1. Superconductivity under pressure in a chromium-based kagome metal.
- Author
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Liu, Yi, Liu, Zi-Yi, Bao, Jin-Ke, Yang, Peng-Tao, Ji, Liang-Wen, Wu, Si-Qi, Shen, Qin-Xin, Luo, Jun, Yang, Jie, Liu, Ji-Yong, Xu, Chen-Chao, Yang, Wu-Zhang, Chai, Wan-Li, Lu, Jia-Yi, Liu, Chang-Chao, Wang, Bo-Sen, Jiang, Hao, Tao, Qian, Ren, Zhi, and Xu, Xiao-Feng
- Abstract
Superconductivity in a highly correlated kagome system has been theoretically proposed for years (refs. 1–5), yet the experimental realization is hard to achieve6,7. The recently discovered vanadium-based kagome materials8, which exhibit both superconductivity9–11 and charge-density-wave orders12–14, are nonmagnetic8,9 and weakly correlated15,16. Thus these materials are unlikely to host the exotic superconductivity theoretically proposed. Here we report the discovery of a chromium-based kagome metal, CsCr
3 Sb5 , which is contrastingly featured with strong electron correlations, frustrated magnetism and characteristic flat bands close to the Fermi level. Under ambient pressure, this kagome metal undergoes a concurrent structural and magnetic phase transition at 55 K, with a stripe-like 4a0 structural modulation. At high pressure, the phase transition evolves into two transitions, possibly associated with charge-density-wave and antiferromagnetic spin-density-wave orderings. These density-wave-like orders are gradually suppressed with pressure and, remarkably, a superconducting dome emerges at 3.65–8.0 GPa. The maximum of the superconducting transition temperature, Tc max = 6.4 K, appears when the density-wave-like orders are completely suppressed at 4.2 GPa, and the normal state exhibits a non-Fermi-liquid behaviour, reminiscent of unconventional superconductivity and quantum criticality in iron-based superconductors17,18. Our work offers an unprecedented platform for investigating superconductivity in correlated kagome systems.The emergence of superconductivity under pressure is reported in a chromium-based kagome metal, CsCr3 Sb5 , which has strong electron correlations, frustrated magnetism and characteristic flat bands close to the Fermi level. [ABSTRACT FROM AUTHOR]- Published
- 2024
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