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Guided 2D exciton-polaritons, resulting from the strong coupling of excitons in semiconductors with non-radiating waveguide modes, provide an attractive approach towards developing novel on-chip optical devices. These quasiparticles are characterized by long propagation distances and efficient nonlinear interaction. However, as guided exciton-polaritons are uncoupled from the free space, it is challenging to investigate them using conventional far-field spectroscopy techniques. Here we demonstrate a powerful approach for probing and manipulating guided polaritons in a Ta$_2$O$_5$ slab integrated with a WS$_2$ monolayer using evanescent coupling through a high-index solid immersion lens. Tuning the nanoscale gap between the lens and the sample, we demonstrate in-situ control over radiative losses and Rabi splitting of guided polaritons at ambient conditions. This extra degree of freedom allows for extracting all the intrinsic parameters of the strongly coupled system under study. Our results enable the future development of integrated optics employing room-temperature exciton-polaritons in 2D semiconductor-based structures.

Deeply subwavelength lasers (or nanolasers) are highly demanded for compact on-chip bioimaging and sensing at the nanoscale. One of the main obstacles for the development of single-particle nanolasers with all three dimensions shorter than the emitting wavelength in the visible range is the high lasing thresholds and the resulting overheating. Here we exploit exciton-polariton condensation and mirror-image Mie modes in a cuboid CsPbBr$_3$ nanoparticle to achieve coherent emission at the visible wavelength of around 0.53~$\mu $m from its ultra-small ($\approx$0.007$\mu$m$^3$ or $\approx\lambda^3$/20) semiconductor nanocavity. The polaritonic nature of the emission from the nanocavity localized in all three dimensions is proven by direct comparison with corresponding one-dimensional and two-dimensional waveguiding systems with similar material parameters. Such a deeply subwavelength nanolaser is enabled not only by the high values for exciton binding energy ($\approx$35 meV), refractive index ($>$2.5 at low temperature), and luminescence quantum yield of CsPbBr$_3$, but also by the optimization of polaritons condensation on the Mie resonances. Moreover, the key parameters for optimal lasing conditions are intermode free spectral range and phonons spectrum in CsPbBr$_3$, which govern polaritons condensation path. Such chemically synthesized colloidal CsPbBr$_3$ nanolasers can be easily deposited on arbitrary surfaces, which makes them a versatile tool for integration with various on-chip systems., Comment: 29 pages, 19 Figures

Systems supporting exciton-polaritons represent solid-state optical platforms with a strong built-in optical nonlinearity provided by exciton-exciton interactions. In conventional semiconductors with hydrogen-like excitons the nonlinearity rate demonstrates the inverse scaling with the binding energy. This makes excitons stable at room temperatures weakly interacting, which obviously limits the possibilities of practical applications of the corresponding materials for nonlinear photonics. We demonstrate experimentally and theoretically, that these limitations can be substantially softened in hybrid perovskites, such as MAPbBr3 due to the crucial role of the polaron effects mediating the inter-particle interactions. The resulting exciton-polaron-polaritons remain both stable and strongly interacting at room temperature, which is confirmed by large nonlinear blueshifts of lower polariton branch energy under resonant femtosecond laser pulse excitation. Our findings open novel perspectives for the management of the exciton-polariton nonlinearities in ambient conditions.

Optical bound states in the continuum (BICs) provide a way to engineer very narrow resonances in photonic crystals. The extended interaction time in such systems is particularly promising for enhancement of nonlinear optical processes and development of the next generation of active optical devices. However, the achievable interaction strength is limited by the purely photonic character of optical BICs. Here, we mix optical BIC in a photonic crystal slab with excitons in atomically thin semiconductor MoSe$_2$ to form nonlinear exciton-polaritons with a Rabi splitting of 27~meV, exhibiting large interaction-induced spectral blueshifts. The asymptotic BIC-like suppression of polariton radiation into far-field towards the BIC wavevector, in combination with effective reduction of excitonic disorder through motional narrowing, results in small polariton linewidths below 3~meV. Together with strongly wavevector-dependent Q-factor, this provides for enhancement and control of polariton--polariton interactions and resulting nonlinear optical effects, paving the way towards tunable BIC-based polaritonic devices for sensing, lasing, and nonlinear optics.

Metasurfaces offer great potential to control near- and far-fields through engineering of optical properties of elementary cells or meta-atoms. Such perspective opens a route to efficient manipulation of the optical signals both at nanoscale and in photonics applications. In this paper we show that by using an effective surface conductivity tensor it is possible to unambigiously describe optical properties of an anisotropic metasurface in the far- and near-field regimes. We begin with retrieving the effective surface conductivity tensor from the comparative analysis of experimental and numerical reflectance spectra of a metasurface composed of elliptical gold nanoparticles. Afterwards restored conductivities are validated in the crosscheck versus semianalytic parameters obtained with the discrete dipole model with and without dipoles interaction contribution. The obtained effective parameters are further used for the dispersion analysis of surface plasmons localized at the metasurface. The effective medium model predicts existence of both TE- and TM-polarized plasmons in a wide range of optical frequencies and describes peculiarities of their dispersion, in particularly, topological transition from the elliptical to hyperbolic regime with eligible accuracy. The analysis in question offers a simple practical way to describe properties of metasurfaces including ones in the near-field zone by extracting effective parameters from the convenient far-field characterisation., Comment: 29 pages, 9 figures

Nanoantennas for highly efficient excitation and manipulation of surface waves at nanoscale are key elements of compact photonic circuits. However, previously implemented designs employ plasmonic nanoantennas with high Ohmic losses, relatively low spectral resolution, and complicated lithographically made architectures. Here we propose an ultracompact and simple dielectric nanoantenna (silicon nanosphere) allowing for both directional launching of surface plasmon polaritons on a thin gold film and their demultiplexing with a high spectral resolution. We show experimentally that mutual interference of magnetic and electric dipole moments supported by the dielectric nanoantenna results in opposite propagation of the excited surface waves whose wavelengths differ by less than 50 nm in the optical range. Broadband reconfigurability of the nanoantennas operational range is achieved simply by varying the diameter of the silicon sphere. Moreover, despite subwavelength size ($, Comment: added relevant references; fixed typos in Supplementary eq. 8,9,11

Photonic structures offer unique opportunities for controlling light-matter interaction, including the photonic spin Hall effect associated with the transverse spin-dependent displacement of light that propagates in specially designed optical media. However, due to small spin-orbit coupling, the photonic spin Hall effect is usually weak at the nanoscale. Here we suggest theoretically and demonstrate experimentally, in both optics and microwave experiments, the photonic spin Hall effect enhanced by topologically protected edge states in subwavelength arrays of resonant dielectric particles. Based on direct near-field measurements, we observe the selective excitation of the topological edge states controlled by the handedness of the incident light. Additionally, we reveal the main requirements to the symmetry of photonic structures to achieve a topology-enhanced spin Hall effect, and also analyse the robustness of the photonic edge states against the long-ranged coupling.

We present the studies on surface-enhanced Raman spectroscopy (SERS) of bacteriorhodopsin in purple membranes using self-assembled silver nanoisland films for Raman signal enhancement. These metal island films were fabricated on soda-lime glass slides subjected to silver-sodium ion exchange in molten Ag 0.05Na 0.95NO 3 at the temperature of 325°C for 20 minutes and subsequent treatment in hydrogen atmosphere at the temperature of 250°C for 10 minutes. The films typically consisted of 20-30 nm closely placed nanoislands. Being tested as SERS substrates for rhodamine 6G the nanoisland films gave the possibility to observe respective characteristic Raman lines from a dried drop of rhodamine 6G dissolved in water in the concentration of 10 -6 M. Similarly fabricated substrates were used to obtain SERS spectra of bacteriorhodopsin in purple membranes dispersed in water, and Raman peaks at 1000-1020 cm -1, 1150-1220 cm -1 and 1530-1570cm -1 were resolved. The substrates made it possible to register characteristic Raman peaks only for an order of magnitude lower concentration of bacteriorhodopsin in contrast to the virgin glass substrate, that is the enhancement of Raman signal was considerably less than for rhodomin 6G. This is supposed to be due to bacteriophodopsin molecules packing in patches, and it prevents bacteriophodopsin in purple membranes from penetration between the nanoislands where the local enhancement of the electric field of exciting light wave is maximal.