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Multi-qubit systems are crucial for the advancement and application of quantum science. Such systems require maintaining long coherence times while increasing the number of qubits available for coherent manipulation. For solid-state spin systems, qubit coherence is closely related to fundamental questions of many-body spin dynamics. Here we apply a coherent spectroscopic technique to characterize the dynamics of the composite solid-state spin environment of nitrogen-vacancy colour centres in room temperature diamond. We identify a possible new mechanism in diamond for suppression of electronic spin-bath dynamics in the presence of a nuclear spin bath of sufficient concentration. This suppression enhances the efficacy of dynamical decoupling techniques, resulting in increased coherence times for multi-spin-qubit systems, thus paving the way for applications in quantum information, sensing and metrology., Physics

We realize anti-reflection (AR) coatings for optical excitation and fluorescence measurements of nitrogen-vacancy (NV) color centers in bulk diamond by depositing quarter-wavelength thick silica layers on the diamondsurface. These AR coatings improve NV-diamond optical measurements by reducing optical reflection at the diamond-air interface from ≈17% to ≈2%, which allows more effective NV optical excitation and more efficient detection of NV fluorescence. We also show that diamondAR coatings eliminate standing-wave interference patterns of excitation laser intensity within bulk diamond, and thereby greatly reduce spatial variations in NV fluorescence, which can degrade spatially resolved magnetic field sensing using NV centers., Engineering and Applied Sciences, Physics

We use multipulse dynamical decoupling to increase the coherence lifetime (T2) of large numbers of nitrogen-vacancy (NV) electronic spins in room temperature diamond, thus enabling scalable applications of multispin quantum information processing and metrology. We realize an order-of-magnitude extension of the NV multispin T2 in three diamond samples with widely differing spin impurity environments. In particular, for samples with nitrogen impurity concentration ≲1 ppm, we extend T2 to >2 ms, comparable to the longest coherence time reported for single NV centers, and demonstrate a tenfold enhancement in NV multispin sensing of ac magnetic fields., Physics

A common limitation of experiments using color centers in diamond is the poor photon collection efficiency of microscope objectives due to refraction at the diamond interface. We present a simple and effective technique to detect a large fraction of photons emitted by color centers within a planar diamond sample by detecting light that is guided to the edges of the diamond via total internal reflection. We describe a prototype device using this “side-collection” technique, which provides a photon collection efficiency ≈47% and a photon detection efficiency ≈39%. We apply the enhanced signal-to-noise ratio gained from side collection to ac magnetometry using ensembles of nitrogen-vacancy (NV) color centers, and demonstrate an ac magnetic field sensitivity ≈100pT/Hz‾‾‾√, limited by added noise in the prototype side-collection device. Technical optimization should allow significant further improvements in photon collection and detection efficiency as well as subpicotesla NV-diamond magnetic field sensitivity using the side-collection technique., Physics

We demonstrate preferential orientation of nitrogen-vacancy (NV) color centers along two of four possible crystallographic axes in diamonds grown by chemical vapor deposition on the {100} face. We identify the relevant growth regime and present a possible explanation of this effect. We show that preferential orientation provides increased optical readout contrast for NV multispin measurements, including enhanced ac magnetic-field sensitivity, thus providing an important step towards high-fidelity multispin-qubit quantum information processing, sensing, and metrology., Physics