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We develop a general theory describing the thermodynamical behavior of open quantum systems coupled to thermal baths beyond perturbation theory. Our approach is based on the exact time-local quantum master equation for the reduced open system states, and on a principle of minimal dissipation. This principle leads to a unique prescription for the decomposition of the master equation into a Hamiltonian part representing coherent time evolution and a dissipator part describing dissipation and decoherence. Employing this decomposition we demonstrate how to define work, heat and entropy production, formulate the first and second law of thermodynamics, and establish the connection between violations of the second law and quantum non-Markovianity., 7 pages, 2 figures. v2: small modifications in the text, references added, example model added

When driven by a potential bias between two finite reservoirs, the particle current across a quantum system evolves from an initial loading through a coherent, followed by a metastable phase, and ultimately fades away upon equilibration. We formulate a theory which fully accounts for the associated, distinct time scales, and identifies the parameter dependence of the decay rate which ultimately controls the convergence towards equilibrium. Our formalism guarantees total particle number conservation and fundamental consistency between macroscopic and internal currents flowing in the system. We furthermore establish a clear imprint of the fermionic or bosonic particle character on the resulting conductance., Comment: 6 pages, 4 figures

How can we detect that our local, controllable quantum system is correlated with some other inaccessible environmental system? The local detection method developed in recent years allows to realize a dynamical witness for correlations without requiring knowledge of or access to the environment that is correlated with the local accessible quantum system. Here, we provide a brief summary of the theoretical method and recent experimental studies with single photons and trapped ions coupled to increasingly complex environments., 12 pages, 3 figures

Trapped atomic ions enable a precise quantification of the flow of information between internal and external degrees of freedom by employing a non-Markovianity measure [H.-P. Breuer et al., Phys. Rev. Lett. 103, 210401 (2009)]. We reveal that the nature of projective measurements in quantum mechanics leads to a fundamental, nontrivial bias in this measure. We observe and study the functional dependence of this bias to permit a demonstration of applications of local quantum probing. An extension of our approach can act as a versatile reference, relevant for understanding complex systems., Comment: 10 pages (incl. Supplemental Material), 8 figures

Mixing dynamical maps describing open quantum systems can lead from Markovian to non-Markovian processes. Being surprising and counter-intuitive, this result has been used as argument against characterization of non-Markovianity in terms of information exchange. Here, we demonstrate that, quite the contrary, mixing can be understood in a natural way which is fully consistent with existing theories of memory effects. In particular, we show how mixing-induced non-Markovianity can be interpreted in terms of the distinguishability of quantum states, system-environment correlations and the information flow between system and environment., Comment: 10 pages, 8 figures

Quantum discord in a bipartite system can be dynamically revealed and quantified through purely local operations on one of the two subsystems. To achieve this, the local detection method harnesses the influence of initial correlations on the reduced dynamics of an interacting bipartite system. This article's aim is to provide an accessible introduction to this method and to review recent theoretical and experimental progress., 24 pages, 11 figures

The dynamical behavior of open quantum systems plays a key role in many applications of quantum mechanics, examples ranging from fundamental problems, such as the environment-induced decay of quantum coherence and relaxation in many-body systems, to applications in condensed matter theory, quantum transport, quantum chemistry and quantum information. In close analogy to a classical Markov process, the interaction of an open quantum system with a noisy environment is often modelled by a dynamical semigroup with a generator in Lindblad form, which describes a memoryless dynamics leading to an irreversible loss of characteristic quantum features. However, in many applications open systems exhibit pronounced memory effects and a revival of genuine quantum properties such as quantum coherence and correlations. Here, recent results on the rich non-Markovian quantum dynamics of open systems are discussed, paying particular attention to the rigorous mathematical definition, to the physical interpretation and classification, as well as to the quantification of memory effects. The general theory is illustrated by a series of examples. The analysis reveals that memory effects of the open system dynamics reflect characteristic features of the environment which opens a new perspective for applications, namely to exploit a small open system as a quantum probe signifying nontrivial features of the environment it is interacting with. This article further explores the various physical sources of non-Markovian quantum dynamics, such as structured spectral densities, nonlocal correlations between environmental degrees of freedom and correlations in the initial system-environment state, in addition to developing schemes for their local detection. Recent experiments on the detection, quantification and control of non-Markovian quantum dynamics are also discussed., 26 pages, 10 figures

We present a scheme allowing to access the squeezing parameter of multimode fields by means of the dynamics of nonlocal quantum probes. The model under consideration is composed of two two-level systems which are coupled locally to an environment consisting of nonlocally correlated field modes given by two-mode Gaussian states. Introducing independently switchable interactions, one observes revivals of nonlocal coherences of the two-qubit system which are unambiguously connected to the squeezing parameter of the Gaussian environmental states. Thus, the locally interacting two two-level systems represent a dynamical quantum probe for the squeezing in multimode fields. It is finally demonstrated that perfectly reviving nonlocal coherences also persists for nonentangled correlated field modes and an explanation for this phenomenon is presented by connecting it to the correlation coefficient of the environmental coupling operators., Comment: 16 pages, 7 figures; title and some sections changed in published version

We review the model of two qubits coupled locally to an environment which consists of nonlocally correlated field modes [Phys. Rev.Lett. 108, 210402 (2012)]. We derive the correct expressions for the reduced dynamics of the two-qubit system and demonstrate that strong nonlocal memory effects are indeed present for suitable initial EPR-type Gaussian environmental states., 6 pages, 1 figure

We discuss the conceptually different definitions used for the non-Markovianity of classical and quantum processes. The well-established definition for non-Markovianity of a classical stochastic process represents a condition on the Kolmogorov hierarchy of the n-point joint probability distributions. Since this definition cannot be transferred to the quantum regime, quantum non-Markovianity has recently been defined and quantified in terms of the underlying quantum dynamical map, using either its divisibility properties or the behavior of the trace distance between pairs of initial states. Here, we investigate and compare these definitions and their relations to the classical notion of non-Markovianity by employing a large class of non-Markovian processes, known as semi-Markov processes, which admit a natural extension to the quantum case. A number of specific physical examples is constructed which allow to study the basic features of the classical and the quantum definitions and to evaluate explicitly the measures for quantum non-Markovianity. Our results clearly demonstrate several fundamental distinctions between the classical and the quantum notion of non-Markovianity, as well as between the various quantum measures for non-Markovianity., Comment: 15 pages, 6 figures

Efficient methods for the description of the non-Markovian dynamics of open systems play an important role in many proposed applications of quantum mechanics. Here we review some of the most important tools that are based on the projection operator techniques of nonequilibrium statistical mechanics. The standard product-state projection is generalized to a new class of correlated projection superoperators that allow the treatment of strong memory effects, and lead to a non-Markovian generalization of the Lindblad equation., 10 pages, to appear in Lecture Notes in Physics, Springer-Verlag

It is shown that the exact dynamics of a composite quantum system can be represented through a pair of product states which evolve according to a Markovian random jump process. This representation is used to design a general Monte Carlo wave function method that enables the stochastic treatment of the full non-Markovian behavior of open quantum systems. Numerical simulations are carried out which demonstrate that the method is applicable to open systems strongly coupled to a bosonic reservoir, as well as to the interaction with a spin bath. Full details of the simulation algorithms are given, together with an investigation of the dynamics of fluctuations. Several potential generalizations of the method are outlined., 14 pages, 5 figures

The non-Markovian behaviour of open quantum systems interacting with a reservoir can often be described in terms of a time-local master equation involving a time-dependent generator which is not in Lindblad form. A systematic perturbation expansion of the generator is obtained either by means of van Kampen's method of ordered cumulants or else by use of the Feynman-Vernon influence functional technique. Both expansions are demonstrated to yield equivalent expressions for the generator in all orders of the system-reservor coupling. Explicit formulae are derived for the second and the fourth order generator in terms of the influence functional., Comment: 10 pages, to be published in Quantum Computing and Quantum Bits in Mesoscopic Systems (Kluwer Academic Plenum Publishers, december 2002)