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Start Over Author "Li, Yuehui" Topic catalysis Journal angewandte chemie international edition

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1. Iron-Catalyzed Hydrogenation for the In Situ Regeneration of an NAD(P)H Model: Biomimetic Reduction of α-Keto-/α-Iminoesters.

Author

Lu, Liang‐Qiu, Li, Yuehui, Junge, Kathrin, and Beller, Matthias

Subjects
*CATALYSIS, *HYDROGENATION, *IRON catalysts, *NAD (Coenzyme), *ADENINE nucleotides
Abstract

Two irons for a smoother finish: An NAD(P)H model was regenerated readily in situ by iron‐catalyzed reduction with molecular hydrogen. The subsequent biomimetic reduction of α‐keto‐/ α‐iminoesters proceeded smoothly in the presence of an iron‐based Lewis acid (LA) to provide α‐hydroxyesters and amino acid esters in good to excellent yields (see scheme; NAD(P)+=nicotinamide adenine dinucleotide (phosphate), TM=transition metal). [ABSTRACT FROM AUTHOR]

Published
2013
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