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Lamb wave resonators (LWRs) exhibiting high-quality factors and clean spectra demonstrate promising applications in RF communication and sensing. This paper discusses the relationship between the spurious mode, the quality factor, and the effective electromechanical coupling factor of resonators. When the resonant frequency of the spurious mode is slightly below the parallel resonant frequency (fp), the quality factor at fp (Qp) decreases dramatically. To enhance Qp and suppress the spurious mode, the LWRs with busbars including only the top electrode (non-overlap busbars) and the LWRs with busbars incorporating both top and bottom electrodes (overlap busbars) are designed and fabricated. The LWR with 12 μm-wide overlap busbars exhibits a notable enhancement in Qp, elevating it from 553.76 to 1488.17 and suppresses the spurious mode simultaneously. This research introduces a promising approach to suppress the spurious mode and enhance the quality factor of Lamb wave resonators, thereby holding great potential for applications in sensors and mobile communication. [ABSTRACT FROM AUTHOR]