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We perform switching current measurements of planar Josephson junctions (JJs) coupled by a common superconducting electrode, with independent control over the two superconducting phase differences. We observe an anomalous phase shift in the current--phase relation of a JJ as a function of gate voltage or phase difference in the second JJ. This demonstrates a nonlocal Josephson effect, and the implementation of a $\varphi_0$-junction which is tunable both electrostatically and magnetically. The anomalous phase shift was larger for shorter distances between the JJs and vanished for distances much longer than the superconducting coherence length. Results are consistent with the hybridization of ABSs, leading to the formation of an Andreev molecule. Our devices constitute a realization of a tunable superconducting phase source, and could enable new coupling schemes for hybrid quantum devices.

Hybrid Josephson junctions with three or more superconducting terminals coupled to a semiconducting region are expected to exhibit a rich variety of phenomena. Andreev bound states (ABSs) arising in such multiterminal devices have been predicted to form unconventional energy band structures, which can be engineered by controlling superconducting phase differences between the individual terminals. Here we report tunnelling spectroscopy measurements of three-terminal Josephson junctions (3TJJs) realised in a gate-tunable InAs/Al heterostructure. The three terminals are connected to form two loops where phase differences are independently controlled. Our results provide a demonstration of phase control over a novel Andreev band structure. Signatures of hybridisation between ABSs, consistent with their overlap in the 3TJJ region, are observed in the form of avoided crossings in the spectrum and are well explained by a numerical model. Future extensions of this work could focus on addressing spin-resolved energy levels, ground state parity transitions and Weyl bands in multiterminal geometries.

Light-matter interaction enables engineering of non-equilibrium quantum systems. In condensed matter, spatially and temporally cyclic Hamiltonians are expected to generate energy-periodic Floquet states, with properties inaccessible at thermal equilibrium. A recent work explored the tunnelling conductance of a planar Josephson junction under microwave irradiation, and interpreted replicas of conductance features as evidence of steady Floquet-Andreev states. Here we realise a similar device in a hybrid superconducting-semiconducting heterostructure, which utilises a tunnelling probe with gate-tunable transparency and allows simultaneous measurements of Andreev spectrum and current-phase relation of the planar Josephson junction. We show that, in our devices, spectral replicas in sub-gap conductance emerging under microwave irradiation are caused by photon assisted tunnelling of electrons into Andreev states. The current-phase relation under microwave irradiation is also explained by the interaction of Andreev states with microwave photons, without the need to invoke Floquet states. The techniques outlined in this study establish a baseline to distinguish photon assisted tunnelling from Floquet-Andreev states in mesoscopic devices, a crucial development towards understanding light-matter coupling in hybrid nanostructures.

Motivated by recent scanning tunneling microscopy experiments on single magnetic impurities on superconducting surfaces, we present here a comprehensive theoretical study of the interplay between Yu-Shiba-Rusinov bound states and (multiple) Andreev reflections. Our theory is based on a combination of an Anderson model with broken spin degeneracy and nonequilibrium Green's function techniques that allows us to describe the electronic transport through a magnetic impurity coupled to superconducting leads for arbitrary junction transparency. Using this combination we are able to elucidate the different tunneling processes that give a significant contribution to the subgap transport. In particular, we predict the occurrence of a large variety of Andreev reflections mediated by Yu-Shiba-Rusinov bound states that clearly differ from the standard Andreev processes in non-magnetic systems. Moreover, we provide concrete guidelines on how to experimentally identify the subgap features originating from these tunneling events. Overall, our work provides new insight into the role of the spin degree of freedom in Andreev transport physics., 15 pages, 10 figures

We present an ab-initio method to simulate the current noise in the presence of electron-vibration interactions in atomic and molecular junctions at finite temperature. Using a combination of nonequilibrium Keldysh Green's function techniques and density functional theory, we study the elastic and inelastic contributions to electron current and shot noise within a wide range of transmission values in systems exhibiting multiple electronic levels and vibrational modes. Within our model we find the upper threshold, at which the inelastic noise contribution changes sign, at a total transmission between $\tau\approx 0.90$ and $0.95$ for gold contacts. This is higher than predicted by the single-level Holstein model but in agreement with earlier experimental observations. We support our theoretical studies by noise measurements on single-atom gold contacts which confirm previous experiments but make use of a new setup with strongly reduced complexity of electronic circuitry. Furthermore, we identify 1,4-benzenedithiol connected to gold electrodes as a system to observe the lower sign change, which we predict at around $\tau\approx 0.2$. Finally, we discuss the influence of vibrational heating on the current noise., Comment: 14 pages, 7 figures

Because of the broken time-translation symmetry, in periodically driven vibrational systems fluctuations of different vibration components have different intensities. Fluctuations of one of the components are often squeezed, whereas fluctutions of the other component, which is shifted in phase by π/2, are increased. Squeezing is a multi-faceted phenomenon, it attracts much attention from the perspective of high-precision measurements. Here we demonstrate a new and hitherto unappreciated side of squeezing: its direct manifestation in the spectra of driven vibrational systems. With a weakly damped nanomechanical resonator, we study the spectrum of thermal fluctuations of a resonantly driven nonlinear mode. In the attained sideband-resolved regime, we show that the asymmetry of the spectrum directly characterizes the squeezing. This opens a way to deduce squeezing of thermal fluctuations in strongly underdamped resonators, for which a direct determination by a standard homodyne measurement is impeded by frequency fluctuations. The experimental and theoretical results are in excellent agreement. We further extend the theory to also describe the spectral manifestation of squeezing of quantum fluctuations. published

We study the effects of spin-splitting and spin-flip scattering in a superconductor (S) on the thermoelectric properties of a tunneling contact to a metallic ferromagnet (F) using the Green's function method. A giant thermopower has been theoretically predicted and experimentally observed in such structures. This is attributed to the spin-dependent particle-hole asymmetry in the tunneling density of states in the S/F heterostructure. Here, we evaluate the S density of states and thermopower for a range of temperatures, Zeeman-splitting, and spin-flip scattering. In contrast to the naive expectation based on the negative effect of spin-flip scattering on Cooper pairing, we find that the spin-flip scattering strongly enhances the thermoelectric performance of the system in the low-field and low-temperature regime. This is attributed to a complex interplay between the charge and spin conductances caused by the softening of the spin-dependent superconducting gaps. The maximal value of the thermopower exceeds $k_{B}/e$ by a factor of $\approx$ 5 and has a nonmonotonic dependence on spin-splitting and spin-flip rate., 10 pages, 6 figures

Transport in superconducting heterostructures is very successfully described with quasiclassical Green's functions augmented by microscopically derived boundary conditions. However, so far the spin-dependence is in the diffusive approach included only for limiting cases. Here, we derive the fully spin-dependent boundary condition completing the Usadel equation and the circuit theory. Both, material specific spin-degrees of freedom and spin-dependent interface effects, i.e. spin-mixing and polarization of the transmission coefficients are treated exactly. This opens the road to accurately describe a completely new class of mesoscopic circuits including materials with strong intrinsic magnetic structure. We also discuss several experimentally relevant cases like the tunnel limit, a ferromagnetic insulator with arbitrarily strong magnetization and the limit of small spin-mixing., Comment: 5 pages

The usually negligibly small thermoelectric effects in superconducting heterostructures can be boosted dramatically due to the simultaneous effect of spin splitting and spin filtering. Building on an idea of our earlier work [Phys. Rev. Lett. $\textbf{110}$, 047002 (2013)], we propose realistic mesoscopic setups to observe thermoelectric effects in superconductor heterostructures with ferromagnetic interfaces or terminals. We focus on the Seebeck effect being a direct measure of the local thermoelectric response and find that a thermopower of the order of $\sim200$ $\mu V/K$ can be achieved in a transistor-like structure, in which a third terminal allows to drain the thermal current. A measurement of the thermopower can furthermore be used to determine quantitatively the spin-dependent interface parameters that induce the spin splitting. For applications in nanoscale cooling we discuss the figure of merit for which we find enormous values exceeding 1 for temperature $\lesssim 1$K.

The quasiclassical theory of superconductivity provides the most successful description of diffusive heterostructures comprising superconducting elements, namely, the Usadel equations for isotropic Green’s functions. Since the quasiclassical and isotropic approximations break down close to interfaces, the Usadel equations have to be supplemented with boundary conditions for isotropic Green’s functions (BCIGF), which are not derivable within the quasiclassical description. For a long time, the BCIGF were available only for spin-degenerate tunnel contacts, which posed a serious limitation on the applicability of the Usadel description to modern structures containing ferromagnetic elements. In this paper, we close this gap and derive spin-dependent BCIGF for a contact encompassing superconducting and ferromagnetic correlations. This finally justifies several simplified versions of the spin-dependent BCIGF, which have been used in the literature so far. In the general case, our BCIGF are valid as soon as the quasiclassical isotropic approximation can be performed. However, their use requires the knowledge of the full scattering matrix of the contact, an information usually not available for realistic interfaces. In the case of a weakly polarized tunnel interface, the BCIGF can be expressed in terms of a few parameters, i.e., the tunnel conductance of the interface and five conductancelike parameters accounting for the spin dependence of the interface scattering amplitudes. In the case of a contact with a ferromagnetic insulator, it is possible to find explicit BCIGF also for stronger polarizations. The BCIGF derived in this paper are sufficiently general to describe a variety of physical situations and may serve as a basis for modeling realistic nanostructures.

We report on electrical transport measurements through a carbon nanotube quantum dot coupled to a normal and a superconducting lead. The ratio of Kondo temperature and superconducting gap $T_{K}/\Delta$ is identified to govern the transport properties of the system. In the case of $T_{K}\Delta$ the conductance resonance persists, however the conductance is not enhanced compared to the normal state due to a relative asymmetry of the lead-dot couplings. Within this limit the data is in agreement with a simple model of a resonant SN-interface., Comment: 4 pages, 2 figures. submitted to the Proc. Rencontres de Moriond on Quantum Information and Decoherence in Nanosystems 2004

We consider a single-electron transistor (SET) whose central island is a nanomechanical oscillator. The gate capacitance of the SET depends on the mechanical displacement, thus, the vibrations of the island vibrations may strongly influence the current-voltage characteristics, current noise, and higher cumulants of the current. Harmonic oscillations of the island and oscillations with random amplitude (e.g., due to the thermal activation) change the transport characteristics in a different way. The noise spectrum has a peak at the frequency of the island oscillations; when the island oscillates harmonically, the peak reduces to a $\delta$-peak. We show that knowledge of the SET transport properties helps to determine in what way the island oscillates, to estimate the amplitude, and the frequency of the oscillations.

Full counting statistics is a fundamentally new concept in quantum transport. After a review of basic statistics theory, we introduce the powerful Green's function approach to full counting statistics. To illustrate the concept we consider a number of examples. For generic two-terminal contacts we show how counting statistics elucidates the common (and different) features of transport between normal and superconducting contacts. Finally, we demonstrate how correlations in multi-terminal structures are naturally included in the formalism., 20 pages, proceedings of Summer School/Conference on Functional Nanostructures, Karlsruhe (2003)

We investigate the Josephson effect in S$_{\rm F}$XS$_{\rm F}$ junctions, where S$_{\rm F}$ is a superconducting material with a ferromagnetic exchange field, and X a weak link. The critical current $I_c$ increases with the (antiparallel) exchange fields if the distribution of transmission eigenvalues of the X-layer has its maximum weight at small values. This exchange field enhancement of the supercurrent does not exist if X is a diffusive normal metal. At low temperatures, there is a correspondence between the critical current in an S$_{\rm F}$IS$_{\rm F}$ junction with collinear orientations of the two exchange fields, and the AC supercurrent amplitude in an SIS tunnel junction. The difference of the exchange fields $h_1-h_2$ in an S$_{\rm F}$IS$_{\rm F}$ junction corresponds to the potential difference $V_1-V_2$ in an SIS junction; i.e., the singularity in $I_c$ [in an S$_{\rm F}$IS$_{\rm F}$ junction] at $|h_1-h_2|=\Delta_1+\Delta_2$ is the analogue of the Riedel peak. We also discuss the AC Josephson effect in S$_{\rm F}$IS$_{\rm F}$ junctions., Comment: 5 pages, 5 figures

The article develops a powerful theoretical tool to obtain the full counting statistics. By a slight extension of the standard Keldysh method we can access immediately all correlation functions of the current operator. Embedded in a quantum generalization of the circuit theory of electronic transport, we are able to study the full counting statistics of a large class of two-terminal contacts and multi-terminal structures, containing superconductors and normal metals as elements. The practical use of the method is demonstrated in many examples., Comment: 35 pages, contribution to "Quantum Noise", ed. by Yu.V. Nazarov and Ya.M. Blanter, minor changes in text, references added

Electronic properties of mesoscopic systems made of normal metal in contact with normal and superconducting reservoirs are determined by Andreev Reflection. We address both experimentally and theoretically how Andreev Reflection manifests itself in shot noise experiments and what physics can be deduced from such measurements. We report high frequency measurements in which Andreev Reflection affects the distribution statistics of the electronic excitations, resulting in a shift of the classical-to-quantum regime or equilibrium-to-shot noise crossovers. We also demonstrate that the effective charge carried by paired electrons contains more information: its deviation from 2e is related to correlations among pairs. This is exemplified by the measurement of phase dependent noise in an Andreev Interferometer. The use of full counting statistics allows us to understand how the correlations occur, and its application to the case of the Andreev Interferometer exhibits a very good agreement between theory and experiment., Comment: 19 pages, 7 figures, for "Quantum Noise", edited by Yu. V. Nazarov and Ya. M. Blanter (Kluwer)

The circuit theory of mesoscopic transport provides a unified framework to describe spin-dependent or superconductivity-related phenomena. We extend this theory to hybrid systems of normal metals, ferromagnets and superconductors. Our main result is an expression for the current through an arbitrary contact between two general isotropic "nodes", which is suitable to describe the presence of superconducting and ferromagnetic elements in the system, as well as magnetically active interfaces/contacts. In certain cases (weak ferromagnet and magnetic tunnel junction) we derive transparent and simple results for the matrix current., Comment: Improvement of this work and final published version can be found in arXiv:0911.4784 / Phys. Rev. B 80, 184511 (2009)

Superconductor-Ferromagnetic-Superconductor (SFS) Josephson junctions are known to exhibit a transition between $��$ and 0 states. In this note we find the $��-0$ phase diagram of an SFS junction depending on the transparency of an intermediate insulating layer (I). We show that in general, the Josephson critical current is nonzero at the $��-0$ transition temperature. Contributions to the current from the two spin channels nearly compensate each other and the first harmonic of the Josephson current as a function of phase difference is suppressed. However, higher harmonics give a nonzero contribution to the supercurrent., 4 pages, 4 figures

We report on the measurement of multiple Andreev resonances at atomic size point contacts between two superconducting nanostructures of Pb under magnetic fields higher than the bulk critical field, where superconductivity is restricted to a mesoscopic region near the contact. The small number of conduction channels in this type of contacts permits a quantitative comparison with theory through the whole field range. We discuss in detail the physical properties of our structure, in which the normal bulk electrodes induce a proximity effect into the mesoscopic superconducting part., Comment: 4 pages

We investigate the magnetic response of normal-metal--superconductor proximity systems for arbitrary concentrations of impurities and at arbitrary temperatures. Using the quasiclassical theory a general linear-response formula is derived which yields a non-local current-field relation in terms of the zero-field Green's functions. Various regimes between clean-limit and (local) dirty-limit response are investigated by analytical methods and by solving the general formula numerically. In the ballistic regime we find that a finite mean free path reduces the non-locality and leads to a stronger screening than in the clean limit even for a mean free path much larger than the system size. Additionally, the range of the kernel describing the non-locality is strongly temperature-dependent in this case. In the diffusive limit we find a cross-over from local to non-local screening, which restricts the applicability of the dirty-limit theory., 10 Pages (revtex), 6 figures (eps, included), version accepted for publication in Phys. Rev. B

We investigate the electronic structure of twin boundaries in orthorhombically distorted high-T$_c$ materials using the quasiclassical theory of superconductivity. At low temperatures we find a local instability to a time-reversal symmetry breaking state at the twin boundary. This state yields spontaneous currents along the twin boundary that are microscopically explained by the structure of the quasiparticle bound states. We calculate the local density of states and find a splitting in the zero-bias peak once the spontaneous currents set in. This splitting is measurable by STM techniques and is a unique signature of time-reversal breaking states at a twin boundary., Comment: 4 pages, LaTeX, 4 eps-figures