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In this paper, we analyzed two decadal long term (2003–2022) data of AOD and cloud parameters to understand the spatial and temporal variations in aerosol radiative characteristics over a highly polluted urbanized region of Northern India. The aerosol and cloud data were derived at spectral wavelength of 550 nm from the MODIS based Terra/Aqua satellites. Detailed AOD quantitative analysis considering monthly, seasonal and interannual changes was investigated in relation to cloud characteristics and zonal synoptic climatic disturbances. HYSPLIT back trajectory 5-day analysis was made to know the pathways of air masses ending at Delhi region of India. Moreover, we applied Student's t-test to mean Terra AOD and cloud properties to examine and further validate the relationship of aerosol-cloud interaction over the urban tropical Delhi zone close to Himalaya range of Northern India. Results indicated that AODs were found to be increased significantly (> 68%) during the 20 years period of 2003–2022, which might be accounted to continuously increased aerosol pollution in atmosphere. On an annual basis, mean Terra AOD exhibited an increasing trend of ~ 0.0009 per year, whereas seasonal mean AOD was observed to be maximum for winter (~ 0.96) and minimum for summer (~ 0.55), respectively. The correlation coefficient was highest (+ 0.73) between AOD and precipitable water vapor, whereas lowest (− 0.46) between AOD and cloud top pressure (CTP). The findings of AOD and cloud parameters have been compared with the earlier findings made on different Indian cities. [ABSTRACT FROM AUTHOR]