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There is debating over the question of whether the large-scale ‘Grain for Green’ program on the Loess Plateau of China threatens regional food security. Self-sufficiency index and cropland pressure index were used to assess food security on the Loess Plateau after the implementation of revegetation program. The results showed that the ‘Grain for Green’ program initially had a considerable impact on regional food security, where grain yield fell from 1999 to 2001, resulting in a lower grain self-sufficiency and increased farmland stress. Subsequently, grain yield in this region increased due to the elevated agricultural material input and increased construction of terraces and check dams. The grain self-sufficiency index would have increased to 96.55% if there were improvements to the agricultural conditions, such as fertilization and irrigation, which would have resulted in an increase in the crop yield per unit of 20%. However, the grain self-sufficiency increased to 105.25% via the construction of terraces and check dams. Thus, the government should further expand the ‘Grain for Green’ program in coordination with improvements to the agricultural production conditions and the construction of terraces and check dams on the Loess Plateau.