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Flexible electronic equipment is an emerging field in recent years, which attaches more attention to be researched and applied in health monitoring and human–machine interface. However, for the existing pressure sensors, even a very slight pressure will greatly reduce their sensitivity, so it is an urgent problem to be solved for achieving high sensitivity and wide application range simultaneously. Hence, a high‐performance piezoresistive pressure sensor based on PAN nanofiber films (PAN NFs) and MXene (Ti3C2Tx) is proposed. The realization of high sensitivity and wide sensing range is based on the microstructure of accordion‐like MXene and the macrostructure of fluffy porous blowing spinning PAN nanofibers, which exhibits a high sensitivity of 81.89 kPa−1 over a wide sensing range of 0.83–38.13 kPa and the dynamic responses to external pressures can reach 98.73 kPa. The pressure sensors based on skin surface‐like 3D patterned interwoven structure are used for health monitoring and tiny pressure detecting. Moreover, the application in human–machine interface is demonstrated. Additionally, to meet the requirement of long‐term wearing, the structure of the sensor is optimized and endowed with excellent breathability and conformal properties, which promotes the further development of flexible electronic equipment. [ABSTRACT FROM AUTHOR]

Improvement of sensitivity of electrical piezoresistive sensors is critical for high‐precision and ultrasensitive detection, which mainly depends on the modulation ability of total resistance of sensor under applied pressure. However, in most of the reported sensor devices, the contact resistance and body resistance (the key parts of total resistance of sensor) generally cannot be modulated simultaneously, which results in the limited sensitivity. In this work, an ultrahighly sensitive piezoresistive pressure sensor with an exquisitely designed structure is demonstrated, providing an uncomparable advantage of synergistic modulation of contact resistance and body resistance under applied pressure. As a result, the sensor shows excellent sensing performance, with the highest sensitivity up to 11 668.6 kPa−1, the detection limit as low as 0.425 Pa, and the great stability over 20 000 cycle measurements. In respect of practical application, the high sensitivity endows the sensor with high‐precision recognition ability for detecting the weak pressure signals such as sound wave of ringtone and fluctuation of breath or pulse. These results suggest the synergistic resistance modulation to be an effective method toward piezoresistive pressure sensors with ultrahigh sensitivity and offer a new strategy for the achievement of high‐performance pressure sensors. [ABSTRACT FROM AUTHOR]