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A new model for greenhouse gas transport has been developed based on Environment and Climate Change Canada's operational weather and environmental prediction models. When provided with realistic posterior fluxes for CO2, the CO2 simulations compare well to NOAA's CarbonTracker fields, and to near surface continuous measurements, columns from the Total Carbon Column Observing Network (TCCON), and NOAA aircraft profiles. This coupled meteorological and tracer transport model is used to study the atmospheric modulation of CO2 transport. The predictability of CO2 due to initial state sensitivity is shorter than that for the temperature field but is consistent with the predictability of the wind fields. However, when broken down into spatial scales, CO2 has predictability at the very largest scales due to long time scale memory in surface CO2 fluxes as well as in land and ocean surface forcing of meteorological fields. The predictability due to the land and ocean surface is most evident in boreal summer when biospheric uptake produces large spatial gradients in the CO2 field. Predictability errors provide an upper limit for errors arising solely from the use of uncertain meteorological analyses. When considering meteorological analysis errors, CO2 can be defined only on large scales. Thus, there is a spatial scale below which information cannot be obtained simply due to the fact that meteorological analyses are imperfect. Compared to the spatial scales resolvable in the context of imperfect atmospheric analyses, the differences between two sets of posterior fluxes are resolvable only for very large scales. Similarly, the impact of convective tracer transport exceeds that due to atmospheric analysis errors for only the largest spatial scales. [ABSTRACT FROM AUTHOR]

A new model for greenhouse gas transport has been developed based on Environment and Climate Change Canada's operational weather and environmental prediction models. When provided with realistic posterior fluxes for CO2, the CO2 simulations compare well to NOAA's CarbonTracker fields, and to near surface continuous measurements, columns from the Total Carbon Column Observing Network (TCCON), and NOAA aircraft profiles. This coupled meteorological and tracer transport model is used to study the atmospheric modulation of CO2 transport. The predictability of CO2 due to initial state sensitivity is shorter than that for the temperature field but is consistent with the predictability of the wind fields. However, when broken down into spatial scales, CO2 has predictability at the very largest scales due to long time scale memory in surface CO2 fluxes as well as in land and ocean surface forcing of meteorological fields. The predictability due to the land and ocean surface is most evident in boreal summer when biospheric uptake produces large spatial gradients in the CO2 field. Predictability errors provide an upper limit for errors arising solely from the use of uncertain meteorological analyses. When considering meteorological analysis errors, CO2 can be defined only on large scales. Thus, there is a spatial scale below which information cannot be obtained simply due to the fact that meteorological analyses are imperfect. Compared to the spatial scales resolvable in the context of imperfect atmospheric analyses, the differences between two sets of posterior fluxes are resolvable only for very large scales. Similarly, the impact of convective tracer transport exceeds that due to atmospheric analysis errors for only the largest spatial scales. [ABSTRACT FROM AUTHOR]