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Metasurfaces represent a new frontier in materials science paving for unprecedented methods of controlling electromagnetic waves, with a range of applications spanning from sensing to imaging and communications. For pulsed terahertz (THz) generation, metasurfaces offer a gateway to tuneable thin emitters that can be utilized for large‐area imaging, microscopy, and spectroscopy. In literature, THz‐emitting metasurfaces generally exhibit high absorption, being based either on metals or on semiconductors excited in highly resonant regimes. Here, the use of a fully dielectric semiconductor exploiting morphology‐mediated resonances and inherent quadratic nonlinear response is proposed. This system exhibits a remarkable 40‐fold efficiency enhancement compared to the unpatterned at the peak of the optimized wavelength range, demonstrating its potential as a scalable emitter design. [ABSTRACT FROM AUTHOR]

Laser cavity-solitons can appear in a microresonator-filtered laser when judiciously balancing the slow nonlinearities of the system. Under certain conditions, such optical states can be made to self-emerge and recover spontaneously, and the understanding of their robustness is critical for practical applications. Here, we study the formation of a bonded state comprising a soliton and a blue-detuned continuous wave, whose coexistence is mediated by dispersion in the nonlinear refractive index. Our real-time dispersive Fourier transform measurements, supported by comprehensive theoretical analysis, reveal the presence of an elastic bonding between the two states, resulting in an enhancement of the soliton's robustness. Cavity-solitons in microresonator-filtered fibre lasers are robust states with self-recovery capabilities that emerge when a delicate balance of energy-dependent nonlinearities is achieved. In this work, the authors make use of the dispersive Fourier transform to understand the dynamics leading to a soliton bonded with a quasi-continuous wave. [ABSTRACT FROM AUTHOR]

The strive for efficiency in the generation of terahertz (THz) waves motivates intense research on novel field–matter interactions. Presently, THz generation via quadratic crystals remains the benchmark thanks to its simple and practical deployment. An interesting problem is whether new mechanisms can be exploited to elicit novel generation approaches and forms of control on the THz output in existing systems. THz generation via quantum interference (QI) leverages a third‐order nonlinear response under resonant absorption, and it has been recently explored to access surface generation in centrosymmetric systems. Its deployment in standard THz quadratic sources can potentially create a physical setting with the concurrence of two different mechanisms. Here, THz generation via QI in noncentrosymmetric crystals concurrent with phase‐matched quadratic generation in a bulk‐transmission setting is demonstrated. Beyond investigating a new physical setting, it is demonstrated that conversion efficiencies much larger than those typically associated with the medium become accessible for a typically adopted crystal, ZnTe. An inherent control on the relative amplitude and sign of the two generated THz components is also achieved. This approach provides disruptive boost and management of the optical‐to‐THz conversion performance of a well‐established technology, with significant ramifications in emerging spectroscopy and imaging applications. [ABSTRACT FROM AUTHOR]

Laser cavity-solitons can appear in systems comprised of a nonlinear microcavity nested within an amplifying fiber loop. These states are robust and self-emergent and constitute an attractive class of solitons that are highly suitable for microcomb generation. Here, we present a detailed study of the free-running stability properties of the carrier frequency and repetition rate of single solitons, which are the most suitable states for developing robust ultrafast and high repetition rate comb sources. We achieve free-running fractional stability on both optical carrier and repetition rate (i.e., 48.9 GHz) frequencies on the order of 1 0 − 9 for a 1 s gate time. The repetition rate results compare well with the performance of state-of-the-art (externally driven) microcomb sources, and the carrier frequency stability is in the range of performance typical of modern free-running fiber lasers. Finally, we show that these quantities can be controlled by modulating the laser pump current and the cavity length, providing a path for active locking and long-term stabilization. [ABSTRACT FROM AUTHOR]

The use of dasatinib and nilotinib in the treatment of patients with chronic myeloid leukemia represents a valid therapeutic option for patients resistant or intolerant to imatinib. In this multicentre study, adherence, persistence and efficacy in real life over two years of treatment were evaluated. Adherence to treatment was calculated as the ratio between the dose received and the prescribed dose. The dose received was calculated using pharmacy refill data. The persistence with treatment was calculated as the difference between the end and the beginning of the treatment. Efficacy was assigned as Progression-Free Survival (PFS) and Events-Free Survival (EFS) and represented through the Kaplan-Meier curve. The number of patients analysed was 117, 70 treated with dasatinib and 47 with nilotinib. Adherence to treatment for dasatinib and nilotinib at two years was 0.91 and 0.82 respectively. Persistence at two years was 77% while the PFS was 92% for both drugs in the study. Adherence to the treatment calculated over two years showed a superiority of dasatinib over nilotinib. Nevertheless, the efficacy in terms of PFS and EFS is superimposable between the two drugs in the study. [ABSTRACT FROM AUTHOR]

We theoretically analyze and experimentally demonstrate optical bi-stability and multi-stability in an integrated nonlinear high-order microring resonator filter based on high-index contrast doped silica glass. We use a nonlinear model accounting for both the Kerr and thermal effects to analyze the instability behavior of the coupled-resonator based filter. The model also accurately predicts the multi-stable behavior of the filter when the input frequency is slightly detuned. To understand the role of the intracavity power distribution, we investigate the detuning of the individual rings of the filter from the optical response with a pump–probe experiment. Such a measurement is performed scanning the filter with a low-power probe beam tuned a few free spectral ranges away from the resonance where the pump is coupled. A comprehensive understanding of the relationship between the nonlinear behavior and the intracavity power distribution for the high-order microring resonator filter will help the design and implementation of future all-optical switching systems using this type of filter. [ABSTRACT FROM AUTHOR]

Microcavity-based frequency combs, or 'microcombs'1,2, have enabled many fundamental breakthroughs3–21 through the discovery of temporal cavity-solitons. These self-localized waves, described by the Lugiato–Lefever equation22, are sustained by a background of radiation usually containing 95% of the total power23. Simple methods for their efficient generation and control are currently being investigated to finally establish microcombs as out-of-the-lab tools24. Here, we demonstrate microcomb laser cavity-solitons. Laser cavity-solitons are intrinsically background-free and have underpinned key breakthroughs in semiconductor lasers22,25–28. By merging their properties with the physics of multimode systems29, we provide a new paradigm for soliton generation and control in microcavities. We demonstrate 50-nm-wide bright soliton combs induced at average powers more than one order of magnitude lower than the Lugiato–Lefever soliton power threshold22, measuring a mode efficiency of 75% versus the theoretical limit of 5% for bright Lugiato–Lefever solitons23. Finally, we can tune the repetition rate by well over a megahertz without any active feedback. By nesting a Kerr microresonator in a fibre loop with gain, 50-nm-wide bright microcavity-based soliton combs with a mode efficiency of 75% can be induced at average powers more than one order of magnitude lower than the Lugiato–Lefever soliton power threshold, facilitating real-world applications. [ABSTRACT FROM AUTHOR]

We report the characterization of a balanced ultrafast photodetector. For this purpose, we use a recently developed time-domain laser-based vector network analyzer (VNA) to determine the common-mode rejection ratio (CMRR) of the device under test. This includes the frequency-domain response above the single-mode frequency of the coaxial connector. Although the balanced photodetector has a nominal bandwidth of 43 GHz, it generates voltage pulses with frequency components up to 180 GHz. We obtain a CMRR of better than 30 dB up to 70 GHz and better than 20 dB up to 110 GHz. The laserbased measurements are compared with the measurements using a digital sampling oscilloscope and with the frequency-domain measurements using a conventional VNA. We obtain good agreement between the three techniques with the laser-based method providing the largest measurement bandwidth, although it also constitutes the most complicated characterization setup. [ABSTRACT FROM AUTHOR]

ABSTRACT Ring opening polymerization (ROP) of N-carboxy anhydride (NCA) amino acids presents a rapid way to synthesize high molecular weight polypeptides with different amino acid compositions. The compositional and functional versatility of polypeptides make these materials an attractive choice for biomaterials. The functional performance of polypeptide materials is equally linked to their conformation which is determined by the amino acid sequence in the polymer chains. Here, the interplay between composition and conformation of synthetic polypeptides obtained by NCA polymerization was explored. Various copolypeptides from Glu(Bzl) and Ser(Bzl) were prepared to investigate how polypeptide composition affected the conformation of the resulting copolymer. Polymerization kinetics indicated that the copolymerization of Glu(Bzl) and Ser(Bzl) preferentially yielded alternating copolymers. Both the polydispersity and the conformation of the polypeptides were dependent on the Ser(Bzl) content in the polymer, demonstrating that polypeptide functionalities could be tuned directly by altering the relative amounts of amino acids in the chain. This work presents the first step toward an improved understanding and control over polypeptide conformation through modulating the amino acid composition of the material. Understanding this sequence-functionality relationship is essential to advancing the use of ROP as a technique to design smart polypeptide based materials with specific functions. © 2016 The Authors. Journal of Polymer Science Part A: Polymer Chemistry Published by Wiley Periodicals, Inc. J. Polym. Sci., Part A: Polym. Chem. 2016, 54, 2331-2336 [ABSTRACT FROM AUTHOR]

Recent developments in quantum photonics have initiated the process of bringing photonic-quantumbased systems out-of-the-lab and into real-world applications. As an example, devices to enable the exchange of a cryptographic key secured by the laws of quantum mechanics are already commercially available. In order to further boost this process, the next step is to transfer the results achieved by means of bulky and expensive setups into miniaturized and affordable devices. Integrated quantum photonics is exactly addressing this issue. In this paper, we briefly review the most recent advancements in the generation of quantum states of light on-chip. In particular, we focus on optical microcavities, as they can offer a solution to the problem of low efficiency that is characteristic of the materials typically used in integrated platforms. In addition, we show that specifically designed microcavities can also offer further advantages, such as compatibility with telecom standards (for exploiting existing fibre networks) and quantum memories (necessary to extend the communication distance), as well as giving a longitudinal multimode character for larger information transfer and processing. This last property (i.e., the increased dimensionality of the photon quantum state) is achieved through the ability to generate multiple photon pairs on a frequency comb, corresponding to the microcavity resonances. Further achievements include the possibility of fully exploiting the polarization degree of freedom, even for integrated devices. These results pave the way for the generation of integrated quantum frequency combs that, in turn, may find important applications toward the realization of a compact quantum-computing platform. [ABSTRACT FROM AUTHOR]

The spatial features of a subwavelength terahertz source are not accessible using time-integrated knife-edge (KE) techniques due to the nonseparable space-time nature of the radiated field and to systematic modifications induced by the blade itself. We show that by combining KE with a time-resolved electro-optical sampling, the space-time coupling can be addressed and the source field profile can be exactly reconstructed. [ABSTRACT FROM PUBLISHER]

We demonstrate temporal measurements of sub-picosecond optical pulses via time-to-frequency conversion in a 45-cm-long CMOS compatible high-index glass spiral waveguide. The measurements are based on efficient four-wave mixing in the C-band, using around 1 W of peak pump power. We achieve a resolution of 400 fs over a time window of 100 ps, representing a time-bandwidth product > 250. [ABSTRACT FROM PUBLISHER]

The recent introduction of coherent optical communications has created a compelling need for ultrafast phase-sensitive measurement techniques operating at milliwatt peak power levels and in timescales ranging from sub-picoseconds to nanoseconds. Previous reports of ultrafast optical signal measurements in integrated platforms include time-lens temporal imaging on a silicon chip and waveguide-based frequency-resolved optical gating (FROG). Time-lens imaging is phase-insensitive, and waveguide-based FROG methods require the integration of long tunable delay lines, which is still an unsolved challenge. Here, we report a device capable of characterizing both the amplitude and phase of ultrafast optical pulses with the aid of a synchronized incoherently related clock pulse. It is based on a novel variation of spectral phase interferometry for direct electric-field reconstruction (SPIDER) that exploits degenerate four-wave mixing in a CMOS-compatible chip. We measure pulses with a peak power of <100 mW, a frequency bandwidth of >1 THz, and up to 100 ps pulsewidths, yielding a time-bandwidth product of >100. [ABSTRACT FROM AUTHOR]

Second-harmonic generation is investigated in lithium niobate channels realized by proton exchange and quasi-phase matched by surface periodic poling. The reduction in conversion efficiency at high powers is interpreted in terms of multiphoton absorption via two-color terms, yielding an estimate of the dominating three-photon process. [ABSTRACT FROM AUTHOR]

We demonstrate ultraviolet generation in lithium tantalate channel waveguides for frequency doubling via quasi-phase-matching. The samples, proton exchanged and nanostructured by electric-field assisted surface periodic poling with domains as deep as 40 μm, yield continuous wave light at 365.4 nm with conversion efficiencies larger than 7.5% W-1 cm-2. [ABSTRACT FROM AUTHOR]

We report on light-induced optical tuning of colloidal photonic crystals doped with gold nanoparticles (Au-nps). By resonantly exciting the Au-np surface plasmon absorption with picosecond pulses at 0.53 μm in a standard pump-probe setup, we observed permanent changes in the stop band resonance around 1.7 μm, with blue wavelength shifts as large as 30 nm and associated to a nanoparticle reshaping. Fine tuning was achieved by controlling either the pulse energy or the irradiation time. [ABSTRACT FROM AUTHOR]

Terahertz (THz) imaging is a rapidly emerging field, thanks to many potential applications in diagnostics, manufacturing, medicine and material characterisation. However, the relatively coarse resolution stemming from the large wavelength limits the deployment of THz imaging in micro- and nano-technologies, keeping its potential benefits out-of-reach in many practical scenarios and devices. In this context, single-pixel techniques are a promising alternative to imaging arrays, in particular when targeting subwavelength resolutions. In this work, we discuss the key advantages and practical challenges in the implementation of time-resolved nonlinear ghost imaging (TIMING), an imaging technique combining nonlinear THz generation with time-resolved time-domain spectroscopy detection. We numerically demonstrate the high-resolution reconstruction of semi-transparent samples, and we show how the Walsh–Hadamard reconstruction scheme can be optimised to significantly reduce the reconstruction time. We also discuss how, in sharp contrast with traditional intensity-based ghost imaging, the field detection at the heart of TIMING enables high-fidelity image reconstruction via low numerical-aperture detection. Even more striking—and to the best of our knowledge, an issue never tackled before—the general concept of "resolution" of the imaging system as the "smallest feature discernible" appears to be not well suited to describing the fidelity limits of nonlinear ghost-imaging systems. Our results suggest that the drop in reconstruction accuracy stemming from non-ideal detection conditions is complex and not driven by the attenuation of high-frequency spatial components (i.e., blurring) as in standard imaging. On the technological side, we further show how achieving efficient optical-to-terahertz conversion in extremely short propagation lengths is crucial regarding imaging performance, and we propose low-bandgap semiconductors as a practical framework to obtain THz emission from quasi-2D structures, i.e., structure in which the interaction occurs on a deeply subwavelength scale. Our results establish a comprehensive theoretical and experimental framework for the development of a new generation of terahertz hyperspectral imaging devices. [ABSTRACT FROM AUTHOR]

The reorientational nonlinearity of nematic liquid crystals enables a self-localized spatial soliton and its waveguide to be deflected or destroyed by a control beam propagating across the cell. We demonstrate a simple all-optical readdressing scheme by exploiting the lens-like perturbation induced by an external beam on both a nematicon and a copolarized guided signal of different wavelength. Angular steering as large as 2.2 deg was obtained for control powers as low as 32 mW in the near infrared. [ABSTRACT FROM AUTHOR]

Modern optical systems increasingly rely on complex physical processes that require accessible control to meet target performance characteristics. In particular, advanced light sources, sought for, for example, imaging and metrology, are based on nonlinear optical dynamics whose output properties must often finely match application requirements. However, in these systems, the availability of control parameters (e.g., the optical field shape, as well as propagation medium properties) and the means to adjust them in a versatile manner are usually limited. Moreover, numerically finding the optimal parameter set for such complex dynamics is typically computationally intractable. Here, we use an actively controlled photonic chip to prepare and manipulate patterns of femtosecond optical pulses that give access to an enhanced parameter space in the framework of supercontinuum generation. Taking advantage of machine learning concepts, we exploit this tunable access and experimentally demonstrate the customization of nonlinear interactions for tailoring supercontinuum properties. [ABSTRACT FROM AUTHOR]