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1. Supported Rh-phosphine complex catalysts for continuous gas-phase decarbonylation of aldehydes.

Author

Malcho P, Garcia-Suarez EJ, Mentzel UV, Engelbrekt C, and Riisager A

Subjects
Aldehydes chemistry, Catalysis, Gases chemistry, Microscopy, Electron, Transmission, Aldehydes metabolism, Coordination Complexes chemistry, Phosphines chemistry, Rhodium chemistry
Abstract

Heterogeneous silica supported rhodium-phosphine complex catalysts are employed for the first time in the catalytic decarbonylation of aldehydes in continuous gas-phase. The reaction protocol is exemplified for the decarbonylation of p-tolualdehyde to toluene and further extended to other aromatic and aliphatic aldehydes achieving excellent results in terms of both conversion and selectivity.

Published
2014
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