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Wearable pressure sensors with wide operating pressure ranges and enhanced wearability via seamless integration with circuits can greatly improve the fields of digital healthcare, prosthetic limbs, and human–machine interfaces. Herein, we report an approach based on a conductive-island-bridging nanonetwork to realize wearable resistive pressure sensors that are operative over ultrawide pressure ranges >400 kPa and are circuit-compatible. The sensor has a simple two-layered structure, where nanonetworks of single-walled carbon nanotubes selectively patterned on a surface-modified elastomeric film interface and bridge conductive Au island patterns on printed circuit boards (PCBs). We show that varying the design of the Au islands and the conductivity of the nanonetworks systematically tunes the sensitivity, linearity, and the operation range of the pressure sensor. In addition, introducing microstructured lead contacts into the sensor based on a Au-island-bridging nanonetwork produces a record-high sensitivity of 0.06 kPa–1at 400 kPa. Furthermore, the PCB that serves as the bottom layer of the pressure sensor and contains embedded interconnects enables facile integration of the sensor with measurement circuits and wireless communication modules. The developed sensor enables the monitoring of wrist pulse waves. Moreover, an insole-shaped PCB-based pressure-sensing system wirelessly monitors pressure distributions and gait kinetics during walking. Our scheme can be extended to other nanomaterials and flexible PCBs and thus provides a simple yet powerful platform for emerging wearable applications.

Flexible piezoresistive sensors have huge potential for health monitoring, human–machine interfaces, prosthetic limbs, and intelligent robotics. A variety of nanomaterials and structural schemes have been proposed for realizing ultrasensitive flexible piezoresistive sensors. However, despite the success of recent efforts, high sensitivity within narrower pressure ranges and/or the challenging adhesion and stability issues still potentially limit their broad applications. Herein, we introduce a biomaterial-based scheme for the development of flexible pressure sensors that are ultrasensitive (resistance change by 5 orders) over a broad pressure range of 0.1–100 kPa, promptly responsive (20 ms), and yet highly stable. We show that employing biomaterial-incorporated conductive networks of single-walled carbon nanotubes as interfacial layers of contact-based resistive pressure sensors significantly enhances piezoresistive response via effective modulation of the interlayer resistance and provides stable interfaces for the pressure sensors. The developed flexible sensor is capable of real-time monitoring of wrist pulse waves under external medium pressure levels and providing pressure profiles applied by a thumb and a forefinger during object manipulation at a low voltage (1 V) and power consumption (<12 μW). This work provides a new insight into the material candidates and approaches for the development of wearable health-monitoring and human–machine interfaces.