical hilly and gully regions are still elusive. Therefore, in this study, five different land-use types, including cropland, abandoned land, grassland, shrubland, and forestland were selected in a typical Chinese loess hilly-gully region, and soil samples were collected from 0 to 200 cm profiles at the upper, middle, and lower slope positions in four seasons. The results demonstrated that the distributions of SOC and soil moisture were jointly significantly affected by land-use types, seasons, and slope positions (P < 0.01). Average SOC content was found to be highest in the shrubland, followed by grassland, abandoned land, forestland, and cropland. SOC storage at the lower slope position was 10.97% higher than that at the upper slope position. SOC storage in winter was 45.47% higher than that in summer. SOC storages of abandoned land, grassland, shrubland, and forestland were 17.38%, 33.08%, 52.52% and 1.26% more than that of cropland, respectively. Soil moisture fluctuated greatly in 0–100 cm layers and was stable beneath the 100 cm layers, which was highest in autumn, and lowest in summer. Whereas, under different land-use types, the soil moisture of cropland was the highest, especially significantly higher than all revegetated treatments in the 60–200 cm soil layers. Compared with cropland, soil water storage at other land-use types was averagely 36.45 % lower in the entire 200 cm soil profile. SOC was positively correlated with soil moisture under different factors. Thus, we recommend planting shrub and grass in watersheds with serious soil erosion in the semi-arid hilly and gully region, because they can sequestrate more SOC and retain more soil water. [ABSTRACT FROM AUTHOR]