Search

In the rapidly evolving field of plasmonic metasurfaces, achieving homogeneous, reliable, and reproducible fabrication of sub-5 nm dielectric nanogaps is a significant challenge. This article presents an advanced fabrication technology that addresses this issue, capable of realizing uniform and reliable vertical nanogap metasurfaces on a whole wafer of 100 mm diameter. By leveraging fast patterning techniques, such as variable-shaped and character projection electron beam lithography (EBL), along with atomic layer deposition (ALD) for defining a few nanometer gaps with sub-nanometer precision, we have developed a flexible nanofabrication technology to achieve gaps as narrow as 2 nm in plasmonic nanoantennas. The quality of our structures is experimentally demonstrated by the observation of resonant localized and collective modes corresponding to the lattice, with Q-factors reaching up to 165. Our technological process opens up new and exciting opportunities to fabricate macroscopic devices harnessing the strong enhancement of light-matter interaction at the single nanometer scale., Competing Interests: Conflict of interest: Authors state no conflicts of interest., (© 2024 the author(s), published by De Gruyter, Berlin/Boston.)

A circularly polarized (CP) beam propagating in a rotated anisotropic material acquires an additional phase delay proportional to the local rotation angle. This phase delay is a particular kind of geometric phase, the Pancharatnam-Berry phase (PBP), stemming from the path of the beam polarization on the Poincaré sphere. A transverse gradient in the geometric phase can thus be imparted by inhomogeneous rotation of the material, with no transverse gradient in the dynamic phase. A waveguide based upon this principle can be induced when the gradient accumulates in propagation, the latter requiring a longitudinal rotation in the optic axis synchronized with the natural rotation of the light polarization. Here, we evaluate numerically and theoretically the robustness of PBP-based waveguides, in the presence of a mismatch between the birefringence length and the external modulation. We find that the mismatch affects mainly the polarization of the quasi-mode, while the confinement is only slightly perturbed.

We investigate experimentally third harmonic generation (THG) from plasmonic metasurfaces consisting of two-dimensional rectangular lattices of centrosymmetric gold nanobars. By varying the incidence angle and the lattice period, we show how surface lattice resonances (SLRs) at the involved wavelengths are the major contributors in determining the magnitude of the nonlinear effects. A further boost on THG is observed when we excite together more than one SLR, either at the same or at different frequency. When such multiple resonances take place, interesting phenomena are observed, such as maximum THG enhancement for counter-propagating surface waves along the metasurface, and cascading effect emulating a third-order nonlinearity.

Second harmonic generation is enhanced at the surface lattice resonance in plasmonic nanoparticle arrays. We carried out a parametric investigation on two-dimensional lattices composed of gold nanobars where the centrosymmetry is broken at oblique incidence. We study the influence of the periodicity, the incidence angle and the direction of the linear input polarization on the second harmonic generation. Excitation of the surface lattice resonance either at the fundamental or second harmonic wavelength, achieved by varying the incidence angle, enhance the conversion efficiency. As a special case, we demonstrate that both the wavelengths can be simultaneously in resonance for a specific period of the lattice. In this double resonant case, maximum second harmonic power is achieved.

The formation of volumetric nanogratings in fused silica by femtosecond laser pulses are shown to afford new opportunities for manipulating the physical shape and tailoring the optical properties of the modification zone by harnessing unconventional beam shapes. The nanograting assembly was observed to rigorously follow the beam elongation effects induced with conical-shaped phase fronts, permitting a scaling up of the writing volume. Detailed optical characterization of birefringence, dichroism, and scattering loss pointed to flexible new ways to tune the macroscopic optical properties, with advantages in decoupling the induced phase retardation from the modification thickness by controlling the conical phase front angle. Further insights into an unexpected asymmetric response from Gaussian beams modified with concave and convex phase fronts have been provided by nonlinear propagation simulations of the shaped-laser light.

We experimentally demonstrate the transverse confinement of light in the presence of a longitudinally periodic photonic potential with vanishing average. In agreement with Kapitza's original findings in classical mechanics, we confirm that light undergoes a transverse localization due to the action of an effective potential proportional to the square of the first derivative of the potential. Experiments are performed based on (1+1) D synthetic dimensions realized in a fiber loop system, allowing for complete control of the transverse and longitudinal distributions of the potential.

We discuss a method to achieve a polarization-independent modulation of the electromagnetic wavefront based upon the Pancharatnam-Berry phase. When the length of the twisted anisotropic material is equal to the birefringence length (i.e., full-wave plate length), a phase delay proportional to the squared transverse derivative of the twisting angle appears. Physically, the phase delay is associated with the Kapitza effect applied to the Pancharatnam-Berry phase. Our theoretical results are confirmed by finite-difference time-domain (FDTD)-based numerical simulations.

We discuss the dynamics of fundamental Gaussian beams launched in saturable and nonlocal nonlinear media. Solely in the presence of a self-focusing saturable nonlinearity, the breathing solitons undergo strong deformation. The addition of a defocusing nonlinearity leads to the generation of couples of solitons. Experimentally, we demonstrate in nematic liquid crystals the formation of multiple spatial solitons starting from a bell-shaped input, with both direction and the number of filaments depending on the input power, confirming the theoretical predictions.

We discuss the effective photonic potential for TM waves in inhomogeneous isotropic media. The model provides an easy and intuitive comprehension of form birefringence, paving the way for a new approach on the design of graded-index optical waveguides on nanometric scales. We investigate the application to nanophotonic devices, including integrated nanoscale wave plates and slot waveguides.

We discuss the role played by time-dependent scattering on light propagation in liquid crystals. In the linear regime, the effects of the molecular disorder accumulate in propagation, yielding a monotonic decrease in the beam spatial coherence. In the nonlinear case, despite the disorder-imposed Brownian-like motion to the self-guided waves, self-focusing increases the spatial coherence of the beam by inducing spatial localization. Eventually, a strong enhancement in the beam oscillations occurs when power is strong enough to induce self-steering, i.e., in the non-perturbative regime.

The topics here deal with some current progress in electromagnetic wave propagation in a family of substances known as metamaterials. To begin with, it is discussed how a pulse can develop a leading edge that steepens and it is emphasised that such self-steepening is an important inclusion within a metamaterial environment together with Raman scattering and third-order dispersion whenever very short pulses are being investigated. It is emphasised that the self-steepening parameter is highly metamaterial-driven compared to Raman scattering, which is associated with a coefficient of the same form whether a normal positive phase, or a metamaterial waveguide is the vehicle for any soliton propagation. It is also shown that the influence of magnetooptics provides a beautiful and important control mechanism for metamaterial devices and that, in the future, this feature will have a significant impact upon the design of data control systems for optical computing. A major objective is fulfiled by the investigations of the fascinating properties of hyperbolic media that exhibit asymmetry of supported modes due to the tilt of optical axes. This is a topic that really merits elaboration because structural and optical asymmetry in optical components that end up manipulating electromagnetic waves is now the foundation of how to operate some of the most successful devices in photonics and electronics. It is pointed out, in this context, that graphene is one of the most famous plasmonic media with very low losses. It is a two-dimensional material that makes the implementation of an effective-medium approximation more feasible. Nonlinear non-stationary diffraction in active planar anisotropic hyperbolic metamaterials is discussed in detail and two approaches are compared. One of them is based on the averaging over a unit cell, while the other one does not include sort of averaging. The formation and propagation of optical spatial solitons in hyperbolic metamaterials is also considered with a model of the response of hyperbolic metamaterials in terms of the homogenisation ('effective medium') approach. The model has a macroscopic dielectric tensor encompassing at least one negative eigenvalue. It is shown that light propagating in the presence of hyperbolic dispersion undergoes negative (anomalous) diffraction. The theory is ten broadened out to include the influence of the orientation of the optical axis with respect to the propagation wave vector. Optical rogue waves are discussed in terms of how they are influenced, but not suppressed, by a metamaterial background. It is strongly discussed that metamaterials and optical rogue waves have both been making headlines in recent years and that they are, separately, large areas of research to study. A brief background of the inevitable linkage of them is considered and important new possibilities are discussed. After this background is revealed some new rogue wave configurations combining the two areas are presented alongside a discussion of the way forward for the future.

We discuss the paraxial approximation for optical waves propagating in a uniaxial anisotropic medium inhomogeneously twisted on the plane normal to the wave vector, with the latter being parallel to one of the two principal axes normal to the optic axis. Such geometry implies a continuous power transfer between the ordinary and extraordinary components, regardless of the input beam polarization. We pinpoint that this peculiar feature, generalizable to any inhomogeneous linear birefringent material, strongly affects the application of the paraxial approximation due to the simultaneous presence of two different phase velocities. We eventually show that a local coordinate transformation permits a correct application of the paraxial approximation.

We investigate nonlinear optical propagation of continuous-wave (CW) beams in bulk nematic liquid crystals. We thoroughly analyze the competing roles of reorientational and thermal nonlinearity with reference to self-focusing/defocusing and, eventually, the formation of nonlinear diffraction-free wavepackets, the so-called spatial optical solitons. To this extent we refer to dye-doped nematic liquid crystals in planar cells excited by a single CW beam in the highly nonlocal limit. To adjust the relative weight between the two nonlinear responses, we employ two distinct wavelengths, inside and outside the absorption band of the dye, respectively. Different concentrations of the dye are considered in order to enhance the thermal effect. The theoretical analysis is complemented by numerical simulations in the highly nonlocal approximation based on a semi-analytic approach. Theoretical results are finally compared to experimental results in the Nematic Liquid Crystals (NLC) 4-trans-4'-n-hexylcyclohexylisothiocyanatobenzene (6CHBT) doped with Sudan Blue dye.

We investigate the inherent influence of light polarization on the intensity distribution in anisotropic media undergoing a local inhomogeneous rotation of the principal axes. Whereas, in general, such a configuration implies a complicated interaction between the geometric and the dynamic phase, we show that, in a medium showing an inhomogeneous circular birefringence, the geometric phase vanishes. Due to the spin-orbit interaction, the two circular polarizations perceive reversed spatial distribution of the dynamic phase. Based on this effect, polarization-selective lenses, waveguides, and beam deflectors are proposed.

We investigate electromagnetic propagation in uniaxial dielectrics with a transversely varying orientation of the optic axis, the latter staying orthogonal everywhere in the propagation direction. In such a geometry, the field experiences no refractive index gradients, yet it acquires a transversely modulated Pancharatnam-Berry phase, that is, a geometric phase originating from a spin-orbit interaction. We show that the periodic evolution of the geometric phase versus propagation gives rise to a longitudinally invariant effective potential. In certain configurations, this geometric phase can provide transverse confinement and waveguiding. The theoretical findings are tested and validated against numerical simulations of the complete Maxwell's equations. Our results introduce and illustrate the role of geometric phases on electromagnetic propagation over distances well exceeding the diffraction length, paving the way to a whole new family of guided waves and waveguides that do not rely on refractive index tailoring.

We investigate the role of competing nonlinear responses in the formation and propagation of bright spatial solitons. We use nematic liquid crystals (NLCs) exhibiting both thermo-optic and reorientational nonlinearities with continuous-wave beams. In a suitably prepared dye-doped sample and dual beam collinear geometry, thermal heating in the visible affects reorientational self-focusing in the near infrared, altering light propagation and self-trapping.

Dynamics and properties of nonlinear matter waves in a trapped BEC subject to a PT-symmetric linear potential, with the trap in the form of a super-Gaussian potential, are investigated via a variational approach accounting for the complex nature of the soliton. In the process, we address how the shape of the imaginary part of the potential, that is, a gain-loss mechanism, affects the self-localization and the stability of the condensate. Variational results are found to be in good agreement with full numerical simulations for predicting the shape, width, and chemical potential of the condensate until the PT breaking point. Variational computation also predicts the existence of solitary solution only above a threshold in the particle number as the gain-loss is increased, in agreement with numerical simulations.

We investigate, both theoretically and experimentally, self-trapping of light beams in nematic liquid crystals arranged so as to exhibit the optical Fréedericksz transition in planar cells. The resulting threshold in the nonlinear reorientational response supports a bistable behavior between diffracting and self-localized beam states, leading to the appearance of a hysteretic loop versus input excitation. Our results confirm the role of nematic liquid crystals in the study of non-perturbative nonlinear photonics.

Refraction at a dielectric interface can take an anomalous character in anisotropic crystals, when light is negatively refracted with incident and refracted beams emerging on the same side of the interface normal. In soft matter subject to reorientation, such as nematic liquid crystals, the nonlinear interaction with light allows tuning of the optical properties. We demonstrate that in such material a beam of light can experience either positive or negative refraction depending on input power, as it can alter the spatial distribution of the optic axis and, in turn, the direction of the energy flow when traveling across an interface. Moreover, the nonlinear optical response yields beam self-focusing and spatial localization into a self-confined solitary wave through the formation of a graded-index waveguide, linking the refractive transition to power-driven readdressing of copolarized guided-wave signals, with a number of output ports not limited by diffraction.

We theoretically investigate light self-trapping in nonlinear dielectrics with a reorientational response subject to threshold, specifically nematic liquid crystals. Beyond a finite excitation, two solitary waves exist for any given power, with an hysteretic dynamics due to feedback between beam size, self-focusing and the nonlinear threshold. Soliton stability is discussed on the basis of the system free energy.

We investigate spatial solitons in nonlocal media with a nonlinear index well modeled by a diffusive equation. We address the role of nonlocality and its interplay with boundary conditions, shedding light on the behavior of accessible solitons in real samples and discussing the accuracy of the highly nonlocal approximation. We find that symmetric solitons exist only above a power threshold, with an existence region that grows larger and larger with nonlocality in the plane width power.

We investigated bistability with light beams in reorientational nematic liquid crystals. For a range of input powers, beams can propagate as either diffracting or self-trapped, the latter corresponding to spatial solitons. The first-order transition in samples exhibiting abrupt self-focusing with a threshold is in agreement with a simple model.

Liquid crystals in the nematic phase exhibit substantial reorientation when the molecules are driven by electric fields of any frequencies. Exploiting such a response at optical frequencies, self-focusing supports transverse localization of light and the propagation of self-confined beams and waveguides, namely "nematicons". Nematicons can guide other light signals and interact with inhomogeneities and other beams. Moreover, they can be effectively deviated by using the electro-optic response of the medium, leading to several strategies for voltage-controlled reconfiguration of light-induced guided-wave circuits and signal readdressing. Hereby, we outline the main features of nematicons and review the outstanding progress achieved in the last twelve years on beam self-trapping and electro-optic readdressing.

We investigate the dynamics of spatial optical solitons launched in a medium with a finite perturbation of the refractive index. For longitudinally short perturbations of super-Gaussian transverse profile, as the input power varies we observe a transition from a wave-like behavior where solitons break up into multiple fringes to a particle-like behavior where solitons acquire a transverse velocity retaining their shape. For longitudinally long perturbations with an attractive potential solitons get trapped inside the well and propagate with transverse periodic oscillations, resulting in an efficient power-dependent angular steering or deflection. Using the Ehrenfest theorem we derive analytical expressions for soliton trajectory, and achieve excellent agreement between theory and numerical simulations for large powers, that is, narrow solitons.

We investigate power-dependent routing of one-dimensional Kerr-like spatial solitons in the presence of a finite photonic potential. Large self-deflections can be obtained using a trapping index well of limited length.

We analyze the angular steering of self-confined light beams, i.e., spatial solitons, in nematic liquid crystals exploiting both their electro-optic response and reorientational nonlinearity. A bias-induced interface is obtained with comb electrodes in a planar cell, applying two distinct voltages to control the spatial distribution of the optic axis. The configuration allows spatial solitons to propagate in a plane and maximize their deflection via refraction and total internal reflection, with an overall deflection of 70° in standard E7., (© 2011 Optical Society of America)

We investigate the attractive interaction between spatial solitons in nematic liquid crystals with a tunable nonlinearity and a constant nonlocality. The experimental study, carried out by controlling the orientation of the optic axis via the electro-optic response, shows how the interactions depend on reorientation, in excellent agreement with a model accounting for the anisotropic nature of the dielectric.

We investigate the propagation of optical solitons interacting with linear defects in the medium. We show that solitons exhibit a wave-particle dualism versus power, i.e., depending on the relative size of soliton and defect, responsible for a soliton trajectory dependent on its waist., (© 2011 Optical Society of America)

We experimentally demonstrate and model dark spatial solitons in azo-doped liquid crystals, in the presence of saturation and nonlocality of the effective nonlinearity due to changes in molecular order. The guiding properties of dark solitons are probed with a weak input of different wavelength.

We theoretically investigate light beam propagation in (1+1)D homogeneous anisotropic uniaxials where ordinary and extraordinary waves are decoupled, accounting for the vectorial character of the electromagnetic field and addressing the nonparaxial limit.

We investigate nonparaxial spatial solitons in uniaxial media with a cubic nonlinearity, accounting for the fully vectorial electromagnetic perturbation and the longitudinal field component in the self-induced index well. We discuss the effective nonlocality arising in purely Kerr media and soliton self-steering owing to nonlinear changes in walk-off.

We model spatial solitons in nematic liquid crystals, accounting for nonperturbative excitation and related effects, such as power-dependent self steering. We also address the interplay between nonlocality and saturation typical of a reorientational medium.

We demonstrate power-dependent steering of self-confined light beams propagating in the nonparaxial regime in a guest-host nonlinear medium. Exploiting the Janossy enhancement in dye-doped liquid crystals with reorientational response, we observe sub-mW spatial soliton self-steering as large as 39 degrees, accompanied by trapping of the light spontaneously emitted by the excited dye. The self-turning is modeled in terms of an effective transverse force stemming from the longitudinal electric field in the tightly confined beams, with good agreement between data and simulations.

We discuss the interactions between self-guided light beams and light-induced perturbations in a liquid crystal light valve. The model and data are in perfect agreement.

A nonlinear phase defect inserted in a coherent coupler can realize an effective all-optical diode. Basic features, design criteria, and suggested implementations are discussed with reference to Kerr-like media.

We investigate, both experimentally and theoretically, the interaction of (2D+1) spatial solitons with the boundaries of a nonlinear medium in the presence of nonlocality. We demonstrate power-dependent nonlinear repulsion at the boundaries, in quantitative agreement with the model predictions.

We investigate the interaction between two beams differing in wavelength and the properties of dual-frequency spatial solitons in nonlocal birefringent reorientational media. We report the first experimental observations of anisotropic nonlocal vector solitons in unbiased nematic liquid crystals. Model and simulations, based on the paraxiality along the Poynting vectors, include joint walk-off and breathing.

We demonstrate that, in suitably designed cells with undoped nematic liquid crystals, extraordinary-wave spatial solitons can be excited at every applied voltage without adjustments in the input polarization. Their walk-off, hence direction of propagation, is externally controlled over angles as large as 7 degrees. The results pave the way not only to polarization-forgiving generation but also to voltage readdressing of these extraordinary-wave nematicons.