1. A comprehensive modeling of the hybrid temperature electric swing adsorption process for CO2 capture.
- Author
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Lillia, S., Bonalumi, D., Manzolini, G., and Grande, C.
- Subjects
TEMPERATURE ,CARBON sequestration ,ADSORPTION (Chemistry) ,ZEOLITES ,MOLECULAR acoustics - Abstract
Adsorption technologies provide high selectivity and low energy consumption making this technique very attractive to be employed in post-combustion carbon capture. In this publication, a material made of activated carbon and zeolite 13X is considered for a hybrid process termed Temperature Electric Swing Adsorption (T/ESA). This hybrid T/ESA can work as a traditional Temperature Swing Adsorption (TSA) heated by hot gas, but can also increase the temperature of the adsorbent very fast by Joule effect as long as the activated carbon provides a continuous conductive matrix for electricity. This paper discusses a detailed modeling of the T/ESA process when applied to three cases. The first case is the simulation of the T/ESA process with exhaust with 12% of CO 2 concentration, which has been chosen to validate the model against literature results. The second and third case studies consider the T/ESA application in a natural gas combined cycle (NGCC) traditional power plant, and in a NGCC plant with exhaust gas recycle (EGR). These cases were selected to investigate the adsorption technology at low CO 2 concentration and quantify the benefit of the EGR for carbon capture applications. Starting from an NGCC overall electric efficiency of 58.3% LHV based, the efficiency of the NGCC with T/ESA technology reduces to 35.3% while with EGR is 38.9% against the 49.9% with the MEA absorption plant. The same results are confirmed by the SPECCA index 13.05 MJ LHV /kg CO2 to 9.64 MJ LHV /kg CO2 against the reference of 3.36 MJ LHV /kg CO2 . The energy penalty of the T/ESA is significant because of electric consumptions required for the heating and fast cooling of the adsorbent. [ABSTRACT FROM AUTHOR]
- Published
- 2018
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