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54 results on '"Schmidt, Joel E."'

1. Detecting Cage Crossing and Filling Clusters of Magnesium and Carbon Atoms in Zeolite SSZ-13 with Atom Probe Tomography

Author

Sub Inorganic Chemistry and Catalysis, Sub ARC Chemical Building Blocks Cons., Faculteit Betawetenschappen, Inorganic Chemistry and Catalysis, Van Vreeswijk, Sophie H., Monai, Matteo, Oord, Ramon, Schmidt, Joel E., Parvulescu, Andrei N., Yarulina, Irina, Karwacki, Lukasz, Poplawsky, Jonathan D., Weckhuysen, Bert M., Sub Inorganic Chemistry and Catalysis, Sub ARC Chemical Building Blocks Cons., Faculteit Betawetenschappen, Inorganic Chemistry and Catalysis, Van Vreeswijk, Sophie H., Monai, Matteo, Oord, Ramon, Schmidt, Joel E., Parvulescu, Andrei N., Yarulina, Irina, Karwacki, Lukasz, Poplawsky, Jonathan D., and Weckhuysen, Bert M.

Published
2022

2. New insights into the NH3-selective catalytic reduction of NO over Cu-ZSM-5 as revealed by operando spectroscopy

Author

Sub Inorganic Chemistry and Catalysis, Sub ARC Chemical Building Blocks Cons., Faculteit Betawetenschappen, Inorganic Chemistry and Catalysis, Ye, Xinwei, Oord, Ramon, Monai, Matteo, Schmidt, Joel E., Chen, Tiehong, Meirer, Florian, Weckhuysen, Bert M., Sub Inorganic Chemistry and Catalysis, Sub ARC Chemical Building Blocks Cons., Faculteit Betawetenschappen, Inorganic Chemistry and Catalysis, Ye, Xinwei, Oord, Ramon, Monai, Matteo, Schmidt, Joel E., Chen, Tiehong, Meirer, Florian, and Weckhuysen, Bert M.

Published
2022

3. Detecting Cage Crossing and Filling Clusters of Magnesium and Carbon Atoms in Zeolite SSZ-13 with Atom Probe Tomography

Author

Sub Inorganic Chemistry and Catalysis, Sub ARC Chemical Building Blocks Cons., Faculteit Betawetenschappen, Inorganic Chemistry and Catalysis, Van Vreeswijk, Sophie H., Monai, Matteo, Oord, Ramon, Schmidt, Joel E., Parvulescu, Andrei N., Yarulina, Irina, Karwacki, Lukasz, Poplawsky, Jonathan D., Weckhuysen, Bert M., Sub Inorganic Chemistry and Catalysis, Sub ARC Chemical Building Blocks Cons., Faculteit Betawetenschappen, Inorganic Chemistry and Catalysis, Van Vreeswijk, Sophie H., Monai, Matteo, Oord, Ramon, Schmidt, Joel E., Parvulescu, Andrei N., Yarulina, Irina, Karwacki, Lukasz, Poplawsky, Jonathan D., and Weckhuysen, Bert M.

Published
2022

4. New insights into the NH3-selective catalytic reduction of NO over Cu-ZSM-5 as revealed by operando spectroscopy

Author

Sub Inorganic Chemistry and Catalysis, Sub ARC Chemical Building Blocks Cons., Faculteit Betawetenschappen, Inorganic Chemistry and Catalysis, Ye, Xinwei, Oord, Ramon, Monai, Matteo, Schmidt, Joel E., Chen, Tiehong, Meirer, Florian, Weckhuysen, Bert M., Sub Inorganic Chemistry and Catalysis, Sub ARC Chemical Building Blocks Cons., Faculteit Betawetenschappen, Inorganic Chemistry and Catalysis, Ye, Xinwei, Oord, Ramon, Monai, Matteo, Schmidt, Joel E., Chen, Tiehong, Meirer, Florian, and Weckhuysen, Bert M.

Published
2022

5. Probing the Location and Speciation of Elements in Zeolites with Correlated Atom Probe Tomography and Scanning Transmission X-Ray Microscopy.

Author

Schmidt, Joel E, Schmidt, Joel E, Ye, Xinwei, van Ravenhorst, Ilse K, Oord, Ramon, Shapiro, David A, Yu, Young-Sang, Bare, Simon R, Meirer, Florian, Poplawsky, Jonathan D, Weckhuysen, Bert M, Schmidt, Joel E, Schmidt, Joel E, Ye, Xinwei, van Ravenhorst, Ilse K, Oord, Ramon, Shapiro, David A, Yu, Young-Sang, Bare, Simon R, Meirer, Florian, Poplawsky, Jonathan D, and Weckhuysen, Bert M

Abstract

Characterizing materials at nanoscale resolution to provide new insights into structure property performance relationships continues to be a challenging research target due to the inherently low signal from small sample volumes, and is even more difficult for nonconductive materials, such as zeolites. Herein, we present the characterization of a single Cu-exchanged zeolite crystal, namely Cu-SSZ-13, used for NOX reduction in automotive emissions, that was subject to a simulated 135,000-mile aging. By correlating Atom Probe Tomography (APT), a single atom microscopy method, and Scanning Transmission X-ray Microscopy (STXM), which produces high spatial resolution X-ray Absorption Near Edge Spectroscopy (XANES) maps, we show that a spatially non-uniform proportion of the Al was removed from the zeolite framework. The techniques reveal that this degradation is heterogeneous at length scales from micrometers to tens of nanometers, providing complementary insight into the long-term deactivation of this catalyst system.

Published
2019

6. Probing the Location and Speciation of Elements in Zeolites with Correlated Atom Probe Tomography and Scanning Transmission X-Ray Microscopy.

Author

Schmidt, Joel E, Schmidt, Joel E, Ye, Xinwei, van Ravenhorst, Ilse K, Oord, Ramon, Shapiro, David A, Yu, Young-Sang, Bare, Simon R, Meirer, Florian, Poplawsky, Jonathan D, Weckhuysen, Bert M, Schmidt, Joel E, Schmidt, Joel E, Ye, Xinwei, van Ravenhorst, Ilse K, Oord, Ramon, Shapiro, David A, Yu, Young-Sang, Bare, Simon R, Meirer, Florian, Poplawsky, Jonathan D, and Weckhuysen, Bert M

Abstract

Characterizing materials at nanoscale resolution to provide new insights into structure property performance relationships continues to be a challenging research target due to the inherently low signal from small sample volumes, and is even more difficult for nonconductive materials, such as zeolites. Herein, we present the characterization of a single Cu-exchanged zeolite crystal, namely Cu-SSZ-13, used for NOX reduction in automotive emissions, that was subject to a simulated 135,000-mile aging. By correlating Atom Probe Tomography (APT), a single atom microscopy method, and Scanning Transmission X-ray Microscopy (STXM), which produces high spatial resolution X-ray Absorption Near Edge Spectroscopy (XANES) maps, we show that a spatially non-uniform proportion of the Al was removed from the zeolite framework. The techniques reveal that this degradation is heterogeneous at length scales from micrometers to tens of nanometers, providing complementary insight into the long-term deactivation of this catalyst system.

Published
2019

7. Deactivation of Cu-Exchanged Automotive-Emission NH3 -SCR Catalysts Elucidated with Nanoscale Resolution Using Scanning Transmission X-ray Microscopy

Author

Sub Inorganic Chemistry and Catalysis, Sub ARC Chemical Building Blocks Cons., Inorganic Chemistry and Catalysis, Ye, Xinwei, Schmidt, Joel E, Wang, Ru-Pan, van Ravenhorst, Ilse K, Oord, Ramon, Chen, Tiehong, de Groot, Frank, Meirer, Florian, Weckhuysen, Bert M, Sub Inorganic Chemistry and Catalysis, Sub ARC Chemical Building Blocks Cons., Inorganic Chemistry and Catalysis, Ye, Xinwei, Schmidt, Joel E, Wang, Ru-Pan, van Ravenhorst, Ilse K, Oord, Ramon, Chen, Tiehong, de Groot, Frank, Meirer, Florian, and Weckhuysen, Bert M

Published
2020

8. Disentangling Reaction Processes of Zeolites within Single-Oriented Channels

Author

Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Fu, Donglong, van der Heijden, Onno, Stanciakova, Katarina, Schmidt, Joel E, Weckhuysen, Bert M, Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Fu, Donglong, van der Heijden, Onno, Stanciakova, Katarina, Schmidt, Joel E, and Weckhuysen, Bert M

Published
2020

9. Deactivation of Cu-Exchanged Automotive-Emission NH3 -SCR Catalysts Elucidated with Nanoscale Resolution Using Scanning Transmission X-ray Microscopy

Author

Sub Inorganic Chemistry and Catalysis, Sub ARC Chemical Building Blocks Cons., Inorganic Chemistry and Catalysis, Ye, Xinwei, Schmidt, Joel E, Wang, Ru-Pan, van Ravenhorst, Ilse K, Oord, Ramon, Chen, Tiehong, de Groot, Frank, Meirer, Florian, Weckhuysen, Bert M, Sub Inorganic Chemistry and Catalysis, Sub ARC Chemical Building Blocks Cons., Inorganic Chemistry and Catalysis, Ye, Xinwei, Schmidt, Joel E, Wang, Ru-Pan, van Ravenhorst, Ilse K, Oord, Ramon, Chen, Tiehong, de Groot, Frank, Meirer, Florian, and Weckhuysen, Bert M

Published
2020

10. Disentangling Reaction Processes of Zeolites within Single-Oriented Channels

Author

Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Fu, Donglong, van der Heijden, Onno, Stanciakova, Katarina, Schmidt, Joel E, Weckhuysen, Bert M, Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Fu, Donglong, van der Heijden, Onno, Stanciakova, Katarina, Schmidt, Joel E, and Weckhuysen, Bert M

Published
2020

11. Disentangling Reaction Processes of Zeolites within Single-Oriented Channels

Author

Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Fu, Donglong, van der Heijden, Onno, Stanciakova, Katarina, Schmidt, Joel E, Weckhuysen, Bert M, Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Fu, Donglong, van der Heijden, Onno, Stanciakova, Katarina, Schmidt, Joel E, and Weckhuysen, Bert M

Published
2020

12. Deactivation of Cu-Exchanged Automotive-Emission NH3 -SCR Catalysts Elucidated with Nanoscale Resolution Using Scanning Transmission X-ray Microscopy

Author

Sub Inorganic Chemistry and Catalysis, Sub ARC Chemical Building Blocks Cons., Inorganic Chemistry and Catalysis, Ye, Xinwei, Schmidt, Joel E, Wang, Ru-Pan, van Ravenhorst, Ilse K, Oord, Ramon, Chen, Tiehong, de Groot, Frank, Meirer, Florian, Weckhuysen, Bert M, Sub Inorganic Chemistry and Catalysis, Sub ARC Chemical Building Blocks Cons., Inorganic Chemistry and Catalysis, Ye, Xinwei, Schmidt, Joel E, Wang, Ru-Pan, van Ravenhorst, Ilse K, Oord, Ramon, Chen, Tiehong, de Groot, Frank, Meirer, Florian, and Weckhuysen, Bert M

Published
2020

13. SSZ-27 : A Small-Pore Zeolite with Large Heart-Shaped Cavities Determined by using Multi-crystal Electron Diffraction

Author

Smeets, Stef, Zones, Stacey I., Xie, Dan, Palatinus, Lukas, Pascual, Jesus, Hwang, Son-Jong, Schmidt, Joel E., McCusker, Lynne B., Smeets, Stef, Zones, Stacey I., Xie, Dan, Palatinus, Lukas, Pascual, Jesus, Hwang, Son-Jong, Schmidt, Joel E., and McCusker, Lynne B.

Abstract

The high-silica zeolite SSZ-27 was synthesized using one of the isomers of the organic structure-directing agent that is known to produce the large-pore zeolite SSZ-26 (CON). The structure of the as-synthesized form was solved using multi-crystal electron diffraction data. Data were collected on eighteen crystals, and to obtain a high-quality and complete data set for structure refinement, hierarchical cluster analysis was employed to select the data sets most suitable for merging. The framework structure of SSZ-27 can be described as a combination of two types of cavities, one of which is shaped like a heart. The cavities are connected through shared 8-ring windows to create straight channels that are linked together in pairs to form a one-dimensional channel system. Once the framework structure was known, molecular modelling was used to find the best fitting isomer, and this, in turn, was isolated to improve the synthesis conditions for SSZ-27.

Published
2019
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14. SSZ-27: A Small-Pore Zeolite with Large Heart-Shaped Cavities Determined by using Multi-crystal Electron Diffraction

Author

Smeets, S. (author), Zones, Stacey I. (author), Xie, Dan (author), Palatinus, Lukáš (author), Pascual, Jesus (author), Hwang, Son Jong (author), Schmidt, Joel E. (author), McCusker, Lynne B. (author), Smeets, S. (author), Zones, Stacey I. (author), Xie, Dan (author), Palatinus, Lukáš (author), Pascual, Jesus (author), Hwang, Son Jong (author), Schmidt, Joel E. (author), and McCusker, Lynne B. (author)

Abstract

The high-silica zeolite SSZ-27 was synthesized using one of the isomers of the organic structure-directing agent that is known to produce the large-pore zeolite SSZ-26 (CON). The structure of the as-synthesized form was solved using multi-crystal electron diffraction data. Data were collected on eighteen crystals, and to obtain a high-quality and complete data set for structure refinement, hierarchical cluster analysis was employed to select the data sets most suitable for merging. The framework structure of SSZ-27 can be described as a combination of two types of cavities, one of which is shaped like a heart. The cavities are connected through shared 8-ring windows to create straight channels that are linked together in pairs to form a one-dimensional channel system. Once the framework structure was known, molecular modelling was used to find the best fitting isomer, and this, in turn, was isolated to improve the synthesis conditions for SSZ-27., BN/Arjen Jakobi Lab

Published
2019
Full Text
View/download PDF

15. Probing the Location and Speciation of Elements in Zeolites with Correlated Atom Probe Tomography and Scanning Transmission X-Ray Microscopy

Author

Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Schmidt, Joel E., Ye, Xinwei, van Ravenhorst, Ilse K., Oord, Ramon, Shapiro, David A., Yu, Young Sang, Bare, Simon R., Meirer, Florian, Poplawsky, Jonathan D., Weckhuysen, Bert M., Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Schmidt, Joel E., Ye, Xinwei, van Ravenhorst, Ilse K., Oord, Ramon, Shapiro, David A., Yu, Young Sang, Bare, Simon R., Meirer, Florian, Poplawsky, Jonathan D., and Weckhuysen, Bert M.

Published
2019

16. Probing the Location and Speciation of Elements in Zeolites with Correlated Atom Probe Tomography and Scanning Transmission X-Ray Microscopy

Author

Inorganic Chemistry and Catalysis, Sub Inorganic Chemistry and Catalysis, Schmidt, Joel E., Ye, Xinwei, van Ravenhorst, Ilse K., Oord, Ramon, Shapiro, David A., Yu, Young Sang, Bare, Simon R., Meirer, Florian, Poplawsky, Jonathan D., Weckhuysen, Bert M., Inorganic Chemistry and Catalysis, Sub Inorganic Chemistry and Catalysis, Schmidt, Joel E., Ye, Xinwei, van Ravenhorst, Ilse K., Oord, Ramon, Shapiro, David A., Yu, Young Sang, Bare, Simon R., Meirer, Florian, Poplawsky, Jonathan D., and Weckhuysen, Bert M.

Published
2019

17. Probing the Location and Speciation of Elements in Zeolites with Correlated Atom Probe Tomography and Scanning Transmission X-Ray Microscopy

Author

Inorganic Chemistry and Catalysis, Sub Inorganic Chemistry and Catalysis, Schmidt, Joel E., Ye, Xinwei, van Ravenhorst, Ilse K., Oord, Ramon, Shapiro, David A., Yu, Young Sang, Bare, Simon R., Meirer, Florian, Poplawsky, Jonathan D., Weckhuysen, Bert M., Inorganic Chemistry and Catalysis, Sub Inorganic Chemistry and Catalysis, Schmidt, Joel E., Ye, Xinwei, van Ravenhorst, Ilse K., Oord, Ramon, Shapiro, David A., Yu, Young Sang, Bare, Simon R., Meirer, Florian, Poplawsky, Jonathan D., and Weckhuysen, Bert M.

Published
2019

18. SSZ-27: A Small-Pore Zeolite with Large Heart-Shaped Cavities Determined by using Multi-crystal Electron Diffraction

Author

Smeets, S. (author), Zones, Stacey I. (author), Xie, Dan (author), Palatinus, Lukáš (author), Pascual, Jesus (author), Hwang, Son Jong (author), Schmidt, Joel E. (author), McCusker, Lynne B. (author), Smeets, S. (author), Zones, Stacey I. (author), Xie, Dan (author), Palatinus, Lukáš (author), Pascual, Jesus (author), Hwang, Son Jong (author), Schmidt, Joel E. (author), and McCusker, Lynne B. (author)

Abstract

The high-silica zeolite SSZ-27 was synthesized using one of the isomers of the organic structure-directing agent that is known to produce the large-pore zeolite SSZ-26 (CON). The structure of the as-synthesized form was solved using multi-crystal electron diffraction data. Data were collected on eighteen crystals, and to obtain a high-quality and complete data set for structure refinement, hierarchical cluster analysis was employed to select the data sets most suitable for merging. The framework structure of SSZ-27 can be described as a combination of two types of cavities, one of which is shaped like a heart. The cavities are connected through shared 8-ring windows to create straight channels that are linked together in pairs to form a one-dimensional channel system. Once the framework structure was known, molecular modelling was used to find the best fitting isomer, and this, in turn, was isolated to improve the synthesis conditions for SSZ-27., BN/Arjen Jakobi Lab

Published
2019
Full Text
View/download PDF

19. Isolating Clusters of Light Elements in Molecular Sieves with Atom Probe Tomography

Author

Sub Inorganic Chemistry and Catalysis, Sub NMR Spectroscopy, Structural geology and EM, NMR Spectroscopy, Inorganic Chemistry and Catalysis, Structural geology & tectonics, Schmidt, Joel E, Peng, Linqing, Paioni, Alessandra Lucini, Ehren, Helena Leona, Guo, Wei, Mazumder, Baishakhi, Matthijs de Winter, D A, Attila, Özgün, Fu, Donglong, Chowdhury, Abhishek Dutta, Houben, Klaartje, Baldus, Marc, Poplawsky, Jonathan D, Weckhuysen, Bert M, Sub Inorganic Chemistry and Catalysis, Sub NMR Spectroscopy, Structural geology and EM, NMR Spectroscopy, Inorganic Chemistry and Catalysis, Structural geology & tectonics, Schmidt, Joel E, Peng, Linqing, Paioni, Alessandra Lucini, Ehren, Helena Leona, Guo, Wei, Mazumder, Baishakhi, Matthijs de Winter, D A, Attila, Özgün, Fu, Donglong, Chowdhury, Abhishek Dutta, Houben, Klaartje, Baldus, Marc, Poplawsky, Jonathan D, and Weckhuysen, Bert M

Published
2018

21. Diagnosing the Internal Architecture of Zeolite Ferrierite

Author

Inorganic Chemistry and Catalysis, Sub Inorganic Chemistry and Catalysis, Sub Crystal and Structural Chemistry, Sub Condensed Matter and Interfaces, Crystal and Structural Chemistry, Condensed Matter and Interfaces, Schmidt, Joel E., Hendriks, Frank C., Lutz, Martin, Post, L. Christiaan, Fu, Donglong, Weckhuysen, Bert, Inorganic Chemistry and Catalysis, Sub Inorganic Chemistry and Catalysis, Sub Crystal and Structural Chemistry, Sub Condensed Matter and Interfaces, Crystal and Structural Chemistry, Condensed Matter and Interfaces, Schmidt, Joel E., Hendriks, Frank C., Lutz, Martin, Post, L. Christiaan, Fu, Donglong, and Weckhuysen, Bert

Published
2018

22. Deconvoluting the Competing Effects of Zeolite Framework Topology and Diffusion Path Length on Methanol to Hydrocarbons Reaction

Author

Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Shen, Yufeng, Le, Thuy T., Fu, Donglong, Schmidt, Joel E., Filez, Matthias, Weckhuysen, Bert M., Rimer, Jeffrey D., Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Shen, Yufeng, Le, Thuy T., Fu, Donglong, Schmidt, Joel E., Filez, Matthias, Weckhuysen, Bert M., and Rimer, Jeffrey D.

Published
2018

23. Uniformly Oriented Zeolite ZSM-5 Membranes with Tunable Wettability on a Porous Ceramic

Author

Inorganic Chemistry and Catalysis, Sub Inorganic Chemistry and Catalysis, Sub Organic Chemistry and Catalysis, Organic Chemistry and Catalysis, Fu, Donglong, Schmidt, Joel E., Pletcher, Paul, Karakiliç, Pelin, Ye, Xinwei, Vis, Carolien M., Bruijnincx, Pieter C.A., Filez, Matthias, Mandemaker, Laurens D.B., Winnubst, Louis, Weckhuysen, Bert M., Inorganic Chemistry and Catalysis, Sub Inorganic Chemistry and Catalysis, Sub Organic Chemistry and Catalysis, Organic Chemistry and Catalysis, Fu, Donglong, Schmidt, Joel E., Pletcher, Paul, Karakiliç, Pelin, Ye, Xinwei, Vis, Carolien M., Bruijnincx, Pieter C.A., Filez, Matthias, Mandemaker, Laurens D.B., Winnubst, Louis, and Weckhuysen, Bert M.

Published
2018

24. Nanoscale Chemical Imaging of Zeolites Using Atom Probe Tomography

Author

Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Schmidt, Joel E., Peng, Linqing, Poplawsky, Jonathan D., Weckhuysen, Bert M., Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Schmidt, Joel E., Peng, Linqing, Poplawsky, Jonathan D., and Weckhuysen, Bert M.

Published
2018

25. Deconvoluting the Competing Effects of Zeolite Framework Topology and Diffusion Path Length on Methanol to Hydrocarbons Reaction

Author

Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Shen, Yufeng, Le, Thuy T., Fu, Donglong, Schmidt, Joel E., Filez, Matthias, Weckhuysen, Bert M., Rimer, Jeffrey D., Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Shen, Yufeng, Le, Thuy T., Fu, Donglong, Schmidt, Joel E., Filez, Matthias, Weckhuysen, Bert M., and Rimer, Jeffrey D.

Published
2018

26. Uniformly Oriented Zeolite ZSM-5 Membranes with Tunable Wettability on a Porous Ceramic

Author

Inorganic Chemistry and Catalysis, Sub Inorganic Chemistry and Catalysis, Sub Organic Chemistry and Catalysis, Organic Chemistry and Catalysis, Fu, Donglong, Schmidt, Joel E., Pletcher, Paul, Karakiliç, Pelin, Ye, Xinwei, Vis, Carolien M., Bruijnincx, Pieter C.A., Filez, Matthias, Mandemaker, Laurens D.B., Winnubst, Louis, Weckhuysen, Bert M., Inorganic Chemistry and Catalysis, Sub Inorganic Chemistry and Catalysis, Sub Organic Chemistry and Catalysis, Organic Chemistry and Catalysis, Fu, Donglong, Schmidt, Joel E., Pletcher, Paul, Karakiliç, Pelin, Ye, Xinwei, Vis, Carolien M., Bruijnincx, Pieter C.A., Filez, Matthias, Mandemaker, Laurens D.B., Winnubst, Louis, and Weckhuysen, Bert M.

Published
2018

27. Nanoscale Chemical Imaging of Zeolites Using Atom Probe Tomography

Author

Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Schmidt, Joel E., Peng, Linqing, Poplawsky, Jonathan D., Weckhuysen, Bert M., Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Schmidt, Joel E., Peng, Linqing, Poplawsky, Jonathan D., and Weckhuysen, Bert M.

Published
2018

28. Isolating Clusters of Light Elements in Molecular Sieves with Atom Probe Tomography

Author

Sub Inorganic Chemistry and Catalysis, Sub NMR Spectroscopy, Structural geology and EM, NMR Spectroscopy, Inorganic Chemistry and Catalysis, Structural geology & tectonics, Schmidt, Joel E, Peng, Linqing, Paioni, Alessandra Lucini, Ehren, Helena Leona, Guo, Wei, Mazumder, Baishakhi, Matthijs de Winter, D A, Attila, Özgün, Fu, Donglong, Chowdhury, Abhishek Dutta, Houben, Klaartje, Baldus, Marc, Poplawsky, Jonathan D, Weckhuysen, Bert M, Sub Inorganic Chemistry and Catalysis, Sub NMR Spectroscopy, Structural geology and EM, NMR Spectroscopy, Inorganic Chemistry and Catalysis, Structural geology & tectonics, Schmidt, Joel E, Peng, Linqing, Paioni, Alessandra Lucini, Ehren, Helena Leona, Guo, Wei, Mazumder, Baishakhi, Matthijs de Winter, D A, Attila, Özgün, Fu, Donglong, Chowdhury, Abhishek Dutta, Houben, Klaartje, Baldus, Marc, Poplawsky, Jonathan D, and Weckhuysen, Bert M

Published
2018

29. Diagnosing the Internal Architecture of Zeolite Ferrierite

Author

Inorganic Chemistry and Catalysis, Sub Inorganic Chemistry and Catalysis, Sub Crystal and Structural Chemistry, Sub Condensed Matter and Interfaces, Crystal and Structural Chemistry, Condensed Matter and Interfaces, Schmidt, Joel E., Hendriks, Frank C., Lutz, Martin, Post, L. Christiaan, Fu, Donglong, Weckhuysen, Bert, Inorganic Chemistry and Catalysis, Sub Inorganic Chemistry and Catalysis, Sub Crystal and Structural Chemistry, Sub Condensed Matter and Interfaces, Crystal and Structural Chemistry, Condensed Matter and Interfaces, Schmidt, Joel E., Hendriks, Frank C., Lutz, Martin, Post, L. Christiaan, Fu, Donglong, and Weckhuysen, Bert

Published
2018

31. Deconvoluting the Competing Effects of Zeolite Framework Topology and Diffusion Path Length on Methanol to Hydrocarbons Reaction

Author

Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Shen, Yufeng, Le, Thuy T., Fu, Donglong, Schmidt, Joel E., Filez, Matthias, Weckhuysen, Bert M., Rimer, Jeffrey D., Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Shen, Yufeng, Le, Thuy T., Fu, Donglong, Schmidt, Joel E., Filez, Matthias, Weckhuysen, Bert M., and Rimer, Jeffrey D.

Published
2018

32. Uniformly Oriented Zeolite ZSM-5 Membranes with Tunable Wettability on a Porous Ceramic

Author

Inorganic Chemistry and Catalysis, Sub Inorganic Chemistry and Catalysis, Sub Organic Chemistry and Catalysis, Organic Chemistry and Catalysis, Fu, Donglong, Schmidt, Joel E., Pletcher, Paul, Karakiliç, Pelin, Ye, Xinwei, Vis, Carolien M., Bruijnincx, Pieter C.A., Filez, Matthias, Mandemaker, Laurens D.B., Winnubst, Louis, Weckhuysen, Bert M., Inorganic Chemistry and Catalysis, Sub Inorganic Chemistry and Catalysis, Sub Organic Chemistry and Catalysis, Organic Chemistry and Catalysis, Fu, Donglong, Schmidt, Joel E., Pletcher, Paul, Karakiliç, Pelin, Ye, Xinwei, Vis, Carolien M., Bruijnincx, Pieter C.A., Filez, Matthias, Mandemaker, Laurens D.B., Winnubst, Louis, and Weckhuysen, Bert M.

Published
2018

33. Nanoscale Chemical Imaging of Zeolites Using Atom Probe Tomography

Author

Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Schmidt, Joel E., Peng, Linqing, Poplawsky, Jonathan D., Weckhuysen, Bert M., Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Schmidt, Joel E., Peng, Linqing, Poplawsky, Jonathan D., and Weckhuysen, Bert M.

Published
2018

34. Isolating Clusters of Light Elements in Molecular Sieves with Atom Probe Tomography

Author

Sub Inorganic Chemistry and Catalysis, Sub NMR Spectroscopy, Structural geology and EM, NMR Spectroscopy, Inorganic Chemistry and Catalysis, Structural geology & tectonics, Schmidt, Joel E, Peng, Linqing, Paioni, Alessandra Lucini, Ehren, Helena Leona, Guo, Wei, Mazumder, Baishakhi, Matthijs de Winter, D A, Attila, Özgün, Fu, Donglong, Chowdhury, Abhishek Dutta, Houben, Klaartje, Baldus, Marc, Poplawsky, Jonathan D, Weckhuysen, Bert M, Sub Inorganic Chemistry and Catalysis, Sub NMR Spectroscopy, Structural geology and EM, NMR Spectroscopy, Inorganic Chemistry and Catalysis, Structural geology & tectonics, Schmidt, Joel E, Peng, Linqing, Paioni, Alessandra Lucini, Ehren, Helena Leona, Guo, Wei, Mazumder, Baishakhi, Matthijs de Winter, D A, Attila, Özgün, Fu, Donglong, Chowdhury, Abhishek Dutta, Houben, Klaartje, Baldus, Marc, Poplawsky, Jonathan D, and Weckhuysen, Bert M

Published
2018

36. Diagnosing the Internal Architecture of Zeolite Ferrierite

Author

Inorganic Chemistry and Catalysis, Sub Inorganic Chemistry and Catalysis, Sub Crystal and Structural Chemistry, Sub Condensed Matter and Interfaces, Crystal and Structural Chemistry, Condensed Matter and Interfaces, Schmidt, Joel E., Hendriks, Frank C., Lutz, Martin, Post, L. Christiaan, Fu, Donglong, Weckhuysen, Bert, Inorganic Chemistry and Catalysis, Sub Inorganic Chemistry and Catalysis, Sub Crystal and Structural Chemistry, Sub Condensed Matter and Interfaces, Crystal and Structural Chemistry, Condensed Matter and Interfaces, Schmidt, Joel E., Hendriks, Frank C., Lutz, Martin, Post, L. Christiaan, Fu, Donglong, and Weckhuysen, Bert

Published
2018

37. Enantiomerically enriched, polycrystalline molecular sieves

Author

Brand, Stephen K., Schmidt, Joel E., Deem, Michael W., Daeyaert, Frits, Ma, Yanhang, Terasaki, Osamu, Orazov, Marat, Davis, Mark E., Brand, Stephen K., Schmidt, Joel E., Deem, Michael W., Daeyaert, Frits, Ma, Yanhang, Terasaki, Osamu, Orazov, Marat, and Davis, Mark E.

Abstract

Zeolite and zeolite-like molecular sieves are being used in a large number of applications such as adsorption and catalysis. Achievement of the long-standing goal of creating a chiral, polycrystalline molecular sieve with bulk enantioenrichment would enable these materials to perform enantioselective functions. Here, we report the synthesis of enantiomerically enriched samples of a molecular sieve. Enantiopure organic structure directing agents are designed with the assistance of computational methods and used to synthesize enantioenriched, polycrystalline molecular sieve samples of either enantiomer. Computational results correctly predicted which enantiomer is obtained, and enantiomeric enrichment is proven by high-resolution transmission electron microscopy. The enantioenriched and racemic samples of the molecular sieves are tested as adsorbents and heterogeneous catalysts. The enantioenriched molecular sieves show enantioselectivity for the ring opening reaction of epoxides and enantioselective adsorption of 2-butanol (the R enantiomer of the molecular sieve shows opposite and approximately equal enantioselectivity compared with the S enantiomer of the molecular sieve, whereas the racemic sample of the molecular sieve shows no enantioselectivity).

Published
2017
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39. Probing Zeolite Crystal Architecture and Structural Imperfections using Differently Sized Fluorescent Organic Probe Molecules

Author

Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Hendriks, Frank C., Schmidt, Joel E., Rombouts, Jeroen A, Lammertsma, Koop, Bruijnincx, Pieter C. A., Weckhuysen, Bert M., Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Hendriks, Frank C., Schmidt, Joel E., Rombouts, Jeroen A, Lammertsma, Koop, Bruijnincx, Pieter C. A., and Weckhuysen, Bert M.

Published
2017

40. Highly Oriented Growth of Catalytically Active Zeolite ZSM-5 Films with a Broad Range of Si/Al Ratios

Author

Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Fu, Donglong, Schmidt, Joel E., Ristanovic, Zoran, Chowdhury, Abhishek Dutta, Meirer, Florian, Weckhuysen, Bert M., Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Fu, Donglong, Schmidt, Joel E., Ristanovic, Zoran, Chowdhury, Abhishek Dutta, Meirer, Florian, and Weckhuysen, Bert M.

Published
2017

41. Highly Oriented Growth of Catalytically Active Zeolite ZSM-5 Films with a Broad Range of Si/Al Ratios

Author

Inorganic Chemistry and Catalysis, Sub Inorganic Chemistry and Catalysis, Fu, Donglong, Schmidt, Joel E., Ristanovic, Zoran, Chowdhury, Abhishek Dutta, Meirer, Florian, Weckhuysen, Bert M., Inorganic Chemistry and Catalysis, Sub Inorganic Chemistry and Catalysis, Fu, Donglong, Schmidt, Joel E., Ristanovic, Zoran, Chowdhury, Abhishek Dutta, Meirer, Florian, and Weckhuysen, Bert M.

Published
2017

42. Probing Zeolite Crystal Architecture and Structural Imperfections using Differently Sized Fluorescent Organic Probe Molecules

Author

Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Hendriks, Frank C., Schmidt, Joel E., Rombouts, Jeroen A, Lammertsma, Koop, Bruijnincx, Pieter C. A., Weckhuysen, Bert M., Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Hendriks, Frank C., Schmidt, Joel E., Rombouts, Jeroen A, Lammertsma, Koop, Bruijnincx, Pieter C. A., and Weckhuysen, Bert M.

Published
2017

44. Probing Zeolite Crystal Architecture and Structural Imperfections using Differently Sized Fluorescent Organic Probe Molecules

Author

Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Hendriks, Frank C., Schmidt, Joel E., Rombouts, Jeroen A, Lammertsma, Koop, Bruijnincx, Pieter C. A., Weckhuysen, Bert M., Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Hendriks, Frank C., Schmidt, Joel E., Rombouts, Jeroen A, Lammertsma, Koop, Bruijnincx, Pieter C. A., and Weckhuysen, Bert M.

Published
2017

46. Highly Oriented Growth of Catalytically Active Zeolite ZSM-5 Films with a Broad Range of Si/Al Ratios

Author

Inorganic Chemistry and Catalysis, Sub Inorganic Chemistry and Catalysis, Fu, Donglong, Schmidt, Joel E., Ristanovic, Zoran, Chowdhury, Abhishek Dutta, Meirer, Florian, Weckhuysen, Bert M., Inorganic Chemistry and Catalysis, Sub Inorganic Chemistry and Catalysis, Fu, Donglong, Schmidt, Joel E., Ristanovic, Zoran, Chowdhury, Abhishek Dutta, Meirer, Florian, and Weckhuysen, Bert M.

Published
2017

47. Template-Framework Interactions in Tetraethylammonium-Directed Zeolite Synthesis

Author

Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Schmidt, Joel E., Fu, Donglong, Deem, Michael W., Weckhuysen, Bert M., Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Schmidt, Joel E., Fu, Donglong, Deem, Michael W., and Weckhuysen, Bert M.

Published
2016

48. Coke Formation in a Zeolite Crystal During the Methanol-to- Hydrocarbons Reaction as Studied with Atom Probe Tomography

Author

Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Schmidt, Joel E, Poplawsky, Jonathan D, Mazumder, Baishakhi, Attila, Özgün, Fu, Donglong, Winter, D A Matthijs De, Meirer, Florian, Bare, Simon R, Weckhuysen, Bert M, Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Schmidt, Joel E, Poplawsky, Jonathan D, Mazumder, Baishakhi, Attila, Özgün, Fu, Donglong, Winter, D A Matthijs De, Meirer, Florian, Bare, Simon R, and Weckhuysen, Bert M

Published
2016

49. Template-Framework Interactions in Tetraethylammonium-Directed Zeolite Synthesis

Author

Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Schmidt, Joel E., Fu, Donglong, Deem, Michael W., Weckhuysen, Bert M., Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Schmidt, Joel E., Fu, Donglong, Deem, Michael W., and Weckhuysen, Bert M.

Published
2016

50. Coke Formation in a Zeolite Crystal During the Methanol-to- Hydrocarbons Reaction as Studied with Atom Probe Tomography

Author

Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Schmidt, Joel E, Poplawsky, Jonathan D, Mazumder, Baishakhi, Attila, Özgün, Fu, Donglong, Winter, D A Matthijs De, Meirer, Florian, Bare, Simon R, Weckhuysen, Bert M, Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Schmidt, Joel E, Poplawsky, Jonathan D, Mazumder, Baishakhi, Attila, Özgün, Fu, Donglong, Winter, D A Matthijs De, Meirer, Florian, Bare, Simon R, and Weckhuysen, Bert M

Published
2016

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