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Stellar spectral template libraries play an important role in the automated analysis of stellar spectra. Synthetic template libraries cover a very large parameter space but suffer from poor matching with observed spectra. In this study, we propose a synthetic-to-observed spectral translation (SOST) method based on generative adversarial networks. The SOST method is able to calibrate synthetic spectra by converting them to the corresponding observed spectra. We applied this method to Kurucz synthetic spectra and observed spectra data from the Large Sky Area Multi-Object Fiber Spectroscopic Telescope (LAMOST). After that, we constructed a stellar spectral library with uniform and broad parameter distributions using the SOST-corrected Kurucz synthetic spectra. Our stellar spectral template library contains 2431 spectra spanning a parameter space of 3500–8000 K for effective temperature (Teff), 0.0–5.0 dex for surface gravity (log g), and −2.0–0.5 dex for metallicity ([Fe/H]). The spectra in the library have a resolution of R ∼ 1800 and cover the wavelength range 3900–8700 Å. In order to verify the accuracy of this template library, we used the template library and the template-matching algorithm to derive the parameters of the PASTEL database. Compared to measurements using the original synthetic template library, the accuracies of the three parameters, Teff, log g, and [Fe/H], are improved, from 140 K, 0.31 dex, and 0.21 dex to 121 K, 0.26 dex, and 0.13 dex, respectively. In addition, we re-parameterised more than six million stellar spectra released by LAMOST DR8. [ABSTRACT FROM AUTHOR]