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Machine learning has been found to be ubiquitously useful across many industries, presenting an opportunity to improve radiation detection performance using data-driven algorithms. Improved detector resolution can aid in the detection, identification, and quantification of radionuclides. In this work, a novel, data-driven, unsupervised learning approach is developed to improve detector spectral characteristics by learning, and subsequently rejecting, poorly performing regions of the pixelated detector. Feature engineering is used to fit individual characteristic photo peaks to a Doniach lineshape with a linear background model. Then, principal component analysis is used to learn a lower-dimension latent space representation of each photo peak where the pixels are clustered, and subsequently ranked, based on the cluster mean distance to an optimal point. Pixels within the worst cluster(s) are rejected to improve the full-width at half-maximum (FWHM) by 10% to 15% (relative to the bulk detector) at 50% net efficiency when applied to training data obtained from measurements of a 100 μCi 154Eu source using a H3D M400i pixelated cadmium zinc telluride detector. These results compare well with, but do not outperform, a greedy algorithm that accumulates pixels in order of FWHM from lowest to highest used as a benchmark. In the future, this approach can be extended to include the detector energy and angular response. Finally, the model is applied to newly seen natural and enriched uranium spectra relevant for nuclear safeguards applications.

The detection, identification, and localization of illicit radiological and nuclear material continue to be key components of nuclear non-proliferation and nuclear security efforts around the world. Networks of radiation detectors deployed at strategic locations in urban environments have the potential to provide continuous radiological/nuclear (R/N) surveillance and provide high probabilities of intercepting threat sources. The integration of contextual information from sensors such as video, Lidar, and meteorological sensors can provide significantly enhanced situational awareness, and improved detection and localization performance through the fusion of the radiological and contextual data. In this work, we present details of our work to establish a city-scale multi-sensor network testbed for intelligent, adaptive R/N detection in urban environments, and develop new techniques that enable city-scale source detection, localization, and tracking.

The ability to formulate maps of minimum detectable activities (MDAs) that describe the sensitivity of an ad hoc measurement that used one or more freely moving radiation detector systems would be significantly beneficial for the conduct and understanding of many radiological search activities. In a real-time scenario with a free-moving detector system, an MDA map can provide useful feedback to the operator about which areas have not been searched as thoroughly as others, thereby allowing the operator to prioritize future actions. Similarly, such a calculation could be used to inform subsequent navigation decisions of autonomous platforms. Here we describe a near real-time MDA mapping approach that can be applied when searching for point sources using detected events in a spectral region of interest (ROI) while assuming a constant, unknown background rate. We show the application of this MDA mapping method to a real scenario, a survey of the interior of a small building using a handheld detector system. Repeated measurements with no sources and with 137Cs sources of different strengths yield results consistent with the estimated thresholds and MDA values; namely, that for background-only measurements no sources are seen above threshold anywhere in the scene, while when sources are present they are detected above the thresholds calculated for their locations.

Using a series of detector measurements taken at different locations to localize a source of radiation is a well-studied problem. The source of radiation is sometimes constrained to a single point-like source, in which case the location of the point source can be found using techniques such as maximum likelihood. Recent advancements have shown the ability to locate point sources in 2-D and even 3-D but few have studied the effect of intervening material on the problem. In this work, we examine gamma-ray data taken from a freely moving system and develop voxelized 3-D models of the scene using data from its onboard light detection and ranging (LiDAR) unit. Ray casting is used to compute the distance each gamma ray travels through the scene material, which is then used to calculate attenuation assuming a single attenuation coefficient for solids within the geometry. Parameter estimation using maximum likelihood is performed to simultaneously find the attenuation coefficient, source activity, and source position that best match the data. Using a simulation, we validate the ability of this method to reconstruct the true location and activity of a source, along with the true attenuation coefficient of the structure it is inside, and then we apply the method to measured data with sources and find good agreement.

The Polaris-LAMP multi-modal 3-D gamma-ray imager is a radiation mapping and imaging platform which uses a commercial off-the-shelf (COTS) detector integrated with a contextual sensor localization and mapping platform. The integration of these systems enables a free-moving radiation imaging capability with proximity mapping, coded-aperture, and Compton imaging modalities, which can create 3-D reconstruction of photon sources from tens of keV to several MeV. Gamma-ray events are recorded using a segmented cadmium zinc telluride (CZT) detector (Polaris-H Quad by H3D Inc., Ann Arbor, MI, USA), while scene data are derived from a contextual sensor and computation package developed by Lawrence Berkeley National Laboratory which includes GPS, laser ranging, and inertial measurement sensors. An onboard computer uses these inputs to create rapidly updating pose (10 Hz) and 3-D scene estimates using a simultaneous localization and mapping (SLAM) algorithm. The precise gamma-ray event location and timing resolution of the Polaris CZT sensor enables Compton imaging above several hundred keV, while photon sources at lower images are localized using coded-aperture imaging techniques. The multi-modal imaging concept enables imaging of diverse radiation sources spanning from the 59-keV emission of 241Am to the 1.1 and 1.3 MeV lines of 60Co. This work focuses on the description of the operational principles of the detector system and demonstrating the 3-D imaging performance in a variety of source detection and mapping scenarios. As a proof of concept, we demonstrate mapping complex environments, including both point source and distributed-source environments using proximity, coded-aperture, and Compton imaging modalities. Furthermore, we show the successful use of the system to perform measurements in high-background environments through analysis of arrays of uranium hexafluoride cylinders at the Paducah UF6 project site.

Using a series of detector measurements taken at different locations tolocalize a source of radiation is a well-studied problem. The source ofradiation is sometimes constrained to a single point-like source, in which casethe location of the point source can be found using techniques such as maximumlikelihood. Recent advancements have shown the ability to locate point sourcesin 2D and even 3D, but few have studied the effect of intervening material onthe problem. In this work we examine gamma-ray data taken from a freely movingsystem and develop voxelized 3-D models of the scene using data from theonboard LiDAR. Ray casting is used to compute the distance each gamma raytravels through the scene material, which is then used to calculate attenuationassuming a single attenuation coefficient for solids within the geometry.Parameter estimation using maximum likelihood is performed to simultaneouslyfind the attenuation coefficient, source activity, and source position thatbest match the data. Using a simulation, we validate the ability of this methodto reconstruct the true location and activity of a source, along with the trueattenuation coefficient of the structure it is inside, and then we apply themethod to measured data with sources and find good agreement.

Using a series of detector measurements taken at different locations tolocalize a source of radiation is a well-studied problem. The source ofradiation is sometimes constrained to a single point-like source, in which casethe location of the point source can be found using techniques such as maximumlikelihood. Recent advancements have shown the ability to locate point sourcesin 2D and even 3D, but few have studied the effect of intervening material onthe problem. In this work we examine gamma-ray data taken from a freely movingsystem and develop voxelized 3-D models of the scene using data from theonboard LiDAR. Ray casting is used to compute the distance each gamma raytravels through the scene material, which is then used to calculate attenuationassuming a single attenuation coefficient for solids within the geometry.Parameter estimation using maximum likelihood is performed to simultaneouslyfind the attenuation coefficient, source activity, and source position thatbest match the data. Using a simulation, we validate the ability of this methodto reconstruct the true location and activity of a source, along with the trueattenuation coefficient of the structure it is inside, and then we apply themethod to measured data with sources and find good agreement.

Networked detector systems can be deployed in urban environments to aid in the detection and localization of radiological and/or nuclear material. However, effectively responding to and interpreting a radiological alarm using spectroscopic data alone may be hampered by a lack of situational awareness, particularly in complex environments. This study investigates the use of Light Detection and Ranging (LiDAR) and streaming video to enable real-time object detection and tracking, and the fusion of this tracking information with radiological data for the purposes of enhanced situational awareness and increased detection sensitivity. This work presents an object detection, tracking, and novel source-object attribution analysis that is capable of operating in real time. By implementing this analysis pipeline on a custom-developed system that comprises a static 2 in. \times 4 in. \times16 in. NaI(Tl) detector colocated with a 64-beam LiDAR and four monocular cameras, we demonstrate the ability to accurately correlate trajectories from tracked objects to spectroscopic gamma-ray data in real time and use physics-based models to reliably discriminate between source-carrying and nonsource-carrying objects. In this work, we describe our approach in detail and present a quantitative performance assessment that characterizes the source-object attribution capabilities of both video and LiDAR. Additionally, we demonstrate the ability to simultaneously track pedestrians and vehicles in a mock urban environment and use this tracking information to improve both detection sensitivity and situational awareness using our contextual-radiological data fusion methodology.

We present an experimental demonstration of additive point source localization (APSL), a sparse parametric imaging algorithm that reconstructs the 3-D positions and activities of multiple gamma-ray point sources. Using a handheld gamma-ray detector array and up to four 8 mu Ci 137Cs gamma-ray sources, we performed both source-search and source-separation experiments in an indoor laboratory environment. In the majority of the source-search measurements, APSL reconstructed the correct number of sources with position accuracies of 20 cm and activity accuracies (unsigned) of 20%, given measurement times of 2 to 3 min and distances of closest approach (to any source) of 20 cm. In source-separation measurements where the detector could be moved freely about the environment, APSL was able to resolve two sources separated by 75 cm or more given only 60 s of measurement time. In these source-separation measurements, APSL produced larger total activity errors of 40%, but obtained source-separation distances accurate to within 15 cm. We also compare our APSL results against traditional maximum likelihood-expectation maximization (ML-EM) reconstructions and demonstrate improved image accuracy and interpretability using APSL over ML-EM. These results indicate that APSL is capable of accurately reconstructing gamma-ray source positions and activities using measurements from existing detector hardware.

The potential of elastic antineutrino-electron scattering in a Gd-doped water Cherenkov detector to determine the direction of a nuclear reactor antineutrino flux was investigated using the recently proposed WATCHMAN antineutrino experiment as a baseline model. The expected scattering rate was determined assuming a 13-km standoff from a 3.758-GWt light water nuclear reactor and the detector response was modeled using a Geant4-based simulation package. Background was estimated via independent simulations and by scaling published measurements from similar detectors. Background contributions were estimated for solar neutrinos, misidentified reactor-based inverse beta decay interactions, cosmogenic radionuclides, water-borne radon, and gamma rays from the photomultiplier tubes (PMTs), detector walls, and surrounding rock. We show that with the use of low background PMTs and sufficient fiducialization, water-borne radon and cosmogenic radionuclides pose the largest threats to sensitivity. Directional sensitivity was then analyzed as a function of radon contamination, detector depth, and detector size. The results provide a list of experimental conditions that, if satisfied in practice, would enable antineutrino directional reconstruction at 3σ significance in large Gd-doped water Cherenkov detectors with greater than 10-km standoff from a nuclear reactor.