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What is the spatiotemporal limit of a macroscopic model that describes the optoelectronic interaction at the interface between different media? This fundamental question has become relevant for time-dependent photoemission from solid surfaces using probes that resolve attosecond electron dynamics on an atomic length scale. We address this fundamental question by investigating how ultrafast electron screening affects the infrared field distribution for a noble metal such as Cu(111) at the solid-vacuum interface. Attosecond photoemission delay measurements performed at different angles of incidence of the light allow us to study the detailed spatiotemporal dependence of the electromagnetic field distribution. Surprisingly, comparison with Monte Carlo semiclassical calculations reveals that the macroscopic Fresnel equations still properly describe the observed phase of the IR field on the Cu(111) surface on an atomic length and an attosecond time scale.

We present our attoline which is a versatile attosecond beamline at the Ultrafast Laser Physics Group at ETH Zurich for attosecond spectroscopy in a variety of targets. High-harmonic generation (HHG) in noble gases with an infrared (IR) driving field is employed to generate pulses in the extreme ultraviolet (XUV) spectral regime for XUV-IR cross-correlation measurements. The IR pulse driving the HHG and the pulse involved in the measurements are used in a non-collinear set-up that gives independent access to the different beams. Single attosecond pulses are generated with the polarization gating technique and temporally characterized with attosecond streaking. This attoline contains two target chambers that can be operated simultaneously. A toroidal mirror relay-images the focus from the first chamber into the second one. In the first interaction region a dedicated double-target allows for a simple change between photoelectron/photoion measurements with a time-of-flight spectrometer and transient absorption experiments. Any end station can occupy the second interaction chamber. A surface analysis chamber containing a hemispherical electron analyzer was employed to demonstrate successful operation. Simultaneous RABBITT measurements in two argon jets were recorded for this purpose.

Motivated by the classical picture of heat flow we construct a stationary temperature gradient in a relativistic microscopic transport model. Employing the relativistic Navier-Stokes ansatz we extract the heat conductivity {\kappa} for a massless Boltzmann gas using only binary collisions with isotropic cross sections. We compare the numerical results to analytical expressions from different theories and discuss the final results. The directly extracted value for the heat conductivity can be referred to as a literature reference within the numerical uncertainties., Comment: 8 pages, 5 figures

Motivated by the classical picture of heat flow we construct a stationary temperature gradient in a relativistic microscopic transport model. Employing the relativistic Navier-Stokes ansatz we extract the heat conductivity {\kappa} for a massless Boltzmann gas using only binary collisions with isotropic cross sections. We compare the numerical results to analytical expressions from different theories and discuss the final results. The directly extracted value for the heat conductivity can be referred to as a literature reference within the numerical uncertainties., Comment: 8 pages, 5 figures

The feasibility of attosecond transversal streaking to probe electron transfer dynamics at surfaces and interfaces has been studied. Our simulations suggest that the temporal resolution compares well to existing methods whereas the use of an s-polarized streaking field significantly reduces above-threshold photoemission (ATP) and thus also enables the detection of low-energy electrons.

The feasibility of attosecond transversal streaking to probe electron transfer dynamics at surfaces and interfaces has been studied. Our simulations suggest that the temporal resolution compares well to existing methods whereas the use of an s-polarized streaking field significantly reduces above-threshold photoemission (ATP) and thus also enables the detection of low-energy electrons.

Photoelectron spectroscopy (PES) is a versatile tool, which provides insight into electronic structure and dynamics in condensed matter, surfaces, interfaces and molecules. The history of PES is briefly outlined and illustrated by current developments in the field of time-resolved PES. Our group's research is mostly aimed at studying ultrafast processes and associated lifetimes related to electronic excitation at solid surfaces.