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1. Use of GEMAS data for risk assessment of cadmium in European agricultural and grazing land soil under the REACH Regulation

Author

Birke, M., Reimann, C., Oorts, K., Uwe, R., Alecos, D., Dinelli, E., Ladenberger, A., Halamić, J., Mateja, G., Jähne Klingberg, F., Andersson, M., Baritz, R., Batista, M. J., Bel Ian, A., Cicchella, D., De Vos, W., Duris, M., Dusza Dobek, A., Eggen, O. A., Eklund, M., Ernsten, V., Filzmoser, P., Flight, D. M. A., Forrester, S., Fügedi, U., Gilcucis, A., Gregorauskiene, V., De Groot, W., Gulan, A., Haslinger, E., Hayoz, P., Hoogewerff, J., Hrvatovic, H., Husnjak, S., Janik, L., Jordan, G., Kaminari, M., Kirby, J., Klos, V., Kwecko, P., Kuti, L., Locutura, J., Lucivjansky, P., Mann, A., Mackovych, D., Mclaughlin, M., Malyuk, B. I., Maquil, R., Meuli, R. G., Mol, G., Negrel, P., ’Connor, P. O, Ottesen, R. T., Pasnieczna, A., Petersell, V., Pfleiderer, S., Ponavi c, M., Prazeres, C., Radusinovic, S., Salpeteur, I., Scanlon, R., Schedl, A., Scheib, A., Schoeters, I., Sefcik, P., Sellersjo, E., Slaninka, I., Soriano Disla, J. M., Sorsa, A., Svrkota, R., Stafilov, T., Tarvainen, T., Tendavilov, V., Valera, P., Verougstraete, V., Vidojevic, D., Zomeni, Z., Zissimos, A., ALBANESE, STEFANO, DE VIVO, BENEDETTO, LIMA, ANNAMARIA, Birke, M., Reimann, C., Oorts, K., Uwe, R., Alecos, D., Dinelli, E., Ladenberger, A., Halamić, J., Mateja, G., Jähne Klingberg, F., Albanese, Stefano, Andersson, M., Baritz, R., Batista, M. J., Bel Ian, A., Cicchella, D., DE VIVO, Benedetto, De Vos, W., Duris, M., Dusza Dobek, A., Eggen, O. A., Eklund, M., Ernsten, V., Filzmoser, P., Flight, D. M. A., Forrester, S., Fügedi, U., Gilcucis, A., Gregorauskiene, V., De Groot, W., Gulan, A., Haslinger, E., Hayoz, P., Hoogewerff, J., Hrvatovic, H., Husnjak, S., Janik, L., Jordan, G., Kaminari, M., Kirby, J., Klos, V., Kwecko, P., Kuti, L., Lima, Annamaria, Locutura, J., Lucivjansky, P., Mann, A., Mackovych, D., Mclaughlin, M., Malyuk, B. I., Maquil, R., Meuli, R. G., Mol, G., Negrel, P., ’Connor, P. O, Ottesen, R. T., Pasnieczna, A., Petersell, V., Pfleiderer, S., Ponavi c, M., Prazeres, C., Radusinovic, S., Salpeteur, I., Scanlon, R., Schedl, A., Scheib, A., Schoeters, I., Sefcik, P., Sellersjo, E., Slaninka, I., Soriano Disla, J. M., Sorsa, A., Svrkota, R., Stafilov, T., Tarvainen, T., Tendavilov, V., Valera, P., Verougstraete, V., Vidojevic, D., Zomeni, Z., Zissimos, A., Birke, Manfred, Reimann, Clemen, Oorts, Koen, Rauch, Uwe, Demetriades, Aleco, Dinelli, Enrico, Ladenberger, Anna, Halamić, Josip, Gosar, Mateja, and Jähne-Klingberg, Fabian

Subjects
Pollution, agricultural soil, grazing land soil, risk assessment, REACH, cadmium, Soil test, media_common.quotation_subject, chemistry.chemical_element, 010501 environmental sciences, 010502 geochemistry & geophysics, Agricultural soil, 01 natural sciences, Ecology and Environment, Geochemistry and Petrology, Grazing, Environmental Chemistry, Risk assessment, 0105 earth and related environmental sciences, media_common, Hydrology, Cadmium, business.industry, Forestry, Expert group, Chemistry, chemistry, Agriculture, Soil water, Earth Sciences, business, Grazing land soil
Abstract

Over 4000 soil samples were collected for the “Geochemical Mapping of Agricultural and Grazing Land Soil of Europe” (GEMAS) project carried out by the EuroGeoSurveys Geochemistry Expert Group. Cadmium concentrations are reported for the

Published
2016

2. GEMAS: Cadmium distribution and its sources in agricultural and grazing land soil of Europe - Original data versus clr-transformed data

Author

BIRKE M., REIMANN C, RAUCH U., LADENBERGER A., DEMETRIADES A., JÄHNEKLINGBERG F., OORTS K, GOSAR M., DINELLI D., HALAMIĆ J., ALBANESE S., ANDERSSON M., BARITZ R., BATISTA M. J., BEL-IAN A., CICCHELLA D., DE VIVO B., DE VOS W., ĎURIŠ M., DUSZA-DOBEK A., EGGEN O. A., EKLUND M., ERNSTEN V., FILZMOSER, FLIGHT D. M. A., FORRESTER S., FÜGEDI U., GILCUCIS A., GREGORAUSKIENE V., DE GROOT W., GULAN A., HASLINGER E., HAYOZ P., HOOGEWERFF J., HRVATOVIC H., HUSNJAK S., JANIK L., JORDAN G., KAMINARI M., KIRBY J., KLOS V., KWEĆKO P., KUTI L., LIMA A., LOCUTURA J., LUCIVJANSKY P., MANN A., MACKOVYCH D., MCLAUGHLIN M., MALYUK B. I., MAQUIL R., MEULI R. G., MOL G., NÉGREL P., O’CONNOR P., OTTESEN R. T., PASNIECZNA A., PETERSELL V., PFLEIDERER S., POŇAVIČ M., PRAZERES C., RADUSINOVIĆ S., SALPETEUR I., SADEGHI M., SCANLON R., SCHEDL A., SCHEIB A., SCHOETERS I., ŠEFČIK P., SELLERSJÖ E., SLANINKA I., SORIANO-DISLA J. M., ŠORŠA A., SVRKOTA R., STAFILOV T., TARVAINEN T., TENDAVILOV V., VALERA P., VEROUGSTRAETE V., VIDOJEVIĆ D., ZOMENI Z., ZISSIMOS A., Birke, Manfred, Reimann, Clemen, Rauch, Uwe, Ladenberger, Anna, Demetriades, Aleco, Jähne-Klingberg, Fabian, Oorts, Koen, Gosar, Mateja, Dinelli, Enrico, Halamić, Josip, Birke, M., Reimann, C, Rauch, U., Ladenberger, A., Demetriades, A., Jähneklingberg, F., Oorts, K, Gosar, M., Dinelli, D., Halamić, J., Albanese, S., Andersson, M., Baritz, R., Batista, M. J., BEL-IAN, A., Cicchella, D., DE VIVO, B., DE VOS, W., Ďuriš, M., DUSZA-DOBEK, A., Eggen, O. A., Eklund, M., Ernsten, V., Filzmoser, Flight, D. M. A., Forrester, S., Fügedi, U., Gilcucis, A., Gregorauskiene, V., DE GROOT, W., Gulan, A., Haslinger, E., Hayoz, P., Hoogewerff, J., Hrvatovic, H., Husnjak, S., Janik, L., Jordan, G., Kaminari, M., Kirby, J., Klos, V., Kwećko, P., Kuti, L., Lima, A., Locutura, J., Lucivjansky, P., Mann, A., Mackovych, D., Mclaughlin, M., Malyuk, B. I., Maquil, R., Meuli, R. G., Mol, G., Négrel, P., O’Connor, P., Ottesen, R. T., Pasnieczna, A., Petersell, V., Pfleiderer, S., Poňavič, M., Prazeres, C., Radusinović, S., Salpeteur, I., Sadeghi, M., Scanlon, R., Schedl, A., Scheib, A., Schoeters, I., Šefčik, P., Sellersjö, E., Slaninka, I., SORIANO-DISLA, J. M., Šorša, A., Svrkota, R., Stafilov, T., Tarvainen, T., Tendavilov, V., Valera, P., Verougstraete, V., Vidojević, D., Zomeni, Z., and Zissimos, A.

Subjects
Cadmium, Agricultural soil, Compositional data analysis, PCA, Continental-scale geochemical mapping, Europe, Soil test, Weathering, 010501 environmental sciences, 010502 geochemistry & geophysics, 01 natural sciences, Compositional data analysi, chemistry.chemical_compound, Geochemistry and Petrology, Grazing, Aqua regia, Glacial period, 0105 earth and related environmental sciences, Hydrology, business.industry, Anomaly (natural sciences), chemistry, Agriculture, Economic Geology, Quaternary, business, Geology
Abstract

Over 4000 agricultural and grazing land soil samples were collected for the “Geochemical Mapping of Agricultural and Grazing Land Soil of Europe” (GEMAS) project carried out by the EuroGeoSurveys Geochemistry Expert Group. The samples were collected in 33 European countries, covering 5.6 million km 2 at a density of 1 sample site per 2500 km 2 . All samples were analysed by ICP-MS following an aqua regia extraction. The European median Cd concentration is 0.182 mg/kg in agricultural soil and 0.197 mg/kg in grazing land soil (including eastern Ukraine). The Cd map demonstrates the existence of two different geochemical background regimes in northern and southern Europe, separated by the southern limit of the Quaternary glaciation. Cadmium shows two times higher background concentrations in the older and more weathered southern European soil than in northern European soil. The spatial distribution patterns of Cd in the collected soil samples are mainly governed by geology (parent material and mineralisation), as well as weathering, soil formation and climate since the last glaciation period. Locally, in several areas, the natural anomaly pattern is overprinted by anthropogenic emissions from former mining, ore processing and related metal industries. Some Cd anomalies can be attributed to urbanisation and the use of fertilisers. A comparison of the raw data Cd concentration map with its clr-transformed counterpart and selected single element ratio maps demonstrates that substantial additional information about sources and processes governing the distribution of Cd in agricultural soil at the European scale can be obtained. Results of a PCA, carried out following the classical approach (standardised) versus a PCA based on the statistically acceptable approach, using clr-transformed data, are quite comparable.

Published
2017

3. GEMAS: CNS concentrations and C/N ratios in European agricultural soil

Author

G. Jordan, Andreas Scheib, Rolf Tore Ottesen, Clemens Reimann, S. Pfleiderer, E. Sellersjö, P. Hayoz, O. A. Eggen, Timo Tarvainen, Mike J. McLaughlin, M. Poňavič, V. Tendavilov, A. Bel-Ian, Alecos Demetriades, B. De Vivo, M. Eklund, Jurian Hoogewerff, Jason K. Kirby, S. Forrester, D. Mackovych, R. Maquil, Stjepan Husnjak, Rainer Baritz, Dee Flight, W. De Groot, G. Mol, Karl Fabian, V. Klos, A. Gilucis, D. Vidojević, Z. Zomeni, I. Schoeters, J. Locutura, U. Rauch, Koen Oorts, Jörg Matschullat, P. Sefcik, B. I. Malyuk, A. Schedl, M. Kaminari, H. Hrvatovic, Maria João Batista, Josip Halamić, I. Salpeteur, V. Ernsten, Andreas M. Zissimos, José M. Soriano-Disla, P. Kwecko, R. Svrkota, V. Gregorauskiene, Domenico Cicchella, S. Radusinović, A. Dusza-Dobek, U. Fugedi, A. Gulan, Enrico Dinelli, W. De Vos, V. Verougstraete, Stefano Albanese, R. G. Meuli, L. Janik, A. Pasnieczna, Paolo Valera, Fabian Jähne-Klingberg, I. Slaninka, Anna Ladenberger, Mateja Gosar, E. Haslinger, Peter Filzmoser, M. Ďuriš, Philippe Négrel, P. O'Connor, Martiya Sadeghi, M. Anderson, Trajče Stafilov, P. Lucivjansky, Debora dos Santos Carvalho, Annamaria Lima, R. Scanlon, C. Prazeres, A. Mann, Ajka Šorša, Manfred Birke, L. Kuti, V. Petersell, Matschullat, Jörg, Reimann, Clemen, Birke, Manfred, dos Santos Carvalho, Debora, Albanese, S., Anderson, M., Baritz, R., Batista, M.J., Bel-Ian, A., Cicchella, D., Demetriades, A., De Vivo, B., De Vos, W., Dinelli, E., Ďuriš, M., Dusza-Dobek, A., Eggen, O.A., Eklund, M., Ernsten, V., Fabian, K., Filzmoser, P., Flight, D.M.A., Forrester, S., Fügedi, U., Gilucis, A., Gosar, M., Gregorauskiene, V., De Groot, W., Gulan, A., Halamić, J., Haslinger, E., Hayoz, P., Hoogewerff, J., Hrvatovic, H., Husnjak, S., Jähne-Klingberg, F., Janik, L., Jordan, G., Kaminari, M., Kirby, J., Klos, V., Kwećko, P., Kuti, L., Ladenberger, A., Lima, A., Locutura, J., Lucivjansky, P., Mann, A., Mackovych, D., McLaughlin, M., Malyuk, B.I., Maquil, R., Meuli, R.G., Mol, G., Négrel, P., O'Connor, P., Oorts, K., Ottesen, R.T., Pasnieczna, A., Petersell, V., Pfleiderer, S., Poňavič, M., Prazeres, C., Radusinović, S., Rauch, U., Sadeghi, M., Salpeteur, I., Scanlon, R., Schedl, A., Scheib, A., Schoeters, I., Šefčik, P., Sellersjö, E., Slaninka, I., Soriano-Disla, J.M., Šorša, A., Svrkota, R., Stafilov, T., Tarvainen, T., Tendavilov, V., Valera, P., Verougstraete, V., Vidojević, D., Zissimos, A., Zomeni, Z., Batista, M. J., Eggen, O. A., Flight, D. M. A., Mclaughlin, M., Malyuk, B. I., Meuli, R. G., Ottesen, R. T., and Soriano-Disla, J. M.

Subjects
Pollution, Environmental Engineering, 010504 meteorology & atmospheric sciences, Nitrogen, media_common.quotation_subject, 010501 environmental sciences, Spatial distribution, 01 natural sciences, Lower limit, Total organic carbon (TOC), Sulphur, Environmental Chemistry, Sampling density, Carbon, GEMAS project, Arable soil, Waste Management and Disposal, 0105 earth and related environmental sciences, media_common, 2. Zero hunger, business.industry, Sampling (statistics), 15. Life on land, Eastern european, Chemistry, Agriculture and Soil Science, 13. Climate action, Agriculture, Total nitrogen, Earth Sciences, Environmental science, Physical geography, business
Abstract

A reliable overview of measured concentrations of TC, TN and TS, TOC/TN ratios, and their regional distribution patterns in agricultural soil at the continental scale and based on measured data has been missing - despite much previous work on local and the European scales. Detection and mapping of natural (ambient) background element concentrations and variability in Europe was the focus of this work. While total C and S data had been presented in the GEMAS atlas already, this work delivers more precise (lower limit of determination) and fully quantitative data, and for the first time high-quality TN data. Samples were collected from the uppermost 20 cm of ploughed soil (Ap horizon) at 2108 sites with an even sampling density of one site per 2500 km2 for one individual land-use class (agricultural) across Europe (33 countries). Laboratory-independent quality control from sampling to analysis guaranteed very good data reliability and accuracy. Total carbon concentrations ranged from 0.37 to 46.3 wt% (median: 2.20 wt%) and TOC from 0.40 to 46.0 wt% (median: 1.80 wt%). Total nitrogen ranged from 0.018 to 2.64 wt% (median: 0.169 wt%) and TS from 0.008 to 9.74 wt% (median: 0.034 wt%), all with large variations in most countries. The TOC/TN ratios ranged from 1.8 to 252 (median: 10.1), with the largest variation in Spain and the smallest in some eastern European countries. Distinct and repetitive patterns emerge at the European scale, reflecting mostly geogenic and longer-term climatic influence responsible for the spatial distribution of TC, TN and TS. Different processes become visible at the continental scale when examining TC, TN and TS concentrations in agricultural soil Europe-wide. This facilitates large-scale land-use management and allows specific areas (subregional to local) to be identified that may require more detailed research.

Published
2018

4. GEMAS: establishing geochemical background and threshold for 53 chemical elements in European agricultural soil

Author

Clemens Reimann, S. Radusinović, U. Fugedi, E. Sellersjö, W. De Vos, I. Schoeters, V. Verougstraete, O. A. Eggen, D. Vidojević, Enrico Dinelli, U. Rauch, Rolf Tore Ottesen, Andreas M. Zissimos, G. Jordan, Andreas Scheib, V. Tendavilov, Anna Ladenberger, José M. Soriano-Disla, Timo Tarvainen, Karl Fabian, Jurian Hoogewerff, R. Maquil, A. Dusza-Dobek, Koen Oorts, Annamaria Lima, P. Hayoz, W. De Groot, G. Mol, L. Janik, Josip Halamić, Jörg Matschullat, B. I. Malyuk, Z. Zomeni, A. Schedl, S. Pfleiderer, Alecos Demetriades, A. Pasnieczna, P. Kwecko, R. Svrkota, Domenico Cicchella, V. Gregorauskiene, R. G. Meuli, M. Poňavič, Maria João Batista, R. Scanlon, A. Gilucis, M. Eklund, Mike J. McLaughlin, M. Ďuriš, Philippe Négrel, Patrice de Caritat, Jason K. Kirby, Stefano Albanese, Martiya Sadeghi, C. Prazeres, M. Kaminari, M. Anderson, Trajče Stafilov, Dee Flight, A. Mann, Ajka Šorša, Mateja Gosar, Paolo Valera, P. Lucivjansky, Manfred Birke, L. Kuti, V. Petersell, Fabian Jähne-Klingberg, E. Haslinger, P. O'Connor, V. Klos, V. Ernsten, A. Bel-Ian, I. Slaninka, Peter Filzmoser, B. De Vivo, Stjepan Husnjak, Rainer Baritz, H. Hrvatovic, I. Salpeteur, J. Locutura, S. Forrester, D. Mackovych, A. Gulan, P. Sefcik, Geological Survey of Norway (NGU), Geological Survey of Norway, Federal Institute for Geosciences and Natural Resources (BGR), Institute of Statistics and Mathematical Methods in Economics, Institute of Geology and Mineral Exploration (IGME), IGME, Bureau de Recherches Géologiques et Minières (BRGM) (BRGM), Université Catholique de Louvain = Catholic University of Louvain (UCL), Bundesanstalt für Geowissenschaften und Rohstoffe (BGR), Departimento di Scienze della Terra [Napoli], Università degli studi di Napoli Federico II, Dipartimento di Scienze Biologiche, Geologiche e Ambientali (BiGeA), Alma Mater Studiorum Università di Bologna [Bologna] (UNIBO), Institut Gilbert-Laustriat : Biomolécules, Biotechnologie, Innovation Thérapeutique, Université Louis Pasteur - Strasbourg I-Centre National de la Recherche Scientifique (CNRS), Université de Nice Sophia-Antipolis (UNSA), Geological Survey of Sweden, sgu, Centre de résonance magnétique biologique et médicale (CRMBM), Aix Marseille Université (AMU)-Assistance Publique - Hôpitaux de Marseille (APHM)-Centre National de la Recherche Scientifique (CNRS), Reimann, Clemen, Fabian, Karl, Birke, Manfred, Filzmoser, Peter, Demetriades, Aleco, Négrel, Philippe, Oorts, Koen, Matschullat, Jörg, de Caritat, Patrice, Albanese, S., Anderson, M., Baritz, R., Batista, M.J., Bel-Ian, A., Cicchella, D., De Vivo, B., De Vos, W., Dinelli, E., Ďuriš, M., Dusza-Dobek, A., Eggen, O.A., Eklund, M., Ernsten, V., Flight, D.M.A., Forrester, S., Fügedi, U., Gilucis, A., Gosar, M., Gregorauskiene, V., De Groot, W., Gulan, A., Halamić, J., Haslinger, E., Hayoz, P., Hoogewerff, J., Hrvatovic, H., Husnjak, S., Jähne-Klingberg, F., Janik, L., Jordan, G., Kaminari, M., Kirby, J., Klos, V., Kwećko, P., Kuti, L., Ladenberger, A., Lima, A., Locutura, J., Lucivjansky, P., Mann, A., Mackovych, D., McLaughlin, M., Malyuk, B.I., Maquil, R., Meuli, R.G., Mol, G., O'Connor, P., Ottesen, R.T., Pasnieczna, A., Petersell, V., Pfleiderer, S., Poňavič, M., Prazeres, C., Radusinović, S., Rauch, U., Salpeteur, I., Scanlon, R., Schedl, A., Scheib, A., Schoeters, I., Šefčik, P., Sellersjö, E., Slaninka, I., Soriano-Disla, J.M., Šorša, A., Svrkota, R., Stafilov, T., Tarvainen, T., Tendavilov, V., Valera, P., Verougstraete, V., Vidojević, D., Zissimos, A., Zomeni, Z., Sadeghi, M., Reimann, C., Fabian, K., Birke, M., Filzmoser, P., Demetriades, A., Negrel, P., Oorts, K., Matschullat, J., de Caritat, P., Batista, M. J., Duris, M., Eggen, O. A., Flight, D. M. A., Fugedi, U., Halamic, J., Jahne-Klingberg, F., Kwecko, P., Mclaughlin, M., Malyuk, B. I., Meuli, R. G., Ottesen, R. T., Ponavic, M., Radusinovic, S., Sefcik, P., Sellersjo, E., Soriano-Disla, J. M., Sorsa, A., and Vidojevic, D.

Subjects
Soil test, Geochemical threshold, 010501 environmental sciences, Spatial distribution, 01 natural sciences, Agricultural soil, Ecology and Environment, chemistry.chemical_compound, Geochemistry and Petrology, Environmental Chemistry, Aqua regia, Continental scale, ComputingMilieux_MISCELLANEOUS, 0105 earth and related environmental sciences, Hydrology, business.industry, 04 agricultural and veterinary sciences, 15. Life on land, Contamination, Pollution, Europe, Chemistry, chemistry, Agriculture and Soil Science, 13. Climate action, Agriculture, [SDU]Sciences of the Universe [physics], Environmental chemistry, Smelting, [SDE]Environmental Sciences, 040103 agronomy & agriculture, Earth Sciences, 0401 agriculture, forestry, and fisheries, Environmental science, business, Background variation
Abstract

The GEMAS (geochemical mapping of agricultural soil) project collected 2108 Ap horizon soil samples from regularly ploughed fields in 33 European countries, covering 5.6 million km(2). The

Published
2018
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