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Problematic smartphone use negatively affects physical and mental health. Despite the wide range of prior research, existing persuasive techniques are not flexible enough to provide dynamic persuasion content based on users' physical contexts and mental states. We first conducted a Wizard-of-Oz study (N=12) and an interview study (N=10) to summarize the mental states behind problematic smartphone use: boredom, stress, and inertia. This informs our design of four persuasion strategies: understanding, comforting, evoking, and scaffolding habits. We leveraged large language models (LLMs) to enable the automatic and dynamic generation of effective persuasion content. We developed MindShift, a novel LLM-powered problematic smartphone use intervention technique. MindShift takes users' in-the-moment app usage behaviors, physical contexts, mental states, goals \& habits as input, and generates personalized and dynamic persuasive content with appropriate persuasion strategies. We conducted a 5-week field experiment (N=25) to compare MindShift with its simplified version (remove mental states) and baseline techniques (fixed reminder). The results show that MindShift improves intervention acceptance rates by 4.7-22.5% and reduces smartphone usage duration by 7.4-9.8%. Moreover, users have a significant drop in smartphone addiction scale scores and a rise in self-efficacy scale scores. Our study sheds light on the potential of leveraging LLMs for context-aware persuasion in other behavior change domains., Comment: Published at ACM CHI'24

Wet scavenging is an efficient pathway for the removal of particulate matter (PM) from the atmosphere. High levels of PM have been a major cause of air pollution in Beijing but have decreased sharply under the Air Pollution Prevention and Control Action Plan launched in 2013. In this study, four years of observations of wet deposition have been conducted using a sequential sampling technique to investigate the detailed variation in chemical components through each rainfall event. We find that the major ions, SO42−, Ca2+, NO3− and NH4+, show significant decreases over the 2013–2017 period (decreasing by 39 %, 35 %, 12 % and 25 %, respectively), revealing the impacts of the Action Plan. An improved sequential sampling method is developed and implemented to estimate the contribution of below-cloud and in-cloud wet deposition over the four-year period. Overall, below-cloud scavenging accounts for between half and two thirds of wet deposition of the four major ions, with the highest contribution for NH4+ at 65 % and lowest for SO42- at 50 %. The contribution of below-cloud scavenging for Ca2+, SO42- and NH4+ decreases from above 50 % in 2014 to below 40 % in 2017. This suggests that the Action Plan has mitigated PM pollution in the surface layer and hence decreased scavenging due to the washout process. In contrast, we find little change in the annual volume weighted average concentration for NO3- where the contribution from below-cloud scavenging remains at ~44 % over the period 2015–2017. While highlighting the importance of different wet scavenging processes, this paper presents a unique new perspective on the effects of the Action Plan and clearly identifies oxidized nitrogen species as a major target for future air pollution controls.

Black carbon (BC) forms an important component of particulate matter globally, due to its impact on climate, the environment and human health. Identifying and quantifying its emission sources are critical for effective policymaking and achieving the desired reduction in air pollution. In this study, we present the first direct measurements of urban BC fluxes using eddy covariance. The measurements were made over Beijing within the UK-China Air Pollution and Human Health (APHH) winter 2016 and summer 2017 campaigns. In both seasons, the mean measured BC mass (winter: 5.49 ng m−2 s−1, summer: 6.10 ng m−2 s−1) and number fluxes (winter: 261.25 particles cm−2 s−1, summer: 334.37 particles cm−2 s−1) were similar. Traffic was determined to be the dominant source of the BC fluxes measured during both seasons. The total BC emissions within the 2013 Multi-resolution Emission Inventory for China (MEIC) are on average too high compared to measured fluxes by a factor of 58.8 (winter) and 47.2 (summer). Only a comparison with the MEIC transport sector shows that emissions are also larger (factor of 37.5 in winter and 37.7 in summer) than the measured flux. Emission ratios of BC ∕ NOx and BC ∕ CO are comparable to vehicular emission control standards implemented in January 2017 for gasoline (China 5) and diesel (China V) engines, indicating a reduction of BC emissions within central Beijing, and extending this to a larger area would further reduce total BC concentrations.

Black carbon (BC) forms an important component of particulate matter globally, due to its impact on climate, the environment and human health. Identifying and quantifying its emission sources are critical for effective policymaking and achieving the desired reduction in air pollution. In this study, we present the first direct measurements of urban BC fluxes using eddy covariance. The measurements were made over Beijing within the UK-China Air Pollution and Human Health (APHH) winter 2016 and summer 2017 campaigns. In both seasons, the mean measured BC mass (winter: 5.49 ng m−2 s−1, summer: 6.10 ng m−2 s−1) and number fluxes (winter: 261.25 particles cm−2 s−1, summer: 334.37 particles cm−2 s−1) were similar. Traffic was determined to be the dominant source of the BC fluxes measured during both seasons. The total BC emissions within the 2013 Multi-resolution Emission Inventory for China (MEIC) are on average too high compared to measured fluxes by a factor of 58.8 (winter) and 47.2 (summer). Only a comparison with the MEIC transport sector shows that emissions are also larger (factor of 37.5 in winter and 37.7 in summer) than the measured flux. Emission ratios of BC ∕ NOx and BC ∕ CO are comparable to vehicular emission control standards implemented in January 2017 for gasoline (China 5) and diesel (China V) engines, indicating a reduction of BC emissions within central Beijing, and extending this to a larger area would further reduce total BC concentrations.

Black carbon (BC) forms an important component of particulate matter globally, due to its impact on climate, the environment and human health. Identifying and quantifying its emission sources are critical for effective policymaking and achieving the desired reduction in air pollution. In this study, we present the first direct measurements of urban BC fluxes using eddy covariance. The measurements were made over Beijing within the UK-China Air Pollution and Human Health (APHH) winter 2016 and summer 2017 campaigns. In both seasons, the mean measured BC mass (winter: 5.49 ng m−2 s−1, summer: 6.10 ng m−2 s−1) and number fluxes (winter: 261.25 particles cm−2 s−1, summer: 334.37 particles cm−2 s−1) were similar. Traffic was determined to be the dominant source of the BC fluxes measured during both seasons. The total BC emissions within the 2013 Multi-resolution Emission Inventory for China (MEIC) are on average too high compared to measured fluxes by a factor of 58.8 (winter) and 47.2 (summer). Only a comparison with the MEIC transport sector shows that emissions are also larger (factor of 37.5 in winter and 37.7 in summer) than the measured flux. Emission ratios of BC ∕ NOx and BC ∕ CO are comparable to vehicular emission control standards implemented in January 2017 for gasoline (China 5) and diesel (China V) engines, indicating a reduction of BC emissions within central Beijing, and extending this to a larger area would further reduce total BC concentrations.

Wet scavenging is an efficient pathway for the removal of particulate matter (PM) from the atmosphere. High levels of PM have been a major cause of air pollution in Beijing but have decreased sharply under the Air Pollution Prevention and Control Action Plan launched in 2013. In this study, four years of observations of wet deposition have been conducted using a sequential sampling technique to investigate the detailed variation in chemical components through each rainfall event. We find that the major ions, SO42−, Ca2+, NO3− and NH4+, show significant decreases over the 2013–2017 period (decreasing by 39 %, 35 %, 12 % and 25 %, respectively), revealing the impacts of the Action Plan. An improved sequential sampling method is developed and implemented to estimate the contribution of below-cloud and in-cloud wet deposition over the four-year period. Overall, below-cloud scavenging accounts for between half and two thirds of wet deposition of the four major ions, with the highest contribution for NH4+ at 65 % and lowest for SO42- at 50 %. The contribution of below-cloud scavenging for Ca2+, SO42- and NH4+ decreases from above 50 % in 2014 to below 40 % in 2017. This suggests that the Action Plan has mitigated PM pollution in the surface layer and hence decreased scavenging due to the washout process. In contrast, we find little change in the annual volume weighted average concentration for NO3- where the contribution from below-cloud scavenging remains at ~44 % over the period 2015–2017. While highlighting the importance of different wet scavenging processes, this paper presents a unique new perspective on the effects of the Action Plan and clearly identifies oxidized nitrogen species as a major target for future air pollution controls.

Wet scavenging is an efficient pathway for the removal of particulate matter (PM) from the atmosphere. High levels of PM have been a major cause of air pollution in Beijing but have decreased sharply under the Air Pollution Prevention and Control Action Plan launched in 2013. In this study, four years of observations of wet deposition have been conducted using a sequential sampling technique to investigate the detailed variation in chemical components through each rainfall event. We find that the major ions, SO42−, Ca2+, NO3− and NH4+, show significant decreases over the 2013–2017 period (decreasing by 39 %, 35 %, 12 % and 25 %, respectively), revealing the impacts of the Action Plan. An improved sequential sampling method is developed and implemented to estimate the contribution of below-cloud and in-cloud wet deposition over the four-year period. Overall, below-cloud scavenging accounts for between half and two thirds of wet deposition of the four major ions, with the highest contribution for NH4+ at 65 % and lowest for SO42- at 50 %. The contribution of below-cloud scavenging for Ca2+, SO42- and NH4+ decreases from above 50 % in 2014 to below 40 % in 2017. This suggests that the Action Plan has mitigated PM pollution in the surface layer and hence decreased scavenging due to the washout process. In contrast, we find little change in the annual volume weighted average concentration for NO3- where the contribution from below-cloud scavenging remains at ~44 % over the period 2015–2017. While highlighting the importance of different wet scavenging processes, this paper presents a unique new perspective on the effects of the Action Plan and clearly identifies oxidized nitrogen species as a major target for future air pollution controls.

China implemented strict emission control measures in Beijing and surrounding regions to ensure good air quality during the 2014 Asia-Pacific Economic Cooperation (APEC) summit. We conducted synchronous aerosol particle measurements with two aerosol mass spectrometers at different heights on a meteorological tower in urban Beijing to investigate the variations in particulate composition, sources and size distributions in response to emission controls. Our results show consistently large reductions in secondary inorganic aerosol (SIA) of 61-67% and 51-57%, and in secondary organic aerosol (SOA) of 55% and 37%, at 260 m and ground level, respectively, during the APEC summit. These changes were mainly caused by large reductions in accumulation mode particles and by suppression of the growth of SIA and SOA by a factor of 2-3, which led to blue sky days during APEC commonly referred to as "APEC Blue". We propose a conceptual framework for the evolution of primary and secondary species and highlight the importance of regional atmospheric transport in the formation of severe pollution episodes in Beijing. Our results indicate that reducing the precursors of secondary aerosol over regional scales is crucial and effective in suppressing the formation of secondary particulates and mitigating PM pollution.

China implemented strict emission control measures in Beijing and surrounding regions to ensure good air quality during the 2014 Asia-Pacific Economic Cooperation (APEC) summit. We conducted synchronous aerosol particle measurements with two aerosol mass spectrometers at different heights on a meteorological tower in urban Beijing to investigate the variations in particulate composition, sources and size distributions in response to emission controls. Our results show consistently large reductions in secondary inorganic aerosol (SIA) of 61-67% and 51-57%, and in secondary organic aerosol (SOA) of 55% and 37%, at 260 m and ground level, respectively, during the APEC summit. These changes were mainly caused by large reductions in accumulation mode particles and by suppression of the growth of SIA and SOA by a factor of 2-3, which led to blue sky days during APEC commonly referred to as "APEC Blue". We propose a conceptual framework for the evolution of primary and secondary species and highlight the importance of regional atmospheric transport in the formation of severe pollution episodes in Beijing. Our results indicate that reducing the precursors of secondary aerosol over regional scales is crucial and effective in suppressing the formation of secondary particulates and mitigating PM pollution.

China implemented strict emission control measures in Beijing and surrounding regions to ensure good air quality during the 2014 Asia-Pacific Economic Cooperation (APEC) summit. We conducted synchronous aerosol particle measurements with two aerosol mass spectrometers at different heights on a meteorological tower in urban Beijing to investigate the variations in particulate composition, sources and size distributions in response to emission controls. Our results show consistently large reductions in secondary inorganic aerosol (SIA) of 61-67% and 51-57%, and in secondary organic aerosol (SOA) of 55% and 37%, at 260 m and ground level, respectively, during the APEC summit. These changes were mainly caused by large reductions in accumulation mode particles and by suppression of the growth of SIA and SOA by a factor of 2-3, which led to blue sky days during APEC commonly referred to as "APEC Blue". We propose a conceptual framework for the evolution of primary and secondary species and highlight the importance of regional atmospheric transport in the formation of severe pollution episodes in Beijing. Our results indicate that reducing the precursors of secondary aerosol over regional scales is crucial and effective in suppressing the formation of secondary particulates and mitigating PM pollution.