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Intense few-cycle laser pulses have a breadth of applications in high energy density science, including particle acceleration and x-ray generation. Multi-amplifier laser system pulses have durations of tens of femtoseconds or longer. To achieve high intensities at the single-cycle limit, a robust and efficient post-compression scheme is required. We demonstrate a staged compression technique using self-phase modulation in thin dielectric media, in which few-cycle pulses can be produced. The few-cycle pulse is then used to generate extreme ultravoilet light via high harmonic generation at strong field intensities and to generate MeV electron beams via laser solid interactions at relativistic intensities.

Intense few-cycle laser pulses have a breadth of applications in high energy density science, including particle acceleration and x-ray generation. Multi-amplifier laser system pulses have durations of tens of femtoseconds or longer. To achieve high intensities at the single-cycle limit, a robust and efficient post-compression scheme is required. We demonstrate a staged compression technique using self-phase modulation in thin dielectric media, in which few-cycle pulses can be produced. The few-cycle pulse is then used to generate extreme ultravoilet light via high harmonic generation at strong field intensities and to generate MeV electron beams via laser solid interactions at relativistic intensities.

Thin-film compression (TFC) and the focusability of high-power laser pulses after self-phase modulation in thin films at transport intensities (∼1 TW∕cm 2 ) for petawatt laser systems is demonstrated. High-energy (∼296 mJ) laser pulses are compressed from ∼55 fs to ∼31 fs. Additionally, the focusability of high-power (∼45–55 TW) flat-top laser pulses after spectral broadening in thin films is found to be largely maintained, showing only modest decreases in the energy contained in the central part of the focal spot. In light of these findings, TFC offers a method for moving toward single-cycle pulse durations at significantly higher energies than those found at present, and if beam instabilities can be mitigated, maybe even higher intensities.

Superponderomotive-energy electrons are observed experimentally from the interaction of an intense laser pulse with a relativistically transparent target. For a relativistically transparent target, kinetic modeling shows that the generation of energetic electrons is dominated by energy transfer within the main, classically overdense, plasma volume. The laser pulse produces a narrowing, funnel-like channel inside the plasma volume that generates a field structure responsible for the electron heating. The field structure combines a slowly evolving azimuthal magnetic field, generated by a strong laser-driven longitudinal electron current, and, unexpectedly, a strong propagating longitudinal electric field, generated by reflections off the walls of the funnel-like channel. The magnetic field assists electron heating by the transverse electric field of the laser pulse through deflections, whereas the longitudinal electric field directly accelerates the electrons in the forward direction. The longitudinal electric field produced by reflections is 30 times stronger than that in the incoming laser beam and the resulting direct laser acceleration contributes roughly one third of the energy transferred by the transverse electric field of the laser pulse to electrons of the super-ponderomotive tail.

Superponderomotive-energy electrons are observed experimentally from the interaction of an intense laser pulse with a relativistically transparent target. For a relativistically transparent target, kinetic modeling shows that the generation of energetic electrons is dominated by energy transfer within the main, classically overdense, plasma volume. The laser pulse produces a narrowing, funnel-like channel inside the plasma volume that generates a field structure responsible for the electron heating. The field structure combines a slowly evolving azimuthal magnetic field, generated by a strong laser-driven longitudinal electron current, and, unexpectedly, a strong propagating longitudinal electric field, generated by reflections off the walls of the funnel-like channel. The magnetic field assists electron heating by the transverse electric field of the laser pulse through deflections, whereas the longitudinal electric field directly accelerates the electrons in the forward direction. The longitudinal electric field produced by reflections is 30 times stronger than that in the incoming laser beam and the resulting direct laser acceleration contributes roughly one third of the energy transferred by the transverse electric field of the laser pulse to electrons of the super-ponderomotive tail.

High harmonic generation driven by femtosecond lasers makes it possible to capture the fastest dynamics in molecules and materials. However, to date the shortest subfemtosecond (attosecond, 10-18 s) pulses have been produced only in the extreme UV region of the spectrum below 100 eV, which limits the range of materials and molecular systems that can be explored. Here we experimentally demonstrate a remarkable convergence of physics: when midinfrared lasers are used to drive high harmonic generation, the conditions for optimal bright, soft X-ray generation naturally coincide with the generation of isolated attosecond pulses. The temporal window over which phase matching occurs shrinks rapidly with increasing driving laser wavelength, to the extent that bright isolated attosecond pulses are the norm for 2-μm driving lasers. Harnessing this realization, we experimentally demonstrate the generation of isolated soft X-ray attosecond pulses at photon energies up to 180 eV for the first time, to our knowledge, with a transform limit of 35 attoseconds (as), and a predicted linear chirp of 300 as. Most surprisingly, advanced theory shows that in contrast with as pulse generation in the extreme UV, long-duration, 10-cycle, driving laser pulses are required to generate isolated soft X-ray bursts efficiently, to mitigate group velocity walk-off between the laser and the X-ray fields that otherwise limit the conversion efficiency. Our work demonstrates a clear and straightforward approach for robustly generating bright isolated attosecond pulses of electromagnetic radiation throughout the soft X-ray region of the spectrum.

Each successive generation of x-ray machines has opened up new frontiers inscience, such as the first radiographs and the determination of the structureof DNA. State-of-the-art x-ray sources can now produce coherent high brightnesskeV x-rays and promise a new revolution in imaging complex systems on nanometreand femtosecond scales. Despite the demand, only a few dedicated synchrotronfacilities exist worldwide, partially due the size and cost of conventional(accelerator) technology. Here we demonstrate the use of a recently developedcompact laser-plasma accelerator to produce a well-collimated,spatially-coherent, intrinsically ultrafast source of hard x-rays. This methodreduces the size of the synchrotron source from the tens of metres tocentimetre scale, accelerating and wiggling a high electron chargesimultaneously. This leads to a narrow-energy spread electron beam and x-raysource that is >1000 times brighter than previously reported plasma wiggler andthus has the potential to facilitate a myriad of uses across the whole spectrumof light-source applications.

Absolute photoionization cross-section measurements for a mixture of ground and metastable states of Xe4+, Xe5+, and Xe6+ are reported in the photon energy range of 4d-nf transitions, which occur within or adjacent to the 13.5 nm window for extreme ultraviolet lithography light source development. The reported values allow the quantification of opacity effects in xenon plasmas due to these 4d-4f autoionizing states. The oscillator strengths for the 4d-4f and 4d-5f transitions in Xeq+ (q=1-6) ions are calculated using nonrelativistic Hartree-Fock and random phase approximations. These are compared with published experimental values for Xe+ to Xe3+ and with the values obtained from the present experimental cross-section measurements for Xe4+ to Xe6+. The calculations assisted in the determination of the metastable content in the ion beams for Xe5+T and Xe6+. The experiments were performed by merging a synchrotron photon beam generated by an undulator beamline of the Advanced Light Source with an ion beam produced by an electron cyclotron resonance ion source.