1. Biaxial strain tuning of exciton energy and polarization in monolayer WS2.
- Author
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Kourmoulakis, G., Michail, A., Paradisanos, I., Marie, X., Glazov, M. M., Jorissen, B., Covaci, L., Stratakis, E., Papagelis, K., Parthenios, J., and Kioseoglou, G.
- Subjects
CIRCULAR polarization ,OSCILLATOR strengths ,OPTICAL properties ,EXCITON theory - Abstract
We perform micro-photoluminescence and Raman experiments to examine the impact of biaxial tensile strain on the optical properties of WS
2 monolayers. A strong shift on the order of −130 meV per % of strain is observed in the neutral exciton emission at room temperature. Under near-resonant excitation, we measure a monotonic decrease in the circular polarization degree under the applied strain. We experimentally separate the effect of the strain-induced energy detuning and evaluate the pure effect coming from the biaxial strain. The analysis shows that the suppression of the circular polarization degree under the biaxial strain is related to an interplay of energy and polarization relaxation channels as well as to variations in the exciton oscillator strength affecting the long-range exchange interaction. [ABSTRACT FROM AUTHOR]- Published
- 2023
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