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Despite offsetting global mean surface temperature, various studies demonstrated that stratospheric aerosol injection (SAI) could influence the recovery of stratospheric ozone and have important impacts on stratospheric and tropospheric circulation, thereby potentially playing an important role in modulating regional and seasonal climate variability. However, so far, most of the assessments of such an approach have come from climate model simulations in which SO 2 is injected only in a single location or a set of locations. Here we use CESM2-WACCM6 SAI simulations under a comprehensive set of SAI strategies achieving the same global mean surface temperature with different locations and/or timing of injections, namely an equatorial injection, an annual injection of equal amounts of SO 2 at 15 ∘ N and 15 ∘ S, an annual injection of equal amounts of SO 2 at 30 ∘ N and 30 ∘ S, and a polar strategy injecting SO 2 at 60 ∘ N and 60 ∘ S only in spring in each hemisphere. We demonstrate that despite achieving the same global mean surface temperature, the different strategies result in contrastingly different magnitudes of the aerosol-induced lower stratospheric warming, stratospheric moistening, strengthening of stratospheric polar jets in both hemispheres, and changes in the speed of the residual circulation. These impacts tend to maximise under the equatorial injection strategy and become smaller as the aerosols are injected away from the Equator into the subtropics and higher latitudes. In conjunction with the differences in direct radiative impacts at the surface, these different stratospheric changes drive different impacts on the extratropical modes of variability (Northern and Southern Annular modes), including important consequences on the northern winter surface climate, and on the intensity of tropical tropospheric Walker and Hadley circulations, which drive tropical precipitation patterns. Finally, we demonstrate that the choice of injection strategy also plays a first-order role in the future evolution of stratospheric ozone under SAI throughout the globe. Overall, our results contribute to an increased understanding of the fine interplay of various radiative, dynamical, and chemical processes driving the atmospheric circulation and ozone response to SAI and lay the foundation for designing an optimal SAI strategy that could form a basis of future multi-model intercomparisons. [ABSTRACT FROM AUTHOR]

Stratosphere-to-troposphere transport (STT) is an important source of ozone for the troposphere, particularly over western North America. STT in this region is predominantly controlled by a combination of the variability and location of the Pacific jet stream and the amount of ozone in the lower stratosphere, two factors which are likely to change if greenhouse gas concentrations continue to increase. Here we use Whole Atmosphere Community Climate Model experiments with a tracer of stratospheric ozone (O3S) to study how end-of-the-century Representative Concentration Pathway (RCP) 8.5 sea surface temperatures (SSTs) and greenhouse gases (GHGs), in isolation and in combination, influence STT of ozone over western North America relative to a preindustrial control background state. We find that O3S increases by up to 37 % during late winter at 700 hPa over western North America in response to RCP8.5 forcing, with the increases tapering off somewhat during spring and summer. When this response to RCP8.5 greenhouse gas forcing is decomposed into the contributions made by future SSTs alone versus future GHGs alone, the latter are found to be primarily responsible for these O3S changes. Both the future SSTs alone and the future GHGs alone accelerate the Brewer–Dobson circulation, which modifies extratropical lower-stratospheric ozone mixing ratios. While the future GHGs alone promote a more zonally symmetric lower-stratospheric ozone change due to enhanced ozone production and some transport, the future SSTs alone increase lower-stratospheric ozone predominantly over the North Pacific via transport associated with a stationary planetary-scale wave. Ozone accumulates in the trough of this anomalous wave and is reduced over the wave's ridges, illustrating that the composition of the lower-stratospheric ozone reservoir in the future is dependent on the phase and position of the stationary planetary-scale wave response to future SSTs alone, in addition to the poleward mass transport provided by the accelerated Brewer–Dobson circulation. Further, the future SSTs alone account for most changes to the large-scale circulation in the troposphere and stratosphere compared to the effect of future GHGs alone. These changes include modifying the position and speed of the future North Pacific jet, lifting the tropopause, accelerating both the Brewer–Dobson circulation's shallow and deep branches, and enhancing two-way isentropic mixing in the stratosphere. [ABSTRACT FROM AUTHOR]

The El Niño–Southern Oscillation (ENSO) is known to modulate the strength and frequency of stratosphere-to-troposphere transport (STT) of ozone over the Pacific–North American region during late winter to early summer. Dynamical processes that have been proposed to account for this variability include variations in the amount of ozone in the lowermost stratosphere that is available for STT and tropospheric circulation-related variations in the frequency and geographic distribution of individual STT events. Here we use a large ensemble of Whole Atmosphere Community Climate Model (WACCM) simulations (forced by sea-surface temperature (SST) boundary conditions consistent with each phase of ENSO) to show that variability in lower-stratospheric ozone and shifts in the Pacific tropospheric jet constructively contribute to the amount of STT of ozone in the North American region during both ENSO phases. In terms of stratospheric variability, ENSO drives ozone anomalies resembling the Pacific–North American teleconnection pattern that span much of the lower stratosphere below 50 hPa. These ozone anomalies, which dominate over other ENSO-driven changes in the Brewer–Dobson circulation (including changes due to both the stratospheric residual circulation and quasi-isentropic mixing), strongly modulate the amount of ozone available for STT transport. As a result, during late winter (February–March), the stratospheric ozone response to the teleconnections constructively reinforces anomalous ENSO-jet-driven STT of ozone. However, as ENSO forcing weakens as spring progresses into summer (April–June), the direct effects of the ENSO-jet-driven STT transport weaken. Nevertheless, the residual impacts of the teleconnections on the amount of ozone in the lower stratosphere persist, and these anomalies in turn continue to cause anomalous STT of ozone. These results should prove helpful for interpreting the utility of ENSO as a subseasonal predictor of both free-tropospheric ozone and the probability of stratospheric ozone intrusion events that may cause exceedances in surface air quality standards. [ABSTRACT FROM AUTHOR]

Stratospheric circulation is a critical part of the Arctic ozone cycle. Sudden stratospheric warming events (SSWs) manifest the strongest alteration of stratospheric dynamics. During SSWs, changes in planetary wave propagation vigorously influence zonal mean zonal wind, temperature, and tracer concentrations in the stratosphere over the high latitudes. In this study, we examine six persistent major SSWs from 2004 to 2020 using the Modern-Era Retrospective analysis for Research and Applications, Version 2 (MERRA-2). Using the unique density of observations around the Greenland sector at high latitudes, we perform comprehensive comparisons of high-latitude observations with the MERRA-2 ozone dataset during the six major SSWs. Our results show that MERRA-2 captures the high variability of mid-stratospheric ozone fluctuations during SSWs over high latitudes. However, larger uncertainties are observed in the lower stratosphere and troposphere. The zonally averaged stratospheric ozone shows a dramatic increase of 9 %–29 % in total column ozone (TCO) near the time of each SSW, which lasts up to 2 months. This study shows that the average shape of the Arctic polar vortex before SSWs influences the geographical extent, timing, and magnitude of ozone changes. The SSWs exhibit a more significant impact on ozone over high northern latitudes when the average polar vortex is mostly elongated as seen in 2009 and 2018 compared to the events in which the polar vortex is displaced towards Europe. Strong correlation (R2=90%) is observed between the magnitude of change in average equivalent potential vorticity before and after SSWs and the associated averaged total column ozone changes over high latitudes. This paper investigates the different terms of the ozone continuity equation using MERRA-2 circulation, which emphasizes the key role of vertical advection in mid-stratospheric ozone during the SSWs and the magnified vertical advection in elongated vortex shape as seen in 2009 and 2018. [ABSTRACT FROM AUTHOR]

Over recent years there have been concomitant advances in the development of stratosphere-resolving numerical models, our understanding of stratosphere–troposphere interaction, and the extension of long-range forecasts to explicitly include the stratosphere. These advances are now allowing for new and improved capability in long-range prediction. We present an overview of this development and show how the inclusion of the stratosphere in forecast systems aids monthly, seasonal, and annual-to-decadal climate predictions and multidecadal projections. We end with an outlook towards the future and identify areas of improvement that could further benefit these rapidly evolving predictions. [ABSTRACT FROM AUTHOR]

It has been suggested that increased stratospheric sulfate aerosol loadings following large, low latitude volcanic eruptions can lead to wintertime warming over Eurasia through dynamical stratosphere–troposphere coupling. We here investigate the proposed connection in the context of hypothetical future stratospheric sulfate geoengineering in the Geoengineering Large Ensemble simulations. In those geoengineering simulations, we find that stratospheric circulation anomalies that resemble the positive phase of the Northern Annular Mode in winter are a distinguishing climate response which is absent when increasing greenhouse gases alone are prescribed. This stratospheric dynamical response projects onto the positive phase of the North Atlantic Oscillation, leading to associated side effects of this climate intervention strategy, such as continental Eurasian warming and precipitation changes. Seasonality is a key signature of the dynamically driven surface response. We find an opposite response of the North Atlantic Oscillation in summer, when no dynamical role of the stratosphere is expected. The robustness of the wintertime forced response stands in contrast to previously proposed volcanic responses. [ABSTRACT FROM AUTHOR]

Stratosphere-to-troposphere mass transport to the planetary boundary layer (STT-PBL) peaks over the western United States during boreal spring, when deep stratospheric intrusions are most frequent. The tropopause-level jet structure modulates the frequency and character of intrusions, although the precise relationship between STT-PBL and jet variability has not been extensively investigated. In this study, we demonstrate how the North Pacific jet transition from winter to summer leads to the observed peak in STT-PBL. We show that the transition enhances STT-PBL through an increase in storm track activity which produces highly amplified Rossby waves and more frequent deep stratospheric intrusions over western North America. This dynamic transition coincides with the gradually deepening PBL, further facilitating STT-PBL in spring. We find that La Niña conditions in late winter are associated with an earlier jet transition and enhanced STT-PBL due to deeper and more frequent tropopause folds. An opposite response is found during El Niño conditions. El Niño–Southern Oscillation (ENSO) conditions also influence STT-PBL in late spring or early summer, during which time La Niña conditions are associated with larger and more frequent tropopause folds than both El Niño and ENSO-neutral conditions. These results suggest that knowledge of ENSO state and the North Pacific jet structure in late winter could be leveraged for predicting the strength of STT-PBL in the following months. [ABSTRACT FROM AUTHOR]

The agreement between reanalysis datasets, in terms of the zonal-mean momentum budget, is evaluated during sudden stratospheric warming (SSW) events. It is revealed that there is a good agreement among datasets in the lower stratosphere and troposphere concerning zonal-mean zonal wind, but less so in the upper stratosphere. Forcing terms of the momentum equation are also relatively similar in the lower atmosphere, but their uncertainties are typically larger than uncertainties of the zonal-wind tendency. Similar to zonal-wind tendency, the agreement among forcing terms is degraded in the upper stratosphere. Discrepancies among reanalyses increase during the onset of SSW events, a period characterized by unusually large fluxes of planetaryscale waves from the troposphere to the stratosphere, and decrease substantially after the onset. While the largest uncertainties in the resolved terms of the momentum budget are found in the Coriolis torque, momentum flux convergence also presents a non-negligible spread among the reanalyses. Such a spread is reduced in the latest reanalysis products, decreasing the uncertainty of the momentum budget. It is also found that the uncertainties in the Coriolis torque depend on the strength of SSW events: the SSW events that exhibit the most intense deceleration of zonal-mean zonal wind are subject to larger discrepancies among reanalyses. These uncertainties in stratospheric circulation, however, are not communicated to the troposphere. [ABSTRACT FROM AUTHOR]