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We describe the experimental production of a beam of 23S1 positronium (Ps) atoms obtained from charge-exchange collisions between a positron beam and Xe held in a gas cell. The angular divergence of the emitted Ps beam was recorded using two position sensitive detectors located at different distances from the gas cell. The fraction of the Ps beam produced in the 23S1 level was measured via the change in the Ps count rate after driving the 23S1 → 23P2 transition with microwave radiation; with optimal experimental parameters, we estimate that up to 10% of the Ps beam is formed in the 23S1 state. The measured properties of the beam were used to evaluate the feasibility of using the system for precision spectroscopy of the n = 2 Ps fine structure using Ramsey interferometry., (© 2023 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/).)

We report the results of a new measurement of the positronium 2 ^{3}S_{1}→2 ^{3}P_{2} (ν_{2}) interval. Using a modified experimental arrangement we have significantly reduced the effects of microwave reflections, which in previous experiments resulted in shifts and asymmetric line shapes. With the improved apparatus we obtain an experimental value of ν_{2}=8627.94±0.95  MHz, which is within 1.3σ of the theoretical value 8626.71±0.08  MHz.

We report a new measurement of the positronium (Ps) 2^{3}S_{1}→2^{3}P_{0} interval. Slow Ps atoms, optically excited to the radiatively metastable 2^{3}S_{1} level, flew through a microwave radiation field tuned to drive the transition to the short-lived 2^{3}P_{0} level, which was detected via the time spectrum of subsequent ground state Ps annihilation radiation. After accounting for Zeeman shifts we obtain a transition frequency ν_{0}=18501.02±0.61  MHz, which is not in agreement with the theoretical value of ν_{0}=18498.25±0.08  MHz.

We report experiments in which positronium (Ps) atoms were guided using inhomogeneous electric fields. Ps atoms in Rydberg-Stark states with principal quantum number n=10 and electric dipole moments up to 610 D were prepared via two-color two-photon optical excitation in the presence of a 670  V cm^{-1} electric field. The Ps atoms were created at the entrance of a 0.4 m long electrostatic quadrupole guide, and were detected at the end of the guide via annihilation gamma radiation. When the lasers were tuned to excite low-field-seeking Stark states, a fivefold increase in the number of atoms reaching the end of the guide was observed, whereas no signal was detected when high-field-seeking states were produced. The data are consistent with the calculated geometrical guide acceptance.

We show that the annihilation dynamics of excited positronium (Ps) atoms can be controlled using parallel electric and magnetic fields. To achieve this, Ps atoms were optically excited to n=2 sublevels in fields that were adjusted to control the amount of short-lived and long-lived character of the resulting mixed states. Inclusion of the former offers a practical approach to detection via annihilation radiation, whereas the increased lifetimes due to the latter can be exploited to optimize resonance-enhanced two-photon excitation processes (e.g., 1^{3}S→2^{3}P→nS/nD), either by minimizing losses through intermediate state decay, or by making it possible to separate the excitation laser pulses in time. In addition, photoexcitation of mixed states with a 2^{3}S_{1} component represents an efficient route to producing long-lived pure 2^{3}S_{1} atoms via single-photon excitation.

We describe a pulsed positron beam that is optimised for positronium (Ps) laser-spectroscopy experiments. The system is based on a two-stage Surko-type buffer gas trap that produces 4 ns wide pulses containing up to 5 × 10(5) positrons at a rate of 0.5-10 Hz. By implanting positrons from the trap into a suitable target material, a dilute positronium gas with an initial density of the order of 10(7) cm(-3) is created in vacuum. This is then probed with pulsed (ns) laser systems, where various Ps-laser interactions have been observed via changes in Ps annihilation rates using a fast gamma ray detector. We demonstrate the capabilities of the apparatus and detection methodology via the observation of Rydberg positronium atoms with principal quantum numbers ranging from 11 to 22 and the Stark broadening of the n = 2 → 11 transition in electric fields.

Rydberg positronium (Ps) atoms have been prepared in selected Stark states via two-step (1s→2p→nd/ns) optical excitation. Two methods have been used to achieve Stark-state selection: a field ionization filter that transmits the outermost states with positive Stark shifts, and state-selected photoexcitation in a strong electric field. The former is demonstrated for n=17 and 18 while the latter is performed for n=11 in a homogeneous electric field of 1.9  kV/cm. The observed spectral intensities and their dependence on the polarization of the laser radiation are in agreement with calculations that include the perturbations of the intermediate n=2 manifold. Our results pave the way for the generation of Rydberg Ps atoms with large electric dipole moments that are required for the realization of schemes to control their motion using inhomogeneous electric fields, an essential feature of some proposed Ps free-fall measurements requiring focused beams of long-lived atoms.

We report Doppler-free measurements of the positronium (Ps) Lyman-α transition using saturated absorption spectroscopy. In addition to a Lamb dip at wavelength λ(L) = 243.0218 ± 0.0005 nm, we also observed a crossover resonance at λ(C) = 243.0035 ± 0.0005 nm, arising from the excitation of 1(3)S(1) atoms to Zeeman mixed 2P states, followed by stimulated emission to the 1(1)S(0) ground state. Since (λ(L)-λ(C)) is related to the Ps hyperfine interval E(hfs), this observation constitutes the first optical measurement of this quantity and yields E(hfs) = 198.4 ± 4.2 GHz. We describe improvements to the methodology that could lead to the ∼ppm level of precision required to address the long-standing discrepancy between QED calculations and precision experiments using microwave radiation to induce transitions between Zeeman shifted triplet Ps states.

We report optical spectroscopic measurements of molecular positronium (Ps(2)), performed via a previously unobserved L=1 excited state. Ps(2) molecules created in a porous silica film, and also in vacuum from an Al(111) crystal, were resonantly excited and then photoionized by pulsed lasers, providing conclusive evidence for the production of this molecular matter-antimatter system and its excited state. Future experiments making use of the photoionized vacuum L=1 Ps(2) could provide a source of Ps(+) ions, as well as other multipositronic systems, such as Ps(2)H(-) or Ps(2)O.

We demonstrate experimentally the production of Rydberg positronium (Ps) atoms in a two-step process, comprising incoherent laser excitation, first to the 2(3)P state and then to states with principal quantum numbers ranging from 10 to 25. We find that excitation of 2(3)P atoms to Rydberg levels occurs very efficiently (~90%) and that the ~25% overall efficiency of the production of Rydberg atoms is determined almost entirely by the spectral overlap of the primary excitation laser and the Doppler broadened width of the 1 (3)S-2(3)P transition. The observed efficiency of Rydberg Ps production can be explained if stimulated emission back to the 2P states is suppressed, for example, by intermixing of the Rydberg state Stark sublevels. The efficient production of long-lived Rydberg Ps in a high magnetic field may make it possible to perform direct measurements of the gravitational free fall of Ps.

Slow positrons implanted into a porous silica film may efficiently form positronium (Ps) atoms that diffuse through a network of interconnected pores. At high Ps densities, the long lifetime of ortho-positronium atoms is reduced due to Ps-Ps spin dependent interactions at a rate that implies an effective free-space scattering cross section, σ(e) = (3.4 ± 0.5) × 10(-14) cm(-2), at least 25 times larger than the theoretical value. This enhanced interaction rate may be explained if the quantum confinement of Ps results in interpore tunneling rates that depend critically on the distribution of pore sizes, so that rather than uniformly sampling the porous matrix Ps diffusion is limited to a small subset of the pores.

We have observed that the amount of positronium (Ps) emitted from the surface of p-Si(100) is substantially increased if the sample is irradiated with 532 nm laser light just prior to the implantation of positrons. The energy of the emitted Ps has a constant value of ∼0.16  eV and is independent of the Si temperature and the applied laser fluence, while the photoemission yield depends on both of these parameters. These observations are consistent with Ps production via a previously observed excitonlike positron surface state that is populated in response to the production of electron-hole pairs in the Si. Possible applications of Ps photoemission include probing surface electron dynamics on Si, the generation of ultrashort Ps or positron pulses using ps lasers, and efficient production of Ps in cryogenic environments.

Zeeman mixing of singlet and triplet 2P states of positronium (Ps) atoms, followed by decay back to the ground state, can effectively turn a long-lived triplet atom into a short-lived singlet state, which would seem to preclude laser cooling of Ps in a magnetic field. Here we report experiments which show that, in fact, because of the large splitting of the n=2 states in a high magnetic field (the Paschen-Back regime), the amount of such mixing diminishes approximately exponentially with an increasing magnetic field >0.01  T and is essentially eliminated above ∼2  T. Thus, laser cooling of Ps should be feasible at high fields, which will facilitate the production of a Ps Bose-Einstein condensate.

We describe experiments in which positronium (Ps) is emitted from the surface of p-doped Si(100), following positron implantation. The observed emission rate is proportional to a Boltzmann factor exp{-E(A)/kT}, which is dependent on the temperature T of the sample and a characteristic energy E(A)=(0.253±0.004) eV. Surprisingly, however, the Ps emission energy has a constant value of ∼0.16 eV, much greater than kT. This observation suggests the spontaneous emission of energetic Ps from a short-lived metastable state that becomes thermally accessible to available surface electrons once the positron is present. A likely candidate for this entity is an electron-positron state analogous to the surface exciton observed on p-Si(100) c(4×2) by Weinelt et al. [Phys. Rev. Lett. 92, 126801 (2004)]., (© 2011 American Physical Society)

We report experiments in which the line shape of the Lyman-alpha (1S-2P) transition was measured for positronium (Ps) atoms both inside and outside a porous silica target. The energy interval ΔE for confined atoms was observed to be larger than that of free Ps by 1.26±0.06  meV. A configuration interaction calculation yields results that are consistent with our ∼5  nm sample, and suggests that ΔE decreases dramatically for larger cavity diameters. The linewidth of the transition, (0.066±0.004)  nm (FWHM), is about half of what one would expect for free Ps at room temperature due to the Dicke line narrowing effect of confinement. Such measurements can be used to determine void sizes in porous films and Ps dynamics therein, and elimination of the Doppler spread of atoms in a porous film could be useful for the efficient excitation of a Ps gas.

Long-lived |m|=1 positronium (Ps) atoms are produced in vacuum when high density bursts of positrons with net polarization p{0} are implanted into a porous silica film in a 2.3 T magnetic field. We observe a decrease in the |m|=1 population as the density of the incident positron beam is increased due to quenching interactions between oppositely polarized Ps atoms within the target. Saturation of this density dependent quenching indicates that the initial positron spin polarization p{0}=28+/-1%, and demonstrates the long term (10{2} s) survival of positron polarization in a Surko-type buffer gas trap. We conclude that, at high Ps densities, the minority spin component is essentially eliminated and the remaining Ps is almost entirely (approximately 96%) polarized, as required for the formation of a Ps Bose-Einstein condensate.

Interactions between pairs of positronium (Ps) atoms confined in porous silica films have been directly observed for the first time. Because of selection rules, the nature of such interactions should depend on the structure of the porous medium: if a Ps surface state exists, dipositronium (Ps2) molecules may be created, and if there is a continuum of cavity energy levels, spin exchanging collisions may occur. Using two structurally different silica films, we have been able to isolate and study these two processes. Our data indicate that Ps2 formation occurs primarily via a Langmuir-Hinshelwood-type mechanism on the internal pore surfaces, with an interaction length of the order of 7 x 10(-8) cm, and that the effective cross section for nonthermalized Ps-Ps spin exchange quenching in porous silica is around 9 x 10(-15) cm2.

It has been known for many years that an electron and its antiparticle, the positron, may together form a metastable hydrogen-like atom, known as positronium or Ps (ref. 1). In 1946, Wheeler speculated that two Ps atoms may combine to form the di-positronium molecule (Ps2), with a binding energy of 0.4 eV. More recently, this molecule has been studied theoretically; however, because Ps has a short lifetime and it is difficult to obtain low-energy positrons in large numbers, Ps2 has not previously been observed unambiguously. Here we show that when intense positron bursts are implanted into a thin film of porous silica, Ps2 is created on the internal pore surfaces. We found that molecule formation occurs much more efficiently than the competing process of spin exchange quenching, which appears to be suppressed in the confined pore geometry. This result experimentally confirms the existence of the Ps2 molecule and paves the way for further multi-positronium work. Using similar techniques, but with a more intense positron source, we expect to increase the Ps density to the point where many thousands of atoms interact and can undergo a phase transition to form a Bose-Einstein condensate. As a purely leptonic, macroscopic quantum matter-antimatter system this would be of interest in its own right, but it would also represent a milestone on the path to produce an annihilation gamma-ray laser.

We have created a high-density gas of interacting positronium (Ps) atoms by irradiating a thin film of nanoporous silica with intense positron bursts and measured the Ps lifetime using a new single-shot technique. When the positrons were compressed to 3.3 x 10(10) cm-2, the apparent intensity of the orthopositronium lifetime component was found to decrease by 33%. We believe this is due to a combination of spin exchange quenching and PS2 molecule formation associated with colliding pairs of oppositely polarized triplet positronium atoms. Our data imply an effective cross section for this process of 2.9 x 10(-14) cm-2.

We report the first observation of electron momentum contributions to the Doppler broadening of radiation produced by in-flight two-photon annihilation in solids. In these experiments an approximately 2.5 MeV positron beam impinged on thin polyethylene, aluminum, and gold targets. Since energetic positrons easily penetrate the nuclear Coulomb potential and do not cause a strong charge polarization, the experimental annihilation line shapes agree well with calculations based on a simple independent-particle model. Moreover, annihilations with the deepest core electrons are greatly enhanced.

Background: It has been suggested that left ventricular unloading at the time of reperfusion provides superior infarct salvage over reperfusion alone. The purpose of this study was to show that the Hemopump transvalvular axial-flow left ventricular assist device provides superior left ventricular unloading, ischemic zone collateral blood flow, and infarct size reduction compared with intra-aortic balloon counterpulsation and reperfusion alone., Methods and Results: Eighteen dogs were instrumented with regional myocardial function sonomicrometers in the ischemic and control zones. The left anterior descending coronary artery just distal to the first diagonal branch was instrumented with a silk snare and Doppler flow probe. Additionally, pressure catheters were placed in the left atrial appendage, left ventricular apex, and ascending aorta for hemodynamic measurements. Regional myocardial blood flow was determined by using 15-microns radioactive microspheres. Measurements were made in the control state, immediately after coronary occlusion, at 1 and 2 hours after coronary occlusion, with reperfusion, and 1 hour after reperfusion. In treated animals, left ventricular assistance was maintained during the entire period of occlusion and reperfusion. The Hemopump was associated with a significant decrease in left ventricular systolic and diastolic pressure, whereas mean arterial pressure was maintained. Intra-aortic balloon counterpulsation resulted in no significant changes in left ventricular systolic pressure and a modest decrease in left ventricular diastolic pressure. Regional unloading as assessed by sonomicrometers was significant in the Hemopump animals and absent in the balloon pump animals. Absolute regional myocardial blood flow in the ischemic zone increased slightly (p = 0.002) in the Hemopump animals and did not change in the balloon pump animals. Infarct size expressed as percentage of the zone at risk was 62.6% in the control animals, 27.22% in the balloon pump animals, and 21.7% in the Hemopump animals., Conclusions: Mechanical unloading of the ventricle during ischemia and reperfusion appears to result in significant infarct salvage compared with reperfusion alone. The Hemopump appears to provide superior left ventricular systolic and diastolic unloading compared with intra-aortic counterpulsation in a canine model.

To test the hypothesis that tortuous, diseased vessels could be successfully treated with a flexible rotational atherectomy device we evaluated the BARD atherectomy device with quantitative angiography and histology in normal canine coronary arteries and diseased human below-knee amputation specimens. The mid left anterior descending and the circumflex vessels were treated in 4 dogs serially with 1 wk separating treatments. The acute and follow-up anterior descending artery size was unchanged (1.41 mm before, 1.39 mm after, and 1.59 mm at 1 week). Similar findings were obtained in the circumflex vessels. In 4 adult human amputated legs, diseased peroneal or tibial arteries were treated with a significant reduction in the percent luminal diameter stenosis from 62.75 prior to intervention to 36.5 following intervention (p = 0.021). The luminal diameter increased from 0.81 to 1.54 mm (p = 0.06). In 2 canine arteries there was histologic evidence of localized perforation of the arterial wall, but there was no angiographic evidence of perforation or dissection and no significant myocardial necrosis in the distribution of the treated vessels at 1 wk. The majority of the diseased human vessels demonstrated smoothly cut atheromas with sparing of the media. The rotational atherectomy catheter system holds promise for removal of plaque in relatively small, diffusely diseased, tortuous vessels.

Technetium-99m (Tc-99m) teboroxime is a new perfusion tracer that is highly extracted and rapidly cleared by the myocardium. To determine the feasibility of Tc-99m teboroxime imaging in the diagnosis of patients with suspected coronary artery disease, 30 patients underwent single photon emission computed tomography imaging with Tc-99m teboroxime (25.2 +/- 1 mCi) at peak exercise and again 60 min later at rest. All patients underwent either a thallium stress test (n = 26) or automated quantitative coronary arteriography (n = 25), or both, without intervening revascularization or infarction. Images were reviewed by two investigators who had no knowledge of clinical data. Coronary lesions with greater than or equal to 50% diameter narrowing by quantitative coronary arteriography were considered significant. Both thallium and Tc-99m teboroxime detected disease in all patients with two or three vessel disease. One vessel disease was detected with Tc-99m teboroxime in 9 of 10 patients and with thallium in 8 of 10 (p = NS). In patients without angiographically significant disease. Tc-99m teboroxime demonstrated normal perfusion in six of eight patients and thallium in three of five (p = NS). Overall, when presence or absence of disease detected by Tc-99m teboroxime or thallium was compared with quantitative coronary arteriography, there was no difference between Tc-99m teboroxime and thallium. These results suggest that Tc-99m teboroxime is comparable to thallium as an imaging agent. The rapid biologic half-life, 5.3 min, allows studies to be completed in 60 to 90 min.

Several issues confront the physician treating the patient with an acute infarction. If the patient is a thrombolytic candidate, a 20 to 30 per cent failure rate still exists, and it is difficult to predict on clinical grounds who has had a successful trial of thrombolytics or not; therefore, considerable clinical judgment must be applied. If the patient has relief of pain and diminished ST segment elevation, it is likely that thrombolytic therapy has been successful. Limitations concerning the benefits of thrombolytic or angioplasty therapy for the acute infarction also exist with regard to baseline patient characteristics. Older patients, especially women, seem to have more complications and less beneficial results from acute revascularization than do others. Patients with anterior infarctions as compared with posterior or inferior wall infarctions probably have a higher benefit from intracoronary thrombolysis. The acute myocardial infarction patient can be treated in multiple ways. Based on the preceding information and our own clinical experience, some recommendations can be made. Other sources with their own recommendations are available as well. First, because of the uncertainty still present in deciding optimum therapy for any given patient, as many patients as possible should be included in randomized prospective clinical trials that are now ongoing. If the patient or treating physician elects not to take part in such a trial, much of the therapy will be based on available resources. In small hospitals without acute catheterization or angioplasty facilities, intravenous thrombolytic therapy should be instituted as quickly as possible. In patients who are not able to receive thrombolytic therapy, acute catheterization with consideration for either angioplasty or acute bypass surgery should be undertaken if the patients are relatively young and early on in their course. Treatment of older patients, especially women, should be tempered by the knowledge that there are diminishing returns in aggressive approaches to these patients. It would appear that the presence of cardiogenic shock itself, although a predictor of higher cardiac mortality, should not preclude an aggressive approach and indeed this patient may benefit greatly from revascularization as well as pharmacologic and mechanical support of the cardiovascular system. If thrombolytic therapy without catheterization is undertaken, there remains the potential for either nonrevascularization or early closure.(ABSTRACT TRUNCATED AT 400 WORDS)