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1. 1,3-dipolar cycloadditions of trimethylsilyldiazomethane revisited: Steric demand of the dipolarophile and the influence on product distribution

Author

Simovic, Dragan, Mingping Di, Marks, Vered, and Chatfield, David C.

Subjects
Methane -- Electric properties, Methane -- Chemical properties, Pyrazoles -- Electric properties, Pyrazoles -- Chemical properties, Ring formation (Chemistry) -- Analysis, Biological sciences, Chemistry
Abstract

An investigation of 1,3-dipolar cycloaddition of trimethylsilyldiazomethane with alpha,beta-unsaturated esters is presented. It is demonstrated that the distribution of 2-pyrazoline products is highly dependent on the relative configuration of the substituents on the 1-pyrazoline intermediate.

Published
2007

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