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Evolution has decided to gift an articular structure to vertebrates, but not to invertebrates, owing to their distinct survival strategies. An articular structure permits kinematic motion in creatures. However, it is inappropriate for creatures whose survival strategy depends on the high deformability of their body. Accordingly, a material in which the presence of the articular structure can be altered, allowing the use of two contradictory strategies, will be advantageous in diverse dynamic applications. Herein, spatial micro‐water molecule manipulation, termed engineering on variable occupation of water (EVO), that is used to realize a material with dual mechanical modes that exhibit extreme differences in stiffness is introduced. A transparent and homogeneous soft material (110 kPa) reversibly converts to an opaque material embodying a mechanical gradient (ranging from 1 GPa to 1 MPa) by on‐demand switching. Intensive theoretical analysis of EVO yields the design of spatial transformation scheme. The EVO gel accomplishes kinematic motion planning and shows great promise for multimodal kinematics. This approach paves the way for the development and application of smart functional materials., In this paper, a strategy that manipulates micro‐water of hydrogel in reversible, selective, and on‐demand manner is reported. It realizes instant switching between a transparent and homogeneously soft gel and an opaque and heterogeneously rigid solid with a monolithic mechanical gradient. These two mechanical dual modes mimicking the characteristic of invertebrate and vertebrate demonstrate multi‐modal kinematics.

Spatial Micro‐Water Manipulation An octopus with homogeneously soft structure can easily hide in rocks, where an athlete can throw javelin in precisely controlled manner thanks to the articular structure. Nature designed these distinctive structures by adjusting the amount of water inside. For taking both of their kinematics, the spatial micro‐water molecule manipulation maneuvers the amount of water in the hydrogel enabling the alteration between two structures. More details can be found in article number 2102536 by Seung Hwan Ko and co‐workers. [Image: see text]