Search

This study quantifies differences among four widely used atmospheric reanalysis datasets (ERA5, JRA-55, MERRA-2, and CFSR) in their representation of the dynamical changes induced by springtime polar stratospheric ozone depletion in the Southern Hemisphere from 1980 to 2001. The intercomparison is undertaken as part of the SPARC (Stratosphere–troposphere Processes and their Role in Climate) Reanalysis Intercomparison Project (S-RIP). The reanalyses are generally in good agreement in their representation of the strengthening of the lower stratospheric polar vortex during the austral spring–summer season, associated with reduced radiative heating due to ozone loss, as well as the descent of anomalously strong westerly winds into the troposphere during summer and the subsequent poleward displacement and intensification of the polar front jet. Differences in the trends in zonal wind between the reanalyses are generally small compared to the mean trends. The exception is CFSR, which exhibits greater disagreement compared to the other three reanalysis datasets, with stronger westerly winds in the lower stratosphere in spring and a larger poleward displacement of the tropospheric westerly jet in summer. The dynamical changes associated with the ozone hole are examined by investigating the momentum budget and then the eddy heat and momentum fluxes in terms of planetary- and synoptic-scale Rossby wave contributions. The dynamical changes are consistently represented across the reanalyses and support our dynamical understanding of the response of the coupled stratosphere–troposphere system to the ozone hole. Although our results suggest a high degree of consistency across the four reanalysis datasets in the representation of these dynamical changes, there are larger differences in the wave forcing, residual circulation, and eddy propagation changes compared to the zonal wind trends. In particular, there is a noticeable disparity in these trends in CFSR compared to the other three reanalyses, while the best agreement is found between ERA5 and JRA-55. Greater uncertainty in the components of the momentum budget, as opposed to mean circulation, suggests that the zonal wind is better constrained by the assimilation of observations compared to the wave forcing, residual circulation, and eddy momentum and heat fluxes, which are more dependent on the model-based forecasts that can differ between reanalyses. Looking forward, however, these findings give us confidence that reanalysis datasets can be used to assess changes associated with the ongoing recovery of stratospheric ozone.

The majority of tropospheric ozone depletion event (ODE) studies have focussed on time-series measurements, with comparatively few studies of the vertical component. Those that exist have almost exclusively used free-flying balloon-borne ozonesondes and almost all have been conducted in the Arctic. Here we use measurements from two separate Antarctic field experiments to examine the vertical profile of ozone during Antarctic ODEs. We use tethersonde data to probe details in the lowest few hundred meters and find considerable structure in the profiles associated with complex atmospheric layering. The profiles were all measured at wind speeds less than 7 ms−1, and on each occasion the lowest inversion height lay between 10 m and 40 m. We also use data from a free-flying ozonesonde study to select events where ozone depletion was recorded at altitudes >1 km above ground level. Using ERA-40 meteorological charts, we find that on every occasion the high altitude depletion was preceded by an atmospheric low pressure system. An examination of limited published ozonesonde data from other Antarctic stations shows this to be a consistent feature. Given the link between BrO and ODEs, we also examine ground-based and satellite BrO measurements and find a strong association between atmospheric low pressure systems and enhanced BrO that must arise in the troposphere. The results suggest that, in Antarctica, such depressions are responsible for driving high altitude ODEs and for generating the large-scale BrO clouds observed from satellites. In the Arctic, the prevailing meteorology differs from that in Antarctica, but, while a less common effect, major low pressure systems in the Arctic can also generate BrO clouds. Such depressions thus appear to be fundamental when considering the broader influence of ODEs, certainly in Antarctica, such as halogen export and the radiative influence of ozone-depleted air masses.

The source of bromine that drives polar boundary layer ozone depletion events (ODEs) is still open to some debate. While ODEs are generally noted to form under conditions of a shallow stable boundary layer, observations of depleted air under high wind conditions are taken as being transport-related. Here we report observations from Antarctica in which an unusually large cloud of BrO formed over the Weddell Sea. The enhanced BrO was observed over Halley station in coastal Antarctica, providing an opportunity to probe the conditions within an active "bromine explosion" event. On this occasion, enhanced BrO and depleted boundary layer ozone coincided with high wind speeds and saline blowing snow. We derive a simple model to consider the environmental conditions that favour ODEs and find two maxima, one at low wind/stable boundary layer and one at high wind speeds with blowing snow. Modelling calculations aiming to reproduce the wider regional or global impacts of ODEs, either via radiative effects or as a halogen source, will also need to account for high wind speed mechanisms.